Engineering unsymmetrically coordinated Cu-S1N3 single atom sites with enhanced oxygen reduction activity
Engineering the coordination environment of single atom catalysts offers to opportunity to optimize electrocatalytic activity. In this work, the authors prepare an unsymmetrical Cu-S1N3 single atom site on porous carbon with high performance in the oxygen reduction reaction.
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| Language: | English |
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Nature Publishing Group
2020-06-01
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| Series: | Nature Communications |
| Online Access: | https://doi.org/10.1038/s41467-020-16848-8 |
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doaj-a6acde3189dd462791c7b3403e8465b22021-06-20T11:13:48ZengNature Publishing GroupNature Communications2041-17232020-06-0111111110.1038/s41467-020-16848-8Engineering unsymmetrically coordinated Cu-S1N3 single atom sites with enhanced oxygen reduction activityHuishan Shang0Xiangyi Zhou1Juncai Dong2Ang Li3Xu Zhao4Qinghua Liu5Yue Lin6Jiajing Pei7Zhi Li8Zhuoli Jiang9Danni Zhou10Lirong Zheng11Yu Wang12Jing Zhou13Zhengkun Yang14Rui Cao15Ritimukta Sarangi16Tingting Sun17Xin Yang18Xusheng Zheng19Wensheng Yan20Zhongbin Zhuang21Jia Li22Wenxing Chen23Dingsheng Wang24Jiatao Zhang25Yadong Li26Beijing Key Laboratory of Construction Tailorable Advanced Functional Materials and Green Applications, School of Materials Science and Engineering, Beijing Institute of TechnologyLaboratory for Computational Materials Engineering, Division of Energy and Environment, Graduate School at Shenzhen, Tsinghua UniversityBeijing Synchrotron Radiation Facility (BSRF), Institute of High Energy Physics, Chinese Academy of SciencesBeijing Key Laboratory of Microstructure and Property of Advanced Materials, Beijing University of TechnologyNational Synchrotron Radiation Laboratory (NSRL), University of Science and Technology of ChinaNational Synchrotron Radiation Laboratory (NSRL), University of Science and Technology of ChinaHefei National Laboratory for Physical Sciences at the Microscale, University of Science and Technology of ChinaState Key Lab of Organic-Inorganic Composites, Beijing University of Chemical TechnologyDepartment of Chemistry, Tsinghua UniversityBeijing Key Laboratory of Construction Tailorable Advanced Functional Materials and Green Applications, School of Materials Science and Engineering, Beijing Institute of TechnologyBeijing Key Laboratory of Construction Tailorable Advanced Functional Materials and Green Applications, School of Materials Science and Engineering, Beijing Institute of TechnologyBeijing Synchrotron Radiation Facility (BSRF), Institute of High Energy Physics, Chinese Academy of SciencesShanghai Synchrotron Radiation Facilities (SSRF), Shanghai Institute of Applied Physics, Chinese Academy of ScienceShanghai Synchrotron Radiation Facilities (SSRF), Shanghai Institute of Applied Physics, Chinese Academy of ScienceCollaborative Innovation Center of Chemistry for Energy Materials, Department of Chemistry, University of Science and Technology of ChinaStanford Synchrotron Radiation Lightsource, SLAC National Accelerator LaboratoryStanford Synchrotron Radiation Lightsource, SLAC National Accelerator LaboratoryBeijing Key Laboratory for Science and Application of Functional Molecular and Crystalline Materials, Department of Chemistry, University of Science and Technology BeijingLaboratory for Computational Materials Engineering, Division of Energy and Environment, Graduate School at Shenzhen, Tsinghua UniversityNational Synchrotron Radiation Laboratory (NSRL), University of Science and Technology of ChinaNational Synchrotron Radiation Laboratory (NSRL), University of Science and Technology of ChinaState Key Lab of Organic-Inorganic Composites, Beijing University of Chemical TechnologyLaboratory for Computational Materials Engineering, Division of Energy and Environment, Graduate School at Shenzhen, Tsinghua UniversityBeijing Key Laboratory of Construction Tailorable Advanced Functional Materials and Green Applications, School of Materials Science and Engineering, Beijing Institute of TechnologyDepartment of Chemistry, Tsinghua UniversityBeijing Key Laboratory of Construction Tailorable Advanced Functional Materials and Green Applications, School of Materials Science and Engineering, Beijing Institute of TechnologyDepartment of Chemistry, Tsinghua UniversityEngineering the coordination environment of single atom catalysts offers to opportunity to optimize electrocatalytic activity. In this work, the authors prepare an unsymmetrical Cu-S1N3 single atom site on porous carbon with high performance in the oxygen reduction reaction.https://doi.org/10.1038/s41467-020-16848-8 |
| collection |
DOAJ |
| language |
English |
| format |
Article |
| sources |
DOAJ |
| author |
Huishan Shang Xiangyi Zhou Juncai Dong Ang Li Xu Zhao Qinghua Liu Yue Lin Jiajing Pei Zhi Li Zhuoli Jiang Danni Zhou Lirong Zheng Yu Wang Jing Zhou Zhengkun Yang Rui Cao Ritimukta Sarangi Tingting Sun Xin Yang Xusheng Zheng Wensheng Yan Zhongbin Zhuang Jia Li Wenxing Chen Dingsheng Wang Jiatao Zhang Yadong Li |
| spellingShingle |
Huishan Shang Xiangyi Zhou Juncai Dong Ang Li Xu Zhao Qinghua Liu Yue Lin Jiajing Pei Zhi Li Zhuoli Jiang Danni Zhou Lirong Zheng Yu Wang Jing Zhou Zhengkun Yang Rui Cao Ritimukta Sarangi Tingting Sun Xin Yang Xusheng Zheng Wensheng Yan Zhongbin Zhuang Jia Li Wenxing Chen Dingsheng Wang Jiatao Zhang Yadong Li Engineering unsymmetrically coordinated Cu-S1N3 single atom sites with enhanced oxygen reduction activity Nature Communications |
| author_facet |
Huishan Shang Xiangyi Zhou Juncai Dong Ang Li Xu Zhao Qinghua Liu Yue Lin Jiajing Pei Zhi Li Zhuoli Jiang Danni Zhou Lirong Zheng Yu Wang Jing Zhou Zhengkun Yang Rui Cao Ritimukta Sarangi Tingting Sun Xin Yang Xusheng Zheng Wensheng Yan Zhongbin Zhuang Jia Li Wenxing Chen Dingsheng Wang Jiatao Zhang Yadong Li |
| author_sort |
Huishan Shang |
| title |
Engineering unsymmetrically coordinated Cu-S1N3 single atom sites with enhanced oxygen reduction activity |
| title_short |
Engineering unsymmetrically coordinated Cu-S1N3 single atom sites with enhanced oxygen reduction activity |
| title_full |
Engineering unsymmetrically coordinated Cu-S1N3 single atom sites with enhanced oxygen reduction activity |
| title_fullStr |
Engineering unsymmetrically coordinated Cu-S1N3 single atom sites with enhanced oxygen reduction activity |
| title_full_unstemmed |
Engineering unsymmetrically coordinated Cu-S1N3 single atom sites with enhanced oxygen reduction activity |
| title_sort |
engineering unsymmetrically coordinated cu-s1n3 single atom sites with enhanced oxygen reduction activity |
| publisher |
Nature Publishing Group |
| series |
Nature Communications |
| issn |
2041-1723 |
| publishDate |
2020-06-01 |
| description |
Engineering the coordination environment of single atom catalysts offers to opportunity to optimize electrocatalytic activity. In this work, the authors prepare an unsymmetrical Cu-S1N3 single atom site on porous carbon with high performance in the oxygen reduction reaction. |
| url |
https://doi.org/10.1038/s41467-020-16848-8 |
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