Probing the Wave Function and Dynamics of the Quintet Multiexciton State with Coherent Control in a Singlet Fission Material
High-spin states play a key role in chemical reactions found in nature. In artificial molecular systems, singlet fission produces a correlated triplet-pair state, a spin-bearing excited state that can be harnessed for more efficient solar-energy conversion and photocatalysis. In particular, triplet-...
Main Authors: | , , , , , , |
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Format: | Article |
Language: | English |
Published: |
American Physical Society
2020-06-01
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Series: | Physical Review X |
Online Access: | http://doi.org/10.1103/PhysRevX.10.021070 |