Impact of the Electronic Band Structure in High-Harmonic Generation Spectra of Solids

• Main Authors: Tancogne-Dejean, Nicolas (Author), Mücke, Oliver D. (Author), Rubio, Angel (Author), Kaertner, Franz X (Contributor)
• Other Authors: Massachusetts Institute of Technology. Research Laboratory of Electronics (Contributor)
• Format: Article
• Language: English
• Published: American Physical Society, 2017-04-06T18:57:40Z.
• Subjects: Article
• Online Access: Get fulltext

An accurate analytic model describing the microscopic mechanism of high-harmonic generation (HHG) in solids is derived. Extensive first-principles simulations within a time-dependent density-functional framework corroborate the conclusions of the model. Our results reveal that (i) the emitted HHG spectra are highly anisotropic and laser-polarization dependent even for cubic crystals; (ii) the harmonic emission is enhanced by the inhomogeneity of the electron-nuclei potential; the yield is increased for heavier atoms; and (iii) the cutoff photon energy is driver-wavelength independent. Moreover, we show that it is possible to predict the laser polarization for optimal HHG in bulk crystals solely from the knowledge of their electronic band structure. Our results pave the way to better control and optimize HHG in solids by engineering their band structure.
European Research Council (Grant ERC-2015-AdG-694097)
European Cooperation in the Field of Scientific and Technical Research (Organization) (Action Grant MP1306)
German Science Foundation. Hamburg Centre for Ultrafast Imaging-Structure, Dynamics and Control of Matter at the Atromic Scale
German Science Foundation (Grant SPP1840 SOLSTICE)