Dominant role of two-photon vertex in nonlinear response in two-dimensional Dirac systems

Abstract We show that the standard concepts of nonlinear response to electromagnetic fields break down in two-dimensional Dirac systems, like graphene, in the quantum regime close to the Dirac point. We present a compelling many-body theory for nonlinear transport focusing on disorder scattering as...

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Bibliographic Details
Main Authors: Habib Rostami, Emmanuele Cappelluti
Format: Article
Language:English
Published: Nature Publishing Group 2021-05-01
Series:npj 2D Materials and Applications
Online Access:https://doi.org/10.1038/s41699-021-00217-0
Description
Summary:Abstract We show that the standard concepts of nonlinear response to electromagnetic fields break down in two-dimensional Dirac systems, like graphene, in the quantum regime close to the Dirac point. We present a compelling many-body theory for nonlinear transport focusing on disorder scattering as a benchmark example. We show that, although the diamagnetic two-photon vertex is absent at the non-interacting level, disorder effects give rise to a self-generation of such two-photon vertex surviving even in the clean limit. We predict that the two-photon vertex self-generation is present only in two dimensions. The impact of such a striking scenario on the nonlinear quantum transport is discussed, predicting a huge enhancement of third-order dc conductivity comparing to the common models.
ISSN:2397-7132