A System of Photocatalysis for NAD+ Regeneration of Product of (S)-1-Pheylethanol by Enzymic Catalysis

In this study, a system of photocatalysis for NAD+ regeneration of enzymatic catalysis was constructed. The optimal conditions for the coupling reaction of photocatalysis and biocatalysis were explored. Blue light was chosen for the efficient reaction and the optimal concentration of VB2 (vitamin B2...

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Main Authors:	Shujin Pu, Xuan Zhang, Han Huang, Chengli Yang, Dali Li, Junfang Yang, Jie Ouyang, Xing Chen, Sidra Naseer, Ruofu Shi
Format:	Article
Language:	English
Published:	Diponegoro University 2019-08-01
Series:	Bulletin of Chemical Reaction Engineering & Catalysis
Subjects:	nad+ photocatalysis biocatalysis riboflavin (r)-1-phenylethanol dehydrogenase
Online Access:	https://ejournal2.undip.ac.id/index.php/bcrec/article/view/3930

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spelling	doaj-a42107ca7f6543d99bab438a1226c03d2021-05-02T00:45:16ZengDiponegoro UniversityBulletin of Chemical Reaction Engineering & Catalysis1978-29932019-08-0114242142610.9767/bcrec.14.2.3930.421-4262274A System of Photocatalysis for NAD+ Regeneration of Product of (S)-1-Pheylethanol by Enzymic CatalysisShujin Pu0Xuan Zhang1Han Huang2Chengli Yang3Dali Li4Junfang Yang5Jie Ouyang6Xing Chen7Sidra Naseer8Ruofu Shi9Department of Bioengineering, Nanjing University of Science & Technology , Nanjing, 210094, ChinaDepartment of Bioengineering, Nanjing University of Science & Technology , Nanjing, 210094, ChinaDepartment of Bioengineering, Nanjing University of Science & Technology , Nanjing, 210094, ChinaDepartment of Bioengineering, Nanjing University of Science & Technology , Nanjing, 210094, ChinaDepartment of Bioengineering, Nanjing University of Science & Technology , Nanjing, 210094, ChinaDepartment of Bioengineering, Nanjing University of Science & Technology , Nanjing, 210094, ChinaDepartment of Bioengineering, Nanjing University of Science & Technology , Nanjing, 210094, ChinaDepartment of Bioengineering, Nanjing University of Science & Technology , Nanjing, 210094, ChinaDepartment of Bioengineering, Nanjing University of Science & Technology , Nanjing, 210094, ChinaDepartment of Bioengineering, Nanjing University of Science & Technology , Nanjing, 210094, ChinaIn this study, a system of photocatalysis for NAD+ regeneration of enzymatic catalysis was constructed. The optimal conditions for the coupling reaction of photocatalysis and biocatalysis were explored. Blue light was chosen for the efficient reaction and the optimal concentration of VB2 (vitamin B2, riboflavin) was determined. NAD+-dependent (R)-1-phenylethanol dehydrogenase was used in the reaction for transforming (R)-1-phenylethanol to acetophenone. The byproducts of the reaction were just H2O and O2 by means of catalase. The coupling reaction of catalysis and photocatalysis can be used for obtaining (S)-1-phenylethanol through racemization of 1-phenylethanol. Copyright © 2019 BCREC Group. All rights reservedhttps://ejournal2.undip.ac.id/index.php/bcrec/article/view/3930nad+photocatalysisbiocatalysisriboflavin(r)-1-phenylethanol dehydrogenase
collection	DOAJ
language	English
format	Article
sources	DOAJ
author	Shujin Pu Xuan Zhang Han Huang Chengli Yang Dali Li Junfang Yang Jie Ouyang Xing Chen Sidra Naseer Ruofu Shi
spellingShingle	Shujin Pu Xuan Zhang Han Huang Chengli Yang Dali Li Junfang Yang Jie Ouyang Xing Chen Sidra Naseer Ruofu Shi A System of Photocatalysis for NAD+ Regeneration of Product of (S)-1-Pheylethanol by Enzymic Catalysis Bulletin of Chemical Reaction Engineering & Catalysis nad+ photocatalysis biocatalysis riboflavin (r)-1-phenylethanol dehydrogenase
author_facet	Shujin Pu Xuan Zhang Han Huang Chengli Yang Dali Li Junfang Yang Jie Ouyang Xing Chen Sidra Naseer Ruofu Shi
author_sort	Shujin Pu
title	A System of Photocatalysis for NAD+ Regeneration of Product of (S)-1-Pheylethanol by Enzymic Catalysis
title_short	A System of Photocatalysis for NAD+ Regeneration of Product of (S)-1-Pheylethanol by Enzymic Catalysis
title_full	A System of Photocatalysis for NAD+ Regeneration of Product of (S)-1-Pheylethanol by Enzymic Catalysis
title_fullStr	A System of Photocatalysis for NAD+ Regeneration of Product of (S)-1-Pheylethanol by Enzymic Catalysis
title_full_unstemmed	A System of Photocatalysis for NAD+ Regeneration of Product of (S)-1-Pheylethanol by Enzymic Catalysis
title_sort	system of photocatalysis for nad+ regeneration of product of (s)-1-pheylethanol by enzymic catalysis
publisher	Diponegoro University
series	Bulletin of Chemical Reaction Engineering & Catalysis
issn	1978-2993
publishDate	2019-08-01
description	In this study, a system of photocatalysis for NAD+ regeneration of enzymatic catalysis was constructed. The optimal conditions for the coupling reaction of photocatalysis and biocatalysis were explored. Blue light was chosen for the efficient reaction and the optimal concentration of VB2 (vitamin B2, riboflavin) was determined. NAD+-dependent (R)-1-phenylethanol dehydrogenase was used in the reaction for transforming (R)-1-phenylethanol to acetophenone. The byproducts of the reaction were just H2O and O2 by means of catalase. The coupling reaction of catalysis and photocatalysis can be used for obtaining (S)-1-phenylethanol through racemization of 1-phenylethanol. Copyright © 2019 BCREC Group. All rights reserved
topic	nad+ photocatalysis biocatalysis riboflavin (r)-1-phenylethanol dehydrogenase
url	https://ejournal2.undip.ac.id/index.php/bcrec/article/view/3930
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A System of Photocatalysis for NAD+ Regeneration of Product of (S)-1-Pheylethanol by Enzymic Catalysis

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