Current-induced transition from particle-by-particle to concurrent intercalation in phase-separating battery electrodes
Many battery electrodes contain ensembles of nanoparticles that phase-separate on (de)intercalation. In such electrodes, the fraction of actively intercalating particles directly impacts cycle life: a vanishing population concentrates the current in a small number of particles, leading to current ho...
Main Authors: | Li, Yiyang (Author), El Gabaly, Farid (Author), Bartelt, Norman C. (Author), Sugar, Joshua D. (Author), Fenton, Kyle R. (Author), Cogswell, Daniel A. (Author), Kilcoyne, A. L. David (Author), Tyliszczak, Tolek (Author), Chueh, William C. (Author), Ferguson, Todd Richard (Contributor), Smith, Raymond Barrett (Contributor), Bazant, Martin Z (Contributor) |
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Other Authors: | Massachusetts Institute of Technology. Department of Chemical Engineering (Contributor), Massachusetts Institute of Technology. Department of Mathematics (Contributor), Bazant, Martin Z. (Contributor) |
Format: | Article |
Language: | English |
Published: |
Nature Publishing Group,
2017-08-03T13:59:55Z.
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Subjects: | |
Online Access: | Get fulltext |
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