Natural new particle formation at the coastal Antarctic site Neumayer

We measured condensation particle (CP) concentrations and particle size distributions at the coastal Antarctic station Neumayer (70°39´ S, 8°15´ W) during two summer campaigns (from 20 January to 26 March 2012 and 1 February to 30 April 2014) and during the polar night between 12 August and 27 Septe...

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Main Authors: R. Weller, K. Schmidt, K. Teinilä, R. Hillamo
Format: Article
Language:English
Published: Copernicus Publications 2015-10-01
Series:Atmospheric Chemistry and Physics
Online Access:http://www.atmos-chem-phys.net/15/11399/2015/acp-15-11399-2015.pdf
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spelling doaj-eb973ba4df024c7c9717938a14a386b52020-11-24T21:40:57ZengCopernicus PublicationsAtmospheric Chemistry and Physics1680-73161680-73242015-10-011519113991141010.5194/acp-15-11399-2015Natural new particle formation at the coastal Antarctic site NeumayerR. Weller0K. Schmidt1K. Teinilä2R. Hillamo3Alfred Wegener Institute for Polar and Marine Research, Am Handelshafen 12, 27570 Bremerhaven, GermanyAlfred Wegener Institute for Polar and Marine Research, Am Handelshafen 12, 27570 Bremerhaven, GermanyFinnish Meteorological Institute, Erik Palménin aukio 1, 00101 Helsinki, FinlandFinnish Meteorological Institute, Erik Palménin aukio 1, 00101 Helsinki, FinlandWe measured condensation particle (CP) concentrations and particle size distributions at the coastal Antarctic station Neumayer (70°39´ S, 8°15´ W) during two summer campaigns (from 20 January to 26 March 2012 and 1 February to 30 April 2014) and during the polar night between 12 August and 27 September 2014 in the particle diameter (<i>D</i><sub>p</sub>) range from 2.94 to 60.4 nm (2012) and from 6.26 to 212.9 nm (2014). During both summer campaigns we identified all in all 44 new particle formation (NPF) events. From 10 NPF events, particle growth rates could be determined to be around 0.90 ± 0.46 nm h<sup>−1</sup> (mean ± SD; range: 0.4–1.9 nm h<sup>−1</sup>). With the exception of one case, particle growth was generally restricted to the nucleation mode (<i>D</i><sub>p</sub> < 25 nm) and the duration of NPF events was typically around 6.0 ± 1.5 h (mean ± SD; range: 4–9 h). Thus, in the surrounding area of Neumayer, particles did not grow up to sizes required for acting as cloud condensation nuclei. NPF during summer usually occurred in the afternoon in coherence with local photochemistry. During winter, two NPF events could be detected, though showing no ascertainable particle growth. A simple estimation indicated that apart from sulfuric acid, the derived growth rates required other low volatile precursor vapours.http://www.atmos-chem-phys.net/15/11399/2015/acp-15-11399-2015.pdf
collection DOAJ
language English
format Article
sources DOAJ
author R. Weller
K. Schmidt
K. Teinilä
R. Hillamo
spellingShingle R. Weller
K. Schmidt
K. Teinilä
R. Hillamo
Natural new particle formation at the coastal Antarctic site Neumayer
Atmospheric Chemistry and Physics
author_facet R. Weller
K. Schmidt
K. Teinilä
R. Hillamo
author_sort R. Weller
title Natural new particle formation at the coastal Antarctic site Neumayer
title_short Natural new particle formation at the coastal Antarctic site Neumayer
title_full Natural new particle formation at the coastal Antarctic site Neumayer
title_fullStr Natural new particle formation at the coastal Antarctic site Neumayer
title_full_unstemmed Natural new particle formation at the coastal Antarctic site Neumayer
title_sort natural new particle formation at the coastal antarctic site neumayer
publisher Copernicus Publications
series Atmospheric Chemistry and Physics
issn 1680-7316
1680-7324
publishDate 2015-10-01
description We measured condensation particle (CP) concentrations and particle size distributions at the coastal Antarctic station Neumayer (70°39´ S, 8°15´ W) during two summer campaigns (from 20 January to 26 March 2012 and 1 February to 30 April 2014) and during the polar night between 12 August and 27 September 2014 in the particle diameter (<i>D</i><sub>p</sub>) range from 2.94 to 60.4 nm (2012) and from 6.26 to 212.9 nm (2014). During both summer campaigns we identified all in all 44 new particle formation (NPF) events. From 10 NPF events, particle growth rates could be determined to be around 0.90 ± 0.46 nm h<sup>−1</sup> (mean ± SD; range: 0.4–1.9 nm h<sup>−1</sup>). With the exception of one case, particle growth was generally restricted to the nucleation mode (<i>D</i><sub>p</sub> < 25 nm) and the duration of NPF events was typically around 6.0 ± 1.5 h (mean ± SD; range: 4–9 h). Thus, in the surrounding area of Neumayer, particles did not grow up to sizes required for acting as cloud condensation nuclei. NPF during summer usually occurred in the afternoon in coherence with local photochemistry. During winter, two NPF events could be detected, though showing no ascertainable particle growth. A simple estimation indicated that apart from sulfuric acid, the derived growth rates required other low volatile precursor vapours.
url http://www.atmos-chem-phys.net/15/11399/2015/acp-15-11399-2015.pdf
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