Formation of beads-on-a-string structures during break-up of viscoelastic filaments

Break-up of viscoelastic filaments is pervasive in both nature and technology. If a filament is formed by placing a drop of saliva between a thumb and forefinger and is stretched, the filament's morphology close to break-up corresponds to beads of several sizes interconnected by slender threads...

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Bibliographic Details
Main Authors: Bhat, Pardeep P. (Author), Appathurai, Santosh (Author), Harris, Michael T. (Author), Pasquali, Matteo (Author), McKinley, Gareth H. (Contributor), Basaran, Osman A. (Author)
Other Authors: Massachusetts Institute of Technology. Department of Mechanical Engineering (Contributor)
Format: Article
Language:English
Published: Nature Publishing Group, 2011-05-24T14:07:58Z.
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Online Access:Get fulltext
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100 1 0 |a Bhat, Pardeep P.  |e author 
100 1 0 |a Massachusetts Institute of Technology. Department of Mechanical Engineering  |e contributor 
100 1 0 |a McKinley, Gareth H.  |e contributor 
100 1 0 |a McKinley, Gareth H.  |e contributor 
700 1 0 |a Appathurai, Santosh  |e author 
700 1 0 |a Harris, Michael T.  |e author 
700 1 0 |a Pasquali, Matteo  |e author 
700 1 0 |a McKinley, Gareth H.  |e author 
700 1 0 |a Basaran, Osman A.  |e author 
245 0 0 |a Formation of beads-on-a-string structures during break-up of viscoelastic filaments 
260 |b Nature Publishing Group,   |c 2011-05-24T14:07:58Z. 
856 |z Get fulltext  |u http://hdl.handle.net/1721.1/63090 
520 |a Break-up of viscoelastic filaments is pervasive in both nature and technology. If a filament is formed by placing a drop of saliva between a thumb and forefinger and is stretched, the filament's morphology close to break-up corresponds to beads of several sizes interconnected by slender threads. Although there is general agreement that formation of such beads-on-a-string (BOAS) structures occurs only for viscoelastic fluids, the underlying physics remains unclear and controversial. The physics leading to the formation of BOAS structures is probed by numerical simulation. Computations reveal that viscoelasticity alone does not give rise to a small, satellite bead between two much larger main beads but that inertia is required for its formation. Viscoelasticity, however, enhances the growth of the bead and delays pinch-off, which leads to a relatively long-lived beaded structure. We also show for the first time theoretically that yet smaller, sub-satellite beads can also form as seen in experiments. 
520 |a National Science Foundation (U.S.). ERC-SOPS (EEC-0540855) 
520 |a Nanoscale Interdisciplinary Research Thrust on 'Directed Self-assembly of Suspended Polymer Fibers' (NSF-DMS0506941) 
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655 7 |a Article 
773 |t Nature Physics