Kinetic multi-layer model of aerosol surface and bulk chemistry (KM-SUB): the influence of interfacial transport and bulk diffusion on the oxidation of oleic acid by ozone
We present a novel kinetic multi-layer model that explicitly resolves mass transport and chemical reaction at the surface and in the bulk of aerosol particles (KM-SUB). The model is based on the PRA framework of gas-particle interactions (Pöschl-Rudich-Ammann, 2007), and it includes reversible adsor...
Main Authors: | M. Shiraiwa, C. Pfrang, U. Pöschl |
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Format: | Article |
Language: | English |
Published: |
Copernicus Publications
2010-04-01
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Series: | Atmospheric Chemistry and Physics |
Online Access: | http://www.atmos-chem-phys.net/10/3673/2010/acp-10-3673-2010.pdf |
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