Operando and three-dimensional visualization of anion depletion and lithium growth by stimulated Raman scattering microscopy

The relationship between Li-ion concentration and Li deposition remains an issue to be addressed. Here the authors show that stimulated Raman scattering microscopy offers insight into the concentration evolution and its impact on the dendrite growth, which is not possible by existing techniques.

Bibliographic Details
Main Authors: Qian Cheng, Lu Wei, Zhe Liu, Nan Ni, Zhe Sang, Bin Zhu, Weiheng Xu, Meijie Chen, Yupeng Miao, Long-Qing Chen, Wei Min, Yuan Yang
Format: Article
Language:English
Published: Nature Publishing Group 2018-07-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-018-05289-z
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spelling doaj-a5404848533d44f8ae50fad7b8f8bded2021-05-11T09:58:15ZengNature Publishing GroupNature Communications2041-17232018-07-019111010.1038/s41467-018-05289-zOperando and three-dimensional visualization of anion depletion and lithium growth by stimulated Raman scattering microscopyQian Cheng0Lu Wei1Zhe Liu2Nan Ni3Zhe Sang4Bin Zhu5Weiheng Xu6Meijie Chen7Yupeng Miao8Long-Qing Chen9Wei Min10Yuan Yang11Department of Applied Physics and Applied Mathematics, Program of Materials Science and Engineering, Columbia UniversityDepartment of Chemistry, Columbia UniversityDepartment of Materials Science and Engineering, The Pennsylvania State UniversityDepartment of Applied Physics and Applied Mathematics, Program of Materials Science and Engineering, Columbia UniversityDepartment of Applied Physics and Applied Mathematics, Program of Materials Science and Engineering, Columbia UniversityDepartment of Applied Physics and Applied Mathematics, Program of Materials Science and Engineering, Columbia UniversityDepartment of Applied Physics and Applied Mathematics, Program of Materials Science and Engineering, Columbia UniversityDepartment of Applied Physics and Applied Mathematics, Program of Materials Science and Engineering, Columbia UniversityDepartment of Chemistry, Columbia UniversityDepartment of Materials Science and Engineering, The Pennsylvania State UniversityDepartment of Chemistry, Columbia UniversityDepartment of Applied Physics and Applied Mathematics, Program of Materials Science and Engineering, Columbia UniversityThe relationship between Li-ion concentration and Li deposition remains an issue to be addressed. Here the authors show that stimulated Raman scattering microscopy offers insight into the concentration evolution and its impact on the dendrite growth, which is not possible by existing techniques.https://doi.org/10.1038/s41467-018-05289-z
collection DOAJ
language English
format Article
sources DOAJ
author Qian Cheng
Lu Wei
Zhe Liu
Nan Ni
Zhe Sang
Bin Zhu
Weiheng Xu
Meijie Chen
Yupeng Miao
Long-Qing Chen
Wei Min
Yuan Yang
spellingShingle Qian Cheng
Lu Wei
Zhe Liu
Nan Ni
Zhe Sang
Bin Zhu
Weiheng Xu
Meijie Chen
Yupeng Miao
Long-Qing Chen
Wei Min
Yuan Yang
Operando and three-dimensional visualization of anion depletion and lithium growth by stimulated Raman scattering microscopy
Nature Communications
author_facet Qian Cheng
Lu Wei
Zhe Liu
Nan Ni
Zhe Sang
Bin Zhu
Weiheng Xu
Meijie Chen
Yupeng Miao
Long-Qing Chen
Wei Min
Yuan Yang
author_sort Qian Cheng
title Operando and three-dimensional visualization of anion depletion and lithium growth by stimulated Raman scattering microscopy
title_short Operando and three-dimensional visualization of anion depletion and lithium growth by stimulated Raman scattering microscopy
title_full Operando and three-dimensional visualization of anion depletion and lithium growth by stimulated Raman scattering microscopy
title_fullStr Operando and three-dimensional visualization of anion depletion and lithium growth by stimulated Raman scattering microscopy
title_full_unstemmed Operando and three-dimensional visualization of anion depletion and lithium growth by stimulated Raman scattering microscopy
title_sort operando and three-dimensional visualization of anion depletion and lithium growth by stimulated raman scattering microscopy
publisher Nature Publishing Group
series Nature Communications
issn 2041-1723
publishDate 2018-07-01
description The relationship between Li-ion concentration and Li deposition remains an issue to be addressed. Here the authors show that stimulated Raman scattering microscopy offers insight into the concentration evolution and its impact on the dendrite growth, which is not possible by existing techniques.
url https://doi.org/10.1038/s41467-018-05289-z
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