The ultrafast onset of exciton formation in 2D semiconductors

The formation dynamics of excitons in 2D transition metal dichalcogenides are challenging to probe directly because of their inherently fast timescales. Here, the authors use extremely short optical pulses to excite an electron-hole plasma, and show the formation of 2D excitons in MoS2 on the timesc...

Full description

Bibliographic Details
Main Authors: Chiara Trovatello, Florian Katsch, Nicholas J. Borys, Malte Selig, Kaiyuan Yao, Rocio Borrego-Varillas, Francesco Scotognella, Ilka Kriegel, Aiming Yan, Alex Zettl, P. James Schuck, Andreas Knorr, Giulio Cerullo, Stefano Dal Conte
Format: Article
Language:English
Published: Nature Publishing Group 2020-10-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-020-18835-5
id doaj-d722f91ef5a1425db9505c5f9ee32c0f
record_format Article
spelling doaj-d722f91ef5a1425db9505c5f9ee32c0f2021-05-11T08:30:35ZengNature Publishing GroupNature Communications2041-17232020-10-011111810.1038/s41467-020-18835-5The ultrafast onset of exciton formation in 2D semiconductorsChiara Trovatello0Florian Katsch1Nicholas J. Borys2Malte Selig3Kaiyuan Yao4Rocio Borrego-Varillas5Francesco Scotognella6Ilka Kriegel7Aiming Yan8Alex Zettl9P. James Schuck10Andreas Knorr11Giulio Cerullo12Stefano Dal Conte13Dipartimento di Fisica, Politecnico di MilanoInstitut für Theoretische Physik, Technische Universität BerlinMolecular Foundry, Lawrence Berkeley National LaboratoryInstitut für Theoretische Physik, Technische Universität BerlinMolecular Foundry, Lawrence Berkeley National LaboratoryDipartimento di Fisica, Politecnico di MilanoDipartimento di Fisica, Politecnico di MilanoMolecular Foundry, Lawrence Berkeley National LaboratoryDepartment of Physics, University of California at BerkeleyDepartment of Physics, University of California at BerkeleyMolecular Foundry, Lawrence Berkeley National LaboratoryInstitut für Theoretische Physik, Technische Universität BerlinDipartimento di Fisica, Politecnico di MilanoDipartimento di Fisica, Politecnico di MilanoThe formation dynamics of excitons in 2D transition metal dichalcogenides are challenging to probe directly because of their inherently fast timescales. Here, the authors use extremely short optical pulses to excite an electron-hole plasma, and show the formation of 2D excitons in MoS2 on the timescale of 30 fs.https://doi.org/10.1038/s41467-020-18835-5
collection DOAJ
language English
format Article
sources DOAJ
author Chiara Trovatello
Florian Katsch
Nicholas J. Borys
Malte Selig
Kaiyuan Yao
Rocio Borrego-Varillas
Francesco Scotognella
Ilka Kriegel
Aiming Yan
Alex Zettl
P. James Schuck
Andreas Knorr
Giulio Cerullo
Stefano Dal Conte
spellingShingle Chiara Trovatello
Florian Katsch
Nicholas J. Borys
Malte Selig
Kaiyuan Yao
Rocio Borrego-Varillas
Francesco Scotognella
Ilka Kriegel
Aiming Yan
Alex Zettl
P. James Schuck
Andreas Knorr
Giulio Cerullo
Stefano Dal Conte
The ultrafast onset of exciton formation in 2D semiconductors
Nature Communications
author_facet Chiara Trovatello
Florian Katsch
Nicholas J. Borys
Malte Selig
Kaiyuan Yao
Rocio Borrego-Varillas
Francesco Scotognella
Ilka Kriegel
Aiming Yan
Alex Zettl
P. James Schuck
Andreas Knorr
Giulio Cerullo
Stefano Dal Conte
author_sort Chiara Trovatello
title The ultrafast onset of exciton formation in 2D semiconductors
title_short The ultrafast onset of exciton formation in 2D semiconductors
title_full The ultrafast onset of exciton formation in 2D semiconductors
title_fullStr The ultrafast onset of exciton formation in 2D semiconductors
title_full_unstemmed The ultrafast onset of exciton formation in 2D semiconductors
title_sort ultrafast onset of exciton formation in 2d semiconductors
publisher Nature Publishing Group
series Nature Communications
issn 2041-1723
publishDate 2020-10-01
description The formation dynamics of excitons in 2D transition metal dichalcogenides are challenging to probe directly because of their inherently fast timescales. Here, the authors use extremely short optical pulses to excite an electron-hole plasma, and show the formation of 2D excitons in MoS2 on the timescale of 30 fs.
url https://doi.org/10.1038/s41467-020-18835-5
work_keys_str_mv AT chiaratrovatello theultrafastonsetofexcitonformationin2dsemiconductors
AT floriankatsch theultrafastonsetofexcitonformationin2dsemiconductors
AT nicholasjborys theultrafastonsetofexcitonformationin2dsemiconductors
AT malteselig theultrafastonsetofexcitonformationin2dsemiconductors
AT kaiyuanyao theultrafastonsetofexcitonformationin2dsemiconductors
AT rocioborregovarillas theultrafastonsetofexcitonformationin2dsemiconductors
AT francescoscotognella theultrafastonsetofexcitonformationin2dsemiconductors
AT ilkakriegel theultrafastonsetofexcitonformationin2dsemiconductors
AT aimingyan theultrafastonsetofexcitonformationin2dsemiconductors
AT alexzettl theultrafastonsetofexcitonformationin2dsemiconductors
AT pjamesschuck theultrafastonsetofexcitonformationin2dsemiconductors
AT andreasknorr theultrafastonsetofexcitonformationin2dsemiconductors
AT giuliocerullo theultrafastonsetofexcitonformationin2dsemiconductors
AT stefanodalconte theultrafastonsetofexcitonformationin2dsemiconductors
AT chiaratrovatello ultrafastonsetofexcitonformationin2dsemiconductors
AT floriankatsch ultrafastonsetofexcitonformationin2dsemiconductors
AT nicholasjborys ultrafastonsetofexcitonformationin2dsemiconductors
AT malteselig ultrafastonsetofexcitonformationin2dsemiconductors
AT kaiyuanyao ultrafastonsetofexcitonformationin2dsemiconductors
AT rocioborregovarillas ultrafastonsetofexcitonformationin2dsemiconductors
AT francescoscotognella ultrafastonsetofexcitonformationin2dsemiconductors
AT ilkakriegel ultrafastonsetofexcitonformationin2dsemiconductors
AT aimingyan ultrafastonsetofexcitonformationin2dsemiconductors
AT alexzettl ultrafastonsetofexcitonformationin2dsemiconductors
AT pjamesschuck ultrafastonsetofexcitonformationin2dsemiconductors
AT andreasknorr ultrafastonsetofexcitonformationin2dsemiconductors
AT giuliocerullo ultrafastonsetofexcitonformationin2dsemiconductors
AT stefanodalconte ultrafastonsetofexcitonformationin2dsemiconductors
_version_ 1721450831838969856