Modelling the Effect of Catalysis on Membrane Contactor Mass Transfer Coefficients for Carbon Dioxide Absorption Systems

Modelling the Effect of Catalysis on Membrane Contactor Mass Transfer Coefficients for Carbon Dioxide Absorption Systems

Bibliographic Details
Main Author: Miller, Jacob
Language:English
Published: University of Cincinnati / OhioLINK 2021
Subjects:
Chemical Engineering
Carbonic Anhydrase
Carbon Capture
Equilibrium Reaction
Reaction Diffusion
Pore Diffusion
Carbon Capture Model
Online Access:http://rave.ohiolink.edu/etdc/view?acc_num=ucin1627662756315225
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spelling ndltd-OhioLink-oai-etd.ohiolink.edu-ucin16276627563152252021-10-16T05:25:21Z Modelling the Effect of Catalysis on Membrane Contactor Mass Transfer Coefficients for Carbon Dioxide Absorption Systems Miller, Jacob Chemical Engineering Carbonic Anhydrase Carbon Capture Equilibrium Reaction Reaction Diffusion Pore Diffusion Carbon Capture Model Pore diffusion from a bulk sour gas phase to a bulk potassium carbonate liquid phase was modelled based solely on pore diffusion resistances. This modelling was done for ideal solutions at varying kinetic rates for the carbon dioxide-water reaction as well as various system parameters. The modelling was done utilizing Python and several pre-built libraries such as Scipy and Jax. The model was constructed starting from the original continuity equations combined with Fick’s Law, and numerically solving the resultant system of differential equations. Primarily, two different methods were required to assess systems with and without kinetic reaction-based diffusion resistances. Assuming infinitely fast reaction in all cases allowed the system to be integrated directly, while the system with kinetic resistances required a collocation algorithm to solve. 2021-10-05 English text University of Cincinnati / OhioLINK http://rave.ohiolink.edu/etdc/view?acc_num=ucin1627662756315225 http://rave.ohiolink.edu/etdc/view?acc_num=ucin1627662756315225 unrestricted This thesis or dissertation is protected by copyright: some rights reserved. It is licensed for use under a Creative Commons license. Specific terms and permissions are available from this document's record in the OhioLINK ETD Center.
collection NDLTD
language English
sources NDLTD
topic Chemical Engineering
Carbonic Anhydrase
Carbon Capture
Equilibrium Reaction
Reaction Diffusion
Pore Diffusion
Carbon Capture Model
spellingShingle Chemical Engineering
Carbonic Anhydrase
Carbon Capture
Equilibrium Reaction
Reaction Diffusion
Pore Diffusion
Carbon Capture Model
Miller, Jacob
Modelling the Effect of Catalysis on Membrane Contactor Mass Transfer Coefficients for Carbon Dioxide Absorption Systems
author Miller, Jacob
author_facet Miller, Jacob
author_sort Miller, Jacob
title Modelling the Effect of Catalysis on Membrane Contactor Mass Transfer Coefficients for Carbon Dioxide Absorption Systems
title_short Modelling the Effect of Catalysis on Membrane Contactor Mass Transfer Coefficients for Carbon Dioxide Absorption Systems
title_full Modelling the Effect of Catalysis on Membrane Contactor Mass Transfer Coefficients for Carbon Dioxide Absorption Systems
title_fullStr Modelling the Effect of Catalysis on Membrane Contactor Mass Transfer Coefficients for Carbon Dioxide Absorption Systems
title_full_unstemmed Modelling the Effect of Catalysis on Membrane Contactor Mass Transfer Coefficients for Carbon Dioxide Absorption Systems
title_sort modelling the effect of catalysis on membrane contactor mass transfer coefficients for carbon dioxide absorption systems
publisher University of Cincinnati / OhioLINK
publishDate 2021
url http://rave.ohiolink.edu/etdc/view?acc_num=ucin1627662756315225
work_keys_str_mv AT millerjacob modellingtheeffectofcatalysisonmembranecontactormasstransfercoefficientsforcarbondioxideabsorptionsystems
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