A versatile route to fabricate single atom catalysts with high chemoselectivity and regioselectivity in hydrogenation

The general synthesis of single atom catalysts (SACs) is of broad interest to chemists but remains a formidable challenge. Here, with the precursor-dilution strategy, the authors successfully prepare 24 different SACs and the Pt SACs exhibit superior chemo- and regio-selectivity in hydrogenation.

Bibliographic Details
Main Authors:	Xiaohui He, Qian He, Yuchen Deng, Mi Peng, Hongyu Chen, Ying Zhang, Siyu Yao, Mengtao Zhang, Dequan Xiao, Ding Ma, Binghui Ge, Hongbing Ji
Format:	Article
Language:	English
Published:	Nature Publishing Group 2019-08-01
Series:	Nature Communications
Online Access:	https://doi.org/10.1038/s41467-019-11619-6

id	doaj-a682a820793f4246a9dc59cd5dc32e95
record_format	Article
spelling	doaj-a682a820793f4246a9dc59cd5dc32e952021-05-11T12:33:01ZengNature Publishing GroupNature Communications2041-17232019-08-011011910.1038/s41467-019-11619-6A versatile route to fabricate single atom catalysts with high chemoselectivity and regioselectivity in hydrogenationXiaohui He0Qian He1Yuchen Deng2Mi Peng3Hongyu Chen4Ying Zhang5Siyu Yao6Mengtao Zhang7Dequan Xiao8Ding Ma9Binghui Ge10Hongbing Ji11Fine Chemical Industry Research Institute, School of Chemistry, Sun Yat-sen UniversityFine Chemical Industry Research Institute, School of Chemistry, Sun Yat-sen UniversityBeijing National Laboratory for Molecular Sciences, College of Chemistry and Molecular Engineering and College of Engineering, and BIC-ESAT, Peking UniversityBeijing National Laboratory for Molecular Sciences, College of Chemistry and Molecular Engineering and College of Engineering, and BIC-ESAT, Peking UniversityFine Chemical Industry Research Institute, School of Chemistry, Sun Yat-sen UniversityFine Chemical Industry Research Institute, School of Chemistry, Sun Yat-sen UniversityBeijing National Laboratory for Molecular Sciences, College of Chemistry and Molecular Engineering and College of Engineering, and BIC-ESAT, Peking UniversityBeijing National Laboratory for Molecular Sciences, College of Chemistry and Molecular Engineering and College of Engineering, and BIC-ESAT, Peking UniversityCenter for Integrative Materials Discovery, Department of Chemistry and Chemical Engineering, University of New HavenBeijing National Laboratory for Molecular Sciences, College of Chemistry and Molecular Engineering and College of Engineering, and BIC-ESAT, Peking UniversityBeijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of SciencesFine Chemical Industry Research Institute, School of Chemistry, Sun Yat-sen UniversityThe general synthesis of single atom catalysts (SACs) is of broad interest to chemists but remains a formidable challenge. Here, with the precursor-dilution strategy, the authors successfully prepare 24 different SACs and the Pt SACs exhibit superior chemo- and regio-selectivity in hydrogenation.https://doi.org/10.1038/s41467-019-11619-6
collection	DOAJ
language	English
format	Article
sources	DOAJ
author	Xiaohui He Qian He Yuchen Deng Mi Peng Hongyu Chen Ying Zhang Siyu Yao Mengtao Zhang Dequan Xiao Ding Ma Binghui Ge Hongbing Ji
spellingShingle	Xiaohui He Qian He Yuchen Deng Mi Peng Hongyu Chen Ying Zhang Siyu Yao Mengtao Zhang Dequan Xiao Ding Ma Binghui Ge Hongbing Ji A versatile route to fabricate single atom catalysts with high chemoselectivity and regioselectivity in hydrogenation Nature Communications
author_facet	Xiaohui He Qian He Yuchen Deng Mi Peng Hongyu Chen Ying Zhang Siyu Yao Mengtao Zhang Dequan Xiao Ding Ma Binghui Ge Hongbing Ji
author_sort	Xiaohui He
title	A versatile route to fabricate single atom catalysts with high chemoselectivity and regioselectivity in hydrogenation
title_short	A versatile route to fabricate single atom catalysts with high chemoselectivity and regioselectivity in hydrogenation
