Catalysis of Organic Pollutants Abatement Based on Pt-Decorated Ag@Cu<sub>2</sub>O Heterostructures
Pt-decorated Ag@Cu<sub>2</sub>O heterostructures were successfully synthesized using a simple and convenient method. The Pt nanoparticle density on the Ag@Cu<sub>2</sub>O can be controlled by changing the concentration of the Pt precursor. The synthesized Ag@Cu<sub>2<...
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doaj-b2edd825bb3d4c09beaf115ea9c17eb72020-11-24T21:51:18ZengMDPI AGMolecules1420-30492019-07-012415272110.3390/molecules24152721molecules24152721Catalysis of Organic Pollutants Abatement Based on Pt-Decorated Ag@Cu<sub>2</sub>O HeterostructuresXiaolong Zhang0Bingbing Han1Yaxin Wang2Yang Liu3Lei Chen4Yongjun Zhang5Key Laboratory of Functional Materials Physics and Chemistry of the Ministry of Education, Jilin Normal University, Changchun 130103, ChinaKey Laboratory of Functional Materials Physics and Chemistry of the Ministry of Education, Jilin Normal University, Changchun 130103, ChinaKey Laboratory of Functional Materials Physics and Chemistry of the Ministry of Education, Jilin Normal University, Changchun 130103, ChinaKey Laboratory of Functional Materials Physics and Chemistry of the Ministry of Education, Jilin Normal University, Changchun 130103, ChinaKey Laboratory of Functional Materials Physics and Chemistry of the Ministry of Education, Jilin Normal University, Changchun 130103, ChinaKey Laboratory of Functional Materials Physics and Chemistry of the Ministry of Education, Jilin Normal University, Changchun 130103, ChinaPt-decorated Ag@Cu<sub>2</sub>O heterostructures were successfully synthesized using a simple and convenient method. The Pt nanoparticle density on the Ag@Cu<sub>2</sub>O can be controlled by changing the concentration of the Pt precursor. The synthesized Ag@Cu<sub>2</sub>O−Pt nanoparticles exhibited excellent catalytic performance, which was greatly affected by changes in the Ag@Cu<sub>2</sub>O−Pt structure. To optimize the material’s properties, the synthesized Ag@Cu<sub>2</sub>O−Pt nanoparticles were used to catalyze toxic pollutants and methyl orange (MO), and nontoxic products were obtained by catalytic reduction. The Pt-decorated Ag@Cu<sub>2</sub>O nanoparticles showed excellent catalytic activity, which significantly decreased the pollutant concentration when the nanoparticles were used for catalytic reduction. The redistribution of charge transfer is the nanoparticles’ main contribution to the catalytic degradation of an organic pollutant. This Pt-decorated Ag@Cu<sub>2</sub>O material has unique optical and structural characteristics that make it suitable for photocatalysis, local surface plasmon resonance, and peroxide catalysis.https://www.mdpi.com/1420-3049/24/15/2721catalysisAg@Cu<sub>2</sub>O–Ptorganic pollutants |
collection |
DOAJ |
language |
English |
format |
Article |
sources |
DOAJ |
author |
Xiaolong Zhang Bingbing Han Yaxin Wang Yang Liu Lei Chen Yongjun Zhang |
spellingShingle |
Xiaolong Zhang Bingbing Han Yaxin Wang Yang Liu Lei Chen Yongjun Zhang Catalysis of Organic Pollutants Abatement Based on Pt-Decorated Ag@Cu<sub>2</sub>O Heterostructures Molecules catalysis Ag@Cu<sub>2</sub>O–Pt organic pollutants |
author_facet |
Xiaolong Zhang Bingbing Han Yaxin Wang Yang Liu Lei Chen Yongjun Zhang |
author_sort |
Xiaolong Zhang |
title |
Catalysis of Organic Pollutants Abatement Based on Pt-Decorated Ag@Cu<sub>2</sub>O Heterostructures |
title_short |
Catalysis of Organic Pollutants Abatement Based on Pt-Decorated Ag@Cu<sub>2</sub>O Heterostructures |
title_full |
Catalysis of Organic Pollutants Abatement Based on Pt-Decorated Ag@Cu<sub>2</sub>O Heterostructures |
title_fullStr |
Catalysis of Organic Pollutants Abatement Based on Pt-Decorated Ag@Cu<sub>2</sub>O Heterostructures |
title_full_unstemmed |
Catalysis of Organic Pollutants Abatement Based on Pt-Decorated Ag@Cu<sub>2</sub>O Heterostructures |
title_sort |
catalysis of organic pollutants abatement based on pt-decorated ag@cu<sub>2</sub>o heterostructures |
publisher |
MDPI AG |
series |
Molecules |
issn |
1420-3049 |
publishDate |
2019-07-01 |
description |
Pt-decorated Ag@Cu<sub>2</sub>O heterostructures were successfully synthesized using a simple and convenient method. The Pt nanoparticle density on the Ag@Cu<sub>2</sub>O can be controlled by changing the concentration of the Pt precursor. The synthesized Ag@Cu<sub>2</sub>O−Pt nanoparticles exhibited excellent catalytic performance, which was greatly affected by changes in the Ag@Cu<sub>2</sub>O−Pt structure. To optimize the material’s properties, the synthesized Ag@Cu<sub>2</sub>O−Pt nanoparticles were used to catalyze toxic pollutants and methyl orange (MO), and nontoxic products were obtained by catalytic reduction. The Pt-decorated Ag@Cu<sub>2</sub>O nanoparticles showed excellent catalytic activity, which significantly decreased the pollutant concentration when the nanoparticles were used for catalytic reduction. The redistribution of charge transfer is the nanoparticles’ main contribution to the catalytic degradation of an organic pollutant. This Pt-decorated Ag@Cu<sub>2</sub>O material has unique optical and structural characteristics that make it suitable for photocatalysis, local surface plasmon resonance, and peroxide catalysis. |
topic |
catalysis Ag@Cu<sub>2</sub>O–Pt organic pollutants |
url |
https://www.mdpi.com/1420-3049/24/15/2721 |
work_keys_str_mv |
AT xiaolongzhang catalysisoforganicpollutantsabatementbasedonptdecoratedagcusub2suboheterostructures AT bingbinghan catalysisoforganicpollutantsabatementbasedonptdecoratedagcusub2suboheterostructures AT yaxinwang catalysisoforganicpollutantsabatementbasedonptdecoratedagcusub2suboheterostructures AT yangliu catalysisoforganicpollutantsabatementbasedonptdecoratedagcusub2suboheterostructures AT leichen catalysisoforganicpollutantsabatementbasedonptdecoratedagcusub2suboheterostructures AT yongjunzhang catalysisoforganicpollutantsabatementbasedonptdecoratedagcusub2suboheterostructures |
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1725879205255708672 |