Stable, active CO2 reduction to formate via redox-modulated stabilization of active sites

Stable electrochemical reduction to formate is still challenging. Here, the authors demonstrate a redox-modulation and active-site stabilization strategy for CO2 to formate conversion over 100 days of continuous operation at 100 mA/cm2 with a cathodic energy efficiency of 70%.

Bibliographic Details
Main Authors: Le Li, Adnan Ozden, Shuyi Guo, F. Pelayo Garcı́a de Arquer, Chuanhao Wang, Mingzhe Zhang, Jin Zhang, Haoyang Jiang, Wei Wang, Hao Dong, David Sinton, Edward H. Sargent, Miao Zhong
Format: Article
Language:English
Published: Nature Publishing Group 2021-09-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-021-25573-9