Kinetic multi-layer model of aerosol surface and bulk chemistry (KM-SUB): the influence of interfacial transport and bulk diffusion on the oxidation of oleic acid by ozone

We present a novel kinetic multi-layer model that explicitly resolves mass transport and chemical reaction at the surface and in the bulk of aerosol particles (KM-SUB). The model is based on the PRA framework of gas-particle interactions (Pöschl-Rudich-Ammann, 2007), and it includes reversible adsor...

Full description

Bibliographic Details
Main Authors: M. Shiraiwa, C. Pfrang, U. Pöschl
Format: Article
Language:English
Published: Copernicus Publications 2010-04-01
Series:Atmospheric Chemistry and Physics
Online Access:http://www.atmos-chem-phys.net/10/3673/2010/acp-10-3673-2010.pdf