Identification of molecular cluster evaporation rates, cluster formation enthalpies and entropies by Monte Carlo method

Identification of molecular cluster evaporation rates, cluster formation enthalpies and entropies by Monte Carlo method

<p>We address the problem of identifying the evaporation rates for neutral molecular clusters from synthetic (computer-simulated) cluster concentrations. We applied Bayesian parameter estimation using a Markov chain Monte Carlo (MCMC) algorithm to determine cluster evaporation/fragmentation ra...

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Bibliographic Details
Main Authors:	A. Shcherbacheva, T. Balehowsky, J. Kubečka, T. Olenius, T. Helin, H. Haario, M. Laine, T. Kurtén, H. Vehkamäki
Format:	Article
Language:	English
Published:	Copernicus Publications 2020-12-01
Series:	Atmospheric Chemistry and Physics
Online Access:	https://acp.copernicus.org/articles/20/15867/2020/acp-20-15867-2020.pdf

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