Balancing activity, stability and conductivity of nanoporous core-shell iridium/iridium oxide oxygen evolution catalysts

Production of affordable, clean hydrogen relies on efficient oxygen evolution, but improving catalytic performance for the reaction in acidic media is challenging. Here the authors show how tuning the nanoporous morphology of iridium/iridium oxide leads to an improvement in activity/stability, compa...

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Main Authors: Yong-Tae Kim, Pietro Papa Lopes, Shin-Ae Park, A-Yeong Lee, Jinkyu Lim, Hyunjoo Lee, Seoin Back, Yousung Jung, Nemanja Danilovic, Vojislav Stamenkovic, Jonah Erlebacher, Joshua Snyder, Nenad M. Markovic
Format: Article
Language:English
Published: Nature Publishing Group 2017-11-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-017-01734-7
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spelling doaj-d5427b7fcd734a87a027c8ceea76c15c2021-05-11T07:41:52ZengNature Publishing GroupNature Communications2041-17232017-11-01811810.1038/s41467-017-01734-7Balancing activity, stability and conductivity of nanoporous core-shell iridium/iridium oxide oxygen evolution catalystsYong-Tae Kim0Pietro Papa Lopes1Shin-Ae Park2A-Yeong Lee3Jinkyu Lim4Hyunjoo Lee5Seoin Back6Yousung Jung7Nemanja Danilovic8Vojislav Stamenkovic9Jonah Erlebacher10Joshua Snyder11Nenad M. Markovic12Department of Energy System, Pusan National UniversityMaterials Science Division, Argonne National LaboratoryDepartment of Energy System, Pusan National UniversityDepartment of Energy System, Pusan National UniversityDepartment of Chemical and Biomolecular Engineering, Korea Advanced Institute of Science and TechnologyDepartment of Chemical and Biomolecular Engineering, Korea Advanced Institute of Science and TechnologyGraduate School of EEWS, Korea Advanced Institute of Science and TechnologyGraduate School of EEWS, Korea Advanced Institute of Science and TechnologyMaterials Science Division, Argonne National LaboratoryMaterials Science Division, Argonne National LaboratoryDepartment of Materials Science and Engineering, Johns Hopkins UniversityDepartment of Chemical and Biological Engineering, Drexel UniversityMaterials Science Division, Argonne National LaboratoryProduction of affordable, clean hydrogen relies on efficient oxygen evolution, but improving catalytic performance for the reaction in acidic media is challenging. Here the authors show how tuning the nanoporous morphology of iridium/iridium oxide leads to an improvement in activity/stability, compared with conventional iridium-based oxides.https://doi.org/10.1038/s41467-017-01734-7
collection DOAJ
language English
format Article
sources DOAJ
author Yong-Tae Kim
Pietro Papa Lopes
Shin-Ae Park
A-Yeong Lee
Jinkyu Lim
Hyunjoo Lee
Seoin Back
Yousung Jung
Nemanja Danilovic
Vojislav Stamenkovic
Jonah Erlebacher
Joshua Snyder
Nenad M. Markovic
spellingShingle Yong-Tae Kim
Pietro Papa Lopes
Shin-Ae Park
A-Yeong Lee
Jinkyu Lim
Hyunjoo Lee
Seoin Back
Yousung Jung
Nemanja Danilovic
Vojislav Stamenkovic
Jonah Erlebacher
Joshua Snyder
Nenad M. Markovic
Balancing activity, stability and conductivity of nanoporous core-shell iridium/iridium oxide oxygen evolution catalysts
Nature Communications
author_facet Yong-Tae Kim
Pietro Papa Lopes
Shin-Ae Park
A-Yeong Lee
Jinkyu Lim
Hyunjoo Lee
Seoin Back
Yousung Jung
Nemanja Danilovic
Vojislav Stamenkovic
Jonah Erlebacher
Joshua Snyder
Nenad M. Markovic
author_sort Yong-Tae Kim
title Balancing activity, stability and conductivity of nanoporous core-shell iridium/iridium oxide oxygen evolution catalysts
title_short Balancing activity, stability and conductivity of nanoporous core-shell iridium/iridium oxide oxygen evolution catalysts
title_full Balancing activity, stability and conductivity of nanoporous core-shell iridium/iridium oxide oxygen evolution catalysts
title_fullStr Balancing activity, stability and conductivity of nanoporous core-shell iridium/iridium oxide oxygen evolution catalysts
title_full_unstemmed Balancing activity, stability and conductivity of nanoporous core-shell iridium/iridium oxide oxygen evolution catalysts
title_sort balancing activity, stability and conductivity of nanoporous core-shell iridium/iridium oxide oxygen evolution catalysts
publisher Nature Publishing Group
series Nature Communications
issn 2041-1723
publishDate 2017-11-01
description Production of affordable, clean hydrogen relies on efficient oxygen evolution, but improving catalytic performance for the reaction in acidic media is challenging. Here the authors show how tuning the nanoporous morphology of iridium/iridium oxide leads to an improvement in activity/stability, compared with conventional iridium-based oxides.
url https://doi.org/10.1038/s41467-017-01734-7
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