Electronic-structural dynamics in graphene

• Main Authors: Isabella Gierz, Andrea Cavalleri
• Format: Article
• Language: English
• Published: AIP Publishing LLC and ACA 2016-09-01
• Series: Structural Dynamics
• Online Access: http://dx.doi.org/10.1063/1.4964777

We review our recent time- and angle-resolved photoemission spectroscopy experiments, which measure the transient electronic structure of optically driven graphene. For pump photon energies in the near infrared ( ℏ ω pump = 950   meV), we have discovered the formation of a population-inverted state near the Dirac point, which may be of interest for the design of THz lasing devices and optical amplifiers. At lower pump photon energies ( ℏ ω pump < 400   meV), for which interband absorption is not possible in doped samples, we find evidence for free carrier absorption. In addition, when mid-infrared pulses are made resonant with an infrared-active in-plane phonon of bilayer graphene ( ℏ ω pump = 200   meV), a transient enhancement of the electron-phonon coupling constant is observed, providing interesting perspective for experiments that report light-enhanced superconductivity in doped fullerites in which a similar lattice mode was excited. All the studies reviewed here have important implications for applications of graphene in optoelectronic devices and for the dynamical engineering of electronic properties with light.