A fast and easy-to-implement inversion algorithm for mobility particle size spectrometers considering particle number size distribution information outside of the detection range

Multiple-charge inversion is an essential procedure to convert the raw mobility distributions recorded by mobility particle size spectrometers, such as the DMPS or SMPS (differential or scanning mobility particle sizers), into true particle number size distributions. In this work, we present a fast...

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Main Authors: S. Pfeifer, W. Birmili, A. Schladitz, T. Müller, A. Nowak, A. Wiedensohler
Format: Article
Language:English
Published: Copernicus Publications 2014-01-01
Series:Atmospheric Measurement Techniques
Online Access:http://www.atmos-meas-tech.net/7/95/2014/amt-7-95-2014.pdf
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spelling doaj-c746008a0328408b9c7c87d7fef430902020-11-24T20:43:42ZengCopernicus PublicationsAtmospheric Measurement Techniques1867-13811867-85482014-01-01719510510.5194/amt-7-95-2014A fast and easy-to-implement inversion algorithm for mobility particle size spectrometers considering particle number size distribution information outside of the detection rangeS. Pfeifer0W. Birmili1A. Schladitz2T. Müller3A. Nowak4A. Wiedensohler5Leibniz Institute for Tropospheric Research, Permoserstraße 15, 04318 Leipzig, GermanyLeibniz Institute for Tropospheric Research, Permoserstraße 15, 04318 Leipzig, GermanyLeibniz Institute for Tropospheric Research, Permoserstraße 15, 04318 Leipzig, GermanyLeibniz Institute for Tropospheric Research, Permoserstraße 15, 04318 Leipzig, GermanyLeibniz Institute for Tropospheric Research, Permoserstraße 15, 04318 Leipzig, GermanyLeibniz Institute for Tropospheric Research, Permoserstraße 15, 04318 Leipzig, GermanyMultiple-charge inversion is an essential procedure to convert the raw mobility distributions recorded by mobility particle size spectrometers, such as the DMPS or SMPS (differential or scanning mobility particle sizers), into true particle number size distributions. In this work, we present a fast and easy-to-implement multiple-charge inversion algorithm with sufficient precision for atmospheric conditions, but extended functionality. The algorithm can incorporate size distribution information from sensors that measure beyond the upper sizing limit of the mobility spectrometer, such as an aerodynamic particle sizer (APS) or an optical particle counter (OPC). This feature can considerably improve the multiple-charge inversion result in the upper size range of the mobility spectrometer, for example, when substantial numbers of coarse particles are present. The program also yields a continuous size distribution from both sensors as an output. The algorithm is able to calculate the propagation of measurement errors, such as those based on counting statistics, into on the final particle number size distribution. As an additional aspect, the algorithm can perform all inversion steps under the assumption of non-spherical particle shape, including constant or size-dependent shape factors.http://www.atmos-meas-tech.net/7/95/2014/amt-7-95-2014.pdf
collection DOAJ
language English
format Article
sources DOAJ
author S. Pfeifer
W. Birmili
A. Schladitz
T. Müller
A. Nowak
A. Wiedensohler
spellingShingle S. Pfeifer
W. Birmili
A. Schladitz
T. Müller
A. Nowak
A. Wiedensohler
A fast and easy-to-implement inversion algorithm for mobility particle size spectrometers considering particle number size distribution information outside of the detection range
Atmospheric Measurement Techniques
author_facet S. Pfeifer
W. Birmili
A. Schladitz
T. Müller
A. Nowak
A. Wiedensohler
author_sort S. Pfeifer
title A fast and easy-to-implement inversion algorithm for mobility particle size spectrometers considering particle number size distribution information outside of the detection range
title_short A fast and easy-to-implement inversion algorithm for mobility particle size spectrometers considering particle number size distribution information outside of the detection range
title_full A fast and easy-to-implement inversion algorithm for mobility particle size spectrometers considering particle number size distribution information outside of the detection range
title_fullStr A fast and easy-to-implement inversion algorithm for mobility particle size spectrometers considering particle number size distribution information outside of the detection range
title_full_unstemmed A fast and easy-to-implement inversion algorithm for mobility particle size spectrometers considering particle number size distribution information outside of the detection range
title_sort fast and easy-to-implement inversion algorithm for mobility particle size spectrometers considering particle number size distribution information outside of the detection range
publisher Copernicus Publications
series Atmospheric Measurement Techniques
issn 1867-1381
1867-8548
publishDate 2014-01-01
description Multiple-charge inversion is an essential procedure to convert the raw mobility distributions recorded by mobility particle size spectrometers, such as the DMPS or SMPS (differential or scanning mobility particle sizers), into true particle number size distributions. In this work, we present a fast and easy-to-implement multiple-charge inversion algorithm with sufficient precision for atmospheric conditions, but extended functionality. The algorithm can incorporate size distribution information from sensors that measure beyond the upper sizing limit of the mobility spectrometer, such as an aerodynamic particle sizer (APS) or an optical particle counter (OPC). This feature can considerably improve the multiple-charge inversion result in the upper size range of the mobility spectrometer, for example, when substantial numbers of coarse particles are present. The program also yields a continuous size distribution from both sensors as an output. The algorithm is able to calculate the propagation of measurement errors, such as those based on counting statistics, into on the final particle number size distribution. As an additional aspect, the algorithm can perform all inversion steps under the assumption of non-spherical particle shape, including constant or size-dependent shape factors.
url http://www.atmos-meas-tech.net/7/95/2014/amt-7-95-2014.pdf
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