Magnetic properties of a LuVO3 single crystal studied by magnetometry, heat capacity and neutron diffraction

We have studied the magnetic properties of a LuVO3 single crystal. The compound shows an orbital ordering at TOO = 179 K followed by the antiferromagnetic spin ordering at TSO = 109 K. In the magnetically ordered regime, there appears an abrupt change at To = 82.5 K in the magnetisation, indicating...

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Main Authors: L.D. Tung, J. Schefer, M.R. Lees, G. Balakrishnan, D.McK. Paul
Format: Article
Language:English
Published: Elsevier 2016-06-01
Series:Journal of Science: Advanced Materials and Devices
Subjects:
Online Access:http://www.sciencedirect.com/science/article/pii/S2468217916300727
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spelling doaj-b6ce4f7d0e734c159f9b79e9a055ae252020-11-24T23:04:17ZengElsevierJournal of Science: Advanced Materials and Devices2468-21792016-06-011217417810.1016/j.jsamd.2016.06.013Magnetic properties of a LuVO3 single crystal studied by magnetometry, heat capacity and neutron diffractionL.D. Tung0J. Schefer1M.R. Lees2G. Balakrishnan3D.McK. Paul4Department of Physics, University College London, Gower Street, London WC1E 6BT, United KingdomLaboratory for Neutron Scattering and Imaging, Paul Scherrer Institute, CH-5232 Villigen PSI, SwitzerlandDepartment of Physics, University of Warwick, Coventry CV4 7AL, United KingdomDepartment of Physics, University of Warwick, Coventry CV4 7AL, United KingdomDepartment of Physics, University of Warwick, Coventry CV4 7AL, United KingdomWe have studied the magnetic properties of a LuVO3 single crystal. The compound shows an orbital ordering at TOO = 179 K followed by the antiferromagnetic spin ordering at TSO = 109 K. In the magnetically ordered regime, there appears an abrupt change at To = 82.5 K in the magnetisation, indicating a first-order transition. The compound has very large negative Weiss temperature observed along all the main crystallographic axes, suggesting a strong antiferromagnetic correlations in the paramagnetic state. The observation of hysteresis curves in the collinear antiferromagnetic regime is discussed in terms of an inhomogeneity generating some spins with weak local fields in a strongly antiferromagnetic matrix.http://www.sciencedirect.com/science/article/pii/S2468217916300727Magnetic materialsSpin orbital orderAntiferromagnetsDisorder materialsHeat capacity
collection DOAJ
language English
format Article
sources DOAJ
author L.D. Tung
J. Schefer
M.R. Lees
G. Balakrishnan
D.McK. Paul
spellingShingle L.D. Tung
J. Schefer
M.R. Lees
G. Balakrishnan
D.McK. Paul
Magnetic properties of a LuVO3 single crystal studied by magnetometry, heat capacity and neutron diffraction
Journal of Science: Advanced Materials and Devices
Magnetic materials
Spin orbital order
Antiferromagnets
Disorder materials
Heat capacity
author_facet L.D. Tung
J. Schefer
M.R. Lees
G. Balakrishnan
D.McK. Paul
author_sort L.D. Tung
title Magnetic properties of a LuVO3 single crystal studied by magnetometry, heat capacity and neutron diffraction
title_short Magnetic properties of a LuVO3 single crystal studied by magnetometry, heat capacity and neutron diffraction
title_full Magnetic properties of a LuVO3 single crystal studied by magnetometry, heat capacity and neutron diffraction
title_fullStr Magnetic properties of a LuVO3 single crystal studied by magnetometry, heat capacity and neutron diffraction
title_full_unstemmed Magnetic properties of a LuVO3 single crystal studied by magnetometry, heat capacity and neutron diffraction
title_sort magnetic properties of a luvo3 single crystal studied by magnetometry, heat capacity and neutron diffraction
publisher Elsevier
series Journal of Science: Advanced Materials and Devices
issn 2468-2179
publishDate 2016-06-01
description We have studied the magnetic properties of a LuVO3 single crystal. The compound shows an orbital ordering at TOO = 179 K followed by the antiferromagnetic spin ordering at TSO = 109 K. In the magnetically ordered regime, there appears an abrupt change at To = 82.5 K in the magnetisation, indicating a first-order transition. The compound has very large negative Weiss temperature observed along all the main crystallographic axes, suggesting a strong antiferromagnetic correlations in the paramagnetic state. The observation of hysteresis curves in the collinear antiferromagnetic regime is discussed in terms of an inhomogeneity generating some spins with weak local fields in a strongly antiferromagnetic matrix.
topic Magnetic materials
Spin orbital order
Antiferromagnets
Disorder materials
Heat capacity
url http://www.sciencedirect.com/science/article/pii/S2468217916300727
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