Increasing ion yield circular dichroism in femtosecond photoionisation using optimal control theory

We investigate how optimal control theory can be used to improve Circular Dichroism (CD) signals for the A-band of fenchone measured via the photoionization yield upon further excitation. These transitions are electric dipole forbidden to first order, which translates into low population transfer to...

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Bibliographic Details
Main Authors: Basilewitsch, D. (Author), Braun, H. (Author), Koch, C.P (Author), Mondelo-Martell, M. (Author), Reich, D.M (Author)
Format: Article
Language:English
Published: NLM (Medline) 2022
Online Access:View Fulltext in Publisher