Biological-Templating of a Segregating Binary Alloy for Nanowire-Like Phase-Change Materials and Memory

One of the best strategies for achieving faster computers is to mitigate the millisecond-order time delays arising from the transfer and storage of information between silicon- A nd magnetic-based memories. Segregating-binary-alloy (SBA)-type phase-change materials (PCMs), such as gallium antimonide...

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Bibliographic Details
Main Authors: Loke, Desmond K. (Author), Clausen, Griffin J. (Author), Ohmura, Jacqueline F. (Author), Belcher, Angela M. (Author)
Other Authors: Massachusetts Institute of Technology. Department of Materials Science and Engineering (Contributor), Massachusetts Institute of Technology. Department of Biological Engineering (Contributor), Koch Institute for Integrative Cancer Research at MIT (Contributor)
Format: Article
Language:English
Published: American Chemical Society (ACS), 2020-04-23T17:11:35Z.
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Online Access:Get fulltext
LEADER 02178 am a22002293u 4500
001 124837
042 |a dc 
100 1 0 |a Loke, Desmond K.  |e author 
100 1 0 |a Massachusetts Institute of Technology. Department of Materials Science and Engineering  |e contributor 
100 1 0 |a Massachusetts Institute of Technology. Department of Biological Engineering  |e contributor 
100 1 0 |a Koch Institute for Integrative Cancer Research at MIT  |e contributor 
700 1 0 |a Clausen, Griffin J.  |e author 
700 1 0 |a Ohmura, Jacqueline F.  |e author 
700 1 0 |a Belcher, Angela M.  |e author 
245 0 0 |a Biological-Templating of a Segregating Binary Alloy for Nanowire-Like Phase-Change Materials and Memory 
260 |b American Chemical Society (ACS),   |c 2020-04-23T17:11:35Z. 
856 |z Get fulltext  |u https://hdl.handle.net/1721.1/124837 
520 |a One of the best strategies for achieving faster computers is to mitigate the millisecond-order time delays arising from the transfer and storage of information between silicon- A nd magnetic-based memories. Segregating-binary-alloy (SBA)-type phase-change materials (PCMs), such as gallium antimonide-based systems, can store information on 10 ns time scales by using a single memory structure; however, these materials are hindered by the high consumption of energies and undergo elemental segregation around 620 K. Nanowire-like PCMs can achieve low-energy consumption but are often synthesized by vapor-liquid-solid methods above 720 K, which would cause irreversible corruption of SBA-based PCMs. Here we control the morphology, composition, and functionality of SBA-type germanium-tin oxide systems using template-driven nucleation that leverages the electrostatic-binding specificity of the M13 bacteriophage surface. A wirelike PCM was achieved, with controllable and reliable phase-changing signatures, capable of tens of nanoseconds switching times. This approach addresses some of the critical material compositional and structural constraints that currently diminish the utility of PCMs in universal memory systems. 
546 |a en 
655 7 |a Article 
773 |t 10.1021/acsanm.8b01508 
773 |t ACS applied materials & interfaces