title_full	A versatile route to fabricate single atom catalysts with high chemoselectivity and regioselectivity in hydrogenation
title_fullStr	A versatile route to fabricate single atom catalysts with high chemoselectivity and regioselectivity in hydrogenation
title_full_unstemmed	A versatile route to fabricate single atom catalysts with high chemoselectivity and regioselectivity in hydrogenation
title_sort	versatile route to fabricate single atom catalysts with high chemoselectivity and regioselectivity in hydrogenation
publisher	Nature Publishing Group
series	Nature Communications
issn	2041-1723
publishDate	2019-08-01
description	The general synthesis of single atom catalysts (SACs) is of broad interest to chemists but remains a formidable challenge. Here, with the precursor-dilution strategy, the authors successfully prepare 24 different SACs and the Pt SACs exhibit superior chemo- and regio-selectivity in hydrogenation.
url	https://doi.org/10.1038/s41467-019-11619-6
work_keys_str_mv	AT xiaohuihe aversatileroutetofabricatesingleatomcatalystswithhighchemoselectivityandregioselectivityinhydrogenation AT qianhe aversatileroutetofabricatesingleatomcatalystswithhighchemoselectivityandregioselectivityinhydrogenation AT yuchendeng aversatileroutetofabricatesingleatomcatalystswithhighchemoselectivityandregioselectivityinhydrogenation AT mipeng aversatileroutetofabricatesingleatomcatalystswithhighchemoselectivityandregioselectivityinhydrogenation AT hongyuchen aversatileroutetofabricatesingleatomcatalystswithhighchemoselectivityandregioselectivityinhydrogenation AT yingzhang aversatileroutetofabricatesingleatomcatalystswithhighchemoselectivityandregioselectivityinhydrogenation AT siyuyao aversatileroutetofabricatesingleatomcatalystswithhighchemoselectivityandregioselectivityinhydrogenation AT mengtaozhang aversatileroutetofabricatesingleatomcatalystswithhighchemoselectivityandregioselectivityinhydrogenation AT dequanxiao aversatileroutetofabricatesingleatomcatalystswithhighchemoselectivityandregioselectivityinhydrogenation AT dingma aversatileroutetofabricatesingleatomcatalystswithhighchemoselectivityandregioselectivityinhydrogenation AT binghuige aversatileroutetofabricatesingleatomcatalystswithhighchemoselectivityandregioselectivityinhydrogenation AT hongbingji aversatileroutetofabricatesingleatomcatalystswithhighchemoselectivityandregioselectivityinhydrogenation AT xiaohuihe versatileroutetofabricatesingleatomcatalystswithhighchemoselectivityandregioselectivityinhydrogenation AT qianhe versatileroutetofabricatesingleatomcatalystswithhighchemoselectivityandregioselectivityinhydrogenation AT yuchendeng versatileroutetofabricatesingleatomcatalystswithhighchemoselectivityandregioselectivityinhydrogenation AT mipeng versatileroutetofabricatesingleatomcatalystswithhighchemoselectivityandregioselectivityinhydrogenation AT hongyuchen versatileroutetofabricatesingleatomcatalystswithhighchemoselectivityandregioselectivityinhydrogenation AT yingzhang versatileroutetofabricatesingleatomcatalystswithhighchemoselectivityandregioselectivityinhydrogenation AT siyuyao versatileroutetofabricatesingleatomcatalystswithhighchemoselectivityandregioselectivityinhydrogenation AT mengtaozhang versatileroutetofabricatesingleatomcatalystswithhighchemoselectivityandregioselectivityinhydrogenation AT dequanxiao versatileroutetofabricatesingleatomcatalystswithhighchemoselectivityandregioselectivityinhydrogenation AT dingma versatileroutetofabricatesingleatomcatalystswithhighchemoselectivityandregioselectivityinhydrogenation AT binghuige versatileroutetofabricatesingleatomcatalystswithhighchemoselectivityandregioselectivityinhydrogenation AT hongbingji versatileroutetofabricatesingleatomcatalystswithhighchemoselectivityandregioselectivityinhydrogenation
_version_	1721444618065674240

A versatile route to fabricate single atom catalysts with high chemoselectivity and regioselectivity in hydrogenation

Similar Items