Catalysis of Organic Pollutants Abatement Based on Pt-Decorated Ag@Cu<sub>2</sub>O Heterostructures

Pt-decorated Ag@Cu<sub>2</sub>O heterostructures were successfully synthesized using a simple and convenient method. The Pt nanoparticle density on the Ag@Cu<sub>2</sub>O can be controlled by changing the concentration of the Pt precursor. The synthesized Ag@Cu<sub>2<...

Full description

Bibliographic Details
Main Authors: Xiaolong Zhang, Bingbing Han, Yaxin Wang, Yang Liu, Lei Chen, Yongjun Zhang
Format: Article
Language:English
Published: MDPI AG 2019-07-01
Series:Molecules
Subjects:
Online Access:https://www.mdpi.com/1420-3049/24/15/2721
id doaj-b2edd825bb3d4c09beaf115ea9c17eb7
record_format Article
spelling doaj-b2edd825bb3d4c09beaf115ea9c17eb72020-11-24T21:51:18ZengMDPI AGMolecules1420-30492019-07-012415272110.3390/molecules24152721molecules24152721Catalysis of Organic Pollutants Abatement Based on Pt-Decorated Ag@Cu<sub>2</sub>O HeterostructuresXiaolong Zhang0Bingbing Han1Yaxin Wang2Yang Liu3Lei Chen4Yongjun Zhang5Key Laboratory of Functional Materials Physics and Chemistry of the Ministry of Education, Jilin Normal University, Changchun 130103, ChinaKey Laboratory of Functional Materials Physics and Chemistry of the Ministry of Education, Jilin Normal University, Changchun 130103, ChinaKey Laboratory of Functional Materials Physics and Chemistry of the Ministry of Education, Jilin Normal University, Changchun 130103, ChinaKey Laboratory of Functional Materials Physics and Chemistry of the Ministry of Education, Jilin Normal University, Changchun 130103, ChinaKey Laboratory of Functional Materials Physics and Chemistry of the Ministry of Education, Jilin Normal University, Changchun 130103, ChinaKey Laboratory of Functional Materials Physics and Chemistry of the Ministry of Education, Jilin Normal University, Changchun 130103, ChinaPt-decorated Ag@Cu<sub>2</sub>O heterostructures were successfully synthesized using a simple and convenient method. The Pt nanoparticle density on the Ag@Cu<sub>2</sub>O can be controlled by changing the concentration of the Pt precursor. The synthesized Ag@Cu<sub>2</sub>O&#8722;Pt nanoparticles exhibited excellent catalytic performance, which was greatly affected by changes in the Ag@Cu<sub>2</sub>O&#8722;Pt structure. To optimize the material&#8217;s properties, the synthesized Ag@Cu<sub>2</sub>O&#8722;Pt nanoparticles were used to catalyze toxic pollutants and methyl orange (MO), and nontoxic products were obtained by catalytic reduction. The Pt-decorated Ag@Cu<sub>2</sub>O nanoparticles showed excellent catalytic activity, which significantly decreased the pollutant concentration when the nanoparticles were used for catalytic reduction. The redistribution of charge transfer is the nanoparticles&#8217; main contribution to the catalytic degradation of an organic pollutant. This Pt-decorated Ag@Cu<sub>2</sub>O material has unique optical and structural characteristics that make it suitable for photocatalysis, local surface plasmon resonance, and peroxide catalysis.https://www.mdpi.com/1420-3049/24/15/2721catalysisAg@Cu<sub>2</sub>O–Ptorganic pollutants
collection DOAJ
language English
format Article
sources DOAJ
author Xiaolong Zhang
Bingbing Han
Yaxin Wang
Yang Liu
Lei Chen
Yongjun Zhang
spellingShingle Xiaolong Zhang
Bingbing Han
Yaxin Wang
Yang Liu
Lei Chen
Yongjun Zhang
Catalysis of Organic Pollutants Abatement Based on Pt-Decorated Ag@Cu<sub>2</sub>O Heterostructures
Molecules
catalysis
Ag@Cu<sub>2</sub>O–Pt
organic pollutants
author_facet Xiaolong Zhang
Bingbing Han
Yaxin Wang
Yang Liu
Lei Chen
Yongjun Zhang
author_sort Xiaolong Zhang
title Catalysis of Organic Pollutants Abatement Based on Pt-Decorated Ag@Cu<sub>2</sub>O Heterostructures
title_short Catalysis of Organic Pollutants Abatement Based on Pt-Decorated Ag@Cu<sub>2</sub>O Heterostructures
title_full Catalysis of Organic Pollutants Abatement Based on Pt-Decorated Ag@Cu<sub>2</sub>O Heterostructures
title_fullStr Catalysis of Organic Pollutants Abatement Based on Pt-Decorated Ag@Cu<sub>2</sub>O Heterostructures
title_full_unstemmed Catalysis of Organic Pollutants Abatement Based on Pt-Decorated Ag@Cu<sub>2</sub>O Heterostructures
title_sort catalysis of organic pollutants abatement based on pt-decorated ag@cu<sub>2</sub>o heterostructures
publisher MDPI AG
series Molecules
issn 1420-3049
publishDate 2019-07-01
description Pt-decorated Ag@Cu<sub>2</sub>O heterostructures were successfully synthesized using a simple and convenient method. The Pt nanoparticle density on the Ag@Cu<sub>2</sub>O can be controlled by changing the concentration of the Pt precursor. The synthesized Ag@Cu<sub>2</sub>O&#8722;Pt nanoparticles exhibited excellent catalytic performance, which was greatly affected by changes in the Ag@Cu<sub>2</sub>O&#8722;Pt structure. To optimize the material&#8217;s properties, the synthesized Ag@Cu<sub>2</sub>O&#8722;Pt nanoparticles were used to catalyze toxic pollutants and methyl orange (MO), and nontoxic products were obtained by catalytic reduction. The Pt-decorated Ag@Cu<sub>2</sub>O nanoparticles showed excellent catalytic activity, which significantly decreased the pollutant concentration when the nanoparticles were used for catalytic reduction. The redistribution of charge transfer is the nanoparticles&#8217; main contribution to the catalytic degradation of an organic pollutant. This Pt-decorated Ag@Cu<sub>2</sub>O material has unique optical and structural characteristics that make it suitable for photocatalysis, local surface plasmon resonance, and peroxide catalysis.
topic catalysis
Ag@Cu<sub>2</sub>O–Pt
organic pollutants
url https://www.mdpi.com/1420-3049/24/15/2721
work_keys_str_mv AT xiaolongzhang catalysisoforganicpollutantsabatementbasedonptdecoratedagcusub2suboheterostructures
AT bingbinghan catalysisoforganicpollutantsabatementbasedonptdecoratedagcusub2suboheterostructures
AT yaxinwang catalysisoforganicpollutantsabatementbasedonptdecoratedagcusub2suboheterostructures
AT yangliu catalysisoforganicpollutantsabatementbasedonptdecoratedagcusub2suboheterostructures
AT leichen catalysisoforganicpollutantsabatementbasedonptdecoratedagcusub2suboheterostructures
AT yongjunzhang catalysisoforganicpollutantsabatementbasedonptdecoratedagcusub2suboheterostructures
_version_ 1725879205255708672