Probing the Wave Function and Dynamics of the Quintet Multiexciton State with Coherent Control in a Singlet Fission Material

High-spin states play a key role in chemical reactions found in nature. In artificial molecular systems, singlet fission produces a correlated triplet-pair state, a spin-bearing excited state that can be harnessed for more efficient solar-energy conversion and photocatalysis. In particular, triplet-...

Full description

Bibliographic Details
Main Authors: S. L. Bayliss, L. R. Weiss, F. Kraffert, D. B. Granger, J. E. Anthony, J. Behrends, R. Bittl
Format: Article
Language:English
Published: American Physical Society 2020-06-01
Series:Physical Review X
Online Access:http://doi.org/10.1103/PhysRevX.10.021070