Electrochemical generation of sulfur vacancies in the basal plane of MoS2 for hydrogen evolution

Electrochemical generation of sulfur vacancies in the basal plane of MoS2 for hydrogen evolution

In order to fully utilize sulfur vacancies in MoS2 catalysts for industrial applications, a facile and general route for making sulfur vacancies in MoS2 is needed. Here, the authors introduce a scalable route towards generating sulfur vacancies on the MoS2basal plane using electrochemical desulfuriz...

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Main Authors: Charlie Tsai, Hong Li, Sangwook Park, Joonsuk Park, Hyun Soo Han, Jens K. Nørskov, Xiaolin Zheng, Frank Abild-Pedersen
Format: Article
Language:English
Published: Nature Publishing Group 2017-04-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/ncomms15113
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spelling doaj-d73cd143577f4800abc7aabf1d4be1492021-05-11T07:16:55ZengNature Publishing GroupNature Communications2041-17232017-04-01811810.1038/ncomms15113Electrochemical generation of sulfur vacancies in the basal plane of MoS2 for hydrogen evolutionCharlie Tsai0Hong Li1Sangwook Park2Joonsuk Park3Hyun Soo Han4Jens K. Nørskov5Xiaolin Zheng6Frank Abild-Pedersen7Department of Chemical Engineering, SUNCAT Center for Interface Science and Catalysis, Stanford UniversityDepartment of Mechanical Engineering, Stanford UniversityDepartment of Mechanical Engineering, Stanford UniversityDepartment of Material Science & Engineering, Stanford UniversityDepartment of Mechanical Engineering, Stanford UniversityDepartment of Chemical Engineering, SUNCAT Center for Interface Science and Catalysis, Stanford UniversityDepartment of Mechanical Engineering, Stanford UniversityDepartment of Chemical Engineering, SUNCAT Center for Interface Science and Catalysis, Stanford UniversityIn order to fully utilize sulfur vacancies in MoS2 catalysts for industrial applications, a facile and general route for making sulfur vacancies in MoS2 is needed. Here, the authors introduce a scalable route towards generating sulfur vacancies on the MoS2basal plane using electrochemical desulfurization.https://doi.org/10.1038/ncomms15113
collection DOAJ
language English
format Article
sources DOAJ
author Charlie Tsai
Hong Li
Sangwook Park
Joonsuk Park
Hyun Soo Han
Jens K. Nørskov
Xiaolin Zheng
Frank Abild-Pedersen
spellingShingle Charlie Tsai
Hong Li
Sangwook Park
Joonsuk Park
Hyun Soo Han
Jens K. Nørskov
Xiaolin Zheng
Frank Abild-Pedersen
Electrochemical generation of sulfur vacancies in the basal plane of MoS2 for hydrogen evolution
Nature Communications
author_facet Charlie Tsai
Hong Li
Sangwook Park
Joonsuk Park
Hyun Soo Han
Jens K. Nørskov
Xiaolin Zheng
Frank Abild-Pedersen
author_sort Charlie Tsai
title Electrochemical generation of sulfur vacancies in the basal plane of MoS2 for hydrogen evolution
title_short Electrochemical generation of sulfur vacancies in the basal plane of MoS2 for hydrogen evolution
title_full Electrochemical generation of sulfur vacancies in the basal plane of MoS2 for hydrogen evolution
title_fullStr Electrochemical generation of sulfur vacancies in the basal plane of MoS2 for hydrogen evolution
title_full_unstemmed Electrochemical generation of sulfur vacancies in the basal plane of MoS2 for hydrogen evolution
title_sort electrochemical generation of sulfur vacancies in the basal plane of mos2 for hydrogen evolution
publisher Nature Publishing Group
series Nature Communications
issn 2041-1723
publishDate 2017-04-01
description In order to fully utilize sulfur vacancies in MoS2 catalysts for industrial applications, a facile and general route for making sulfur vacancies in MoS2 is needed. Here, the authors introduce a scalable route towards generating sulfur vacancies on the MoS2basal plane using electrochemical desulfurization.
url https://doi.org/10.1038/ncomms15113
work_keys_str_mv AT charlietsai electrochemicalgenerationofsulfurvacanciesinthebasalplaneofmos2forhydrogenevolution
AT hongli electrochemicalgenerationofsulfurvacanciesinthebasalplaneofmos2forhydrogenevolution
AT sangwookpark electrochemicalgenerationofsulfurvacanciesinthebasalplaneofmos2forhydrogenevolution
AT joonsukpark electrochemicalgenerationofsulfurvacanciesinthebasalplaneofmos2forhydrogenevolution
AT hyunsoohan electrochemicalgenerationofsulfurvacanciesinthebasalplaneofmos2forhydrogenevolution
AT jensknørskov electrochemicalgenerationofsulfurvacanciesinthebasalplaneofmos2forhydrogenevolution
AT xiaolinzheng electrochemicalgenerationofsulfurvacanciesinthebasalplaneofmos2forhydrogenevolution
AT frankabildpedersen electrochemicalgenerationofsulfurvacanciesinthebasalplaneofmos2forhydrogenevolution
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