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02642nam a2200421Ia 4500 |
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10.1103-PhysRevLett.128.153602 |
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220510s2022 CNT 000 0 und d |
| 020 |
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|a 00319007 (ISSN)
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|a Prolonged Orbital Relaxation by Locally Modified Phonon Density of States for the SiV- Center in Nanodiamonds
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| 260 |
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|b American Physical Society
|c 2022
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| 856 |
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|z View Fulltext in Publisher
|u https://doi.org/10.1103/PhysRevLett.128.153602
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|a Coherent quantum systems are a key resource for emerging quantum technology. Solid-state spin systems are of particular importance for compact and scalable devices. However, interaction with the solid-state host degrades the coherence properties. The negatively charged silicon vacancy center in diamond is such an example. While spectral properties are outstanding, with optical coherence protected by the defects symmetry, the spin coherence is susceptible to rapid orbital relaxation limiting the spin dephasing time. A prolongation of the orbital relaxation time is therefore of utmost urgency and has been tackled by operating at very low temperatures or by introducing large strain. However, both methods have significant drawbacks: the former requires use of dilution refrigerators and the latter affects intrinsic symmetries. Here, a novel method is presented to prolong the orbital relaxation with a locally modified phonon density of states in the relevant frequency range, by restricting the diamond host to below 100 nm. Subsequently measured coherent population trapping shows an extended spin dephasing time compared to the phonon-limited time in a pure bulk diamond. The method works at liquid helium temperatures of few Kelvin and in the low-strain regime. © 2022 American Physical Society.
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|a Coherence properties
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|a Dephasing time
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|a Key resources
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|a Nanodiamonds
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|a Orbital relaxation
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|a Phonon density of state
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|a Phonons
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|a Quantum optics
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|a Quantum system
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|a Quantum technologies
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|a Spin dephasing
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|a Spin systems
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|a Spin-s systems
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| 650 |
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|a Superfluid helium
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|a Agafonov, V.N.
|e author
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1 |
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|a Davydov, V.A.
|e author
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1 |
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|a Doherty, M.W.
|e author
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1 |
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|a Fehler, K.G.
|e author
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|a Häußler, S.
|e author
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1 |
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|a Klotz, M.
|e author
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1 |
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|a Kubanek, A.
|e author
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|a Kulikova, L.F.
|e author
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|a Reddy, P.
|e author
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|a Steiger, E.S.
|e author
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|a Waltrich, R.
|e author
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| 773 |
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|t Physical Review Letters
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