Unprecedented generation of 3D heterostructures by mechanochemical disassembly and re-ordering of incommensurate metal chalcogenides

3D heterostructures offer properties that are inaccessible in bulk single-phase solids, but synthetic approaches are limited. The authors use mechanochemical reshuffling of binary precursors and subsequent annealing to design structurally aligned misfit heterostructures with well-defined atomic arra...

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Main Authors:	Oleksandr Dolotko, Ihor Z. Hlova, Arjun K. Pathak, Yaroslav Mudryk, Vitalij K. Pecharsky, Prashant Singh, Duane D. Johnson, Brett W. Boote, Jingzhe Li, Emily A. Smith, Scott L. Carnahan, Aaron J. Rossini, Lin Zhou, Ely M. Eastman, Viktor P. Balema
Format:	Article
Language:	English
Published:	Nature Publishing Group 2020-06-01
Series:	Nature Communications
Online Access:	https://doi.org/10.1038/s41467-020-16672-0

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spelling	doaj-a0eb3d35fd2b4023a870f889d86ef5b82021-06-13T11:18:38ZengNature Publishing GroupNature Communications2041-17232020-06-0111111010.1038/s41467-020-16672-0Unprecedented generation of 3D heterostructures by mechanochemical disassembly and re-ordering of incommensurate metal chalcogenidesOleksandr Dolotko0Ihor Z. Hlova1Arjun K. Pathak2Yaroslav Mudryk3Vitalij K. Pecharsky4Prashant Singh5Duane D. Johnson6Brett W. Boote7Jingzhe Li8Emily A. Smith9Scott L. Carnahan10Aaron J. Rossini11Lin Zhou12Ely M. Eastman13Viktor P. Balema14Ames Laboratory of US Department of Energy, Iowa State UniversityAmes Laboratory of US Department of Energy, Iowa State UniversityAmes Laboratory of US Department of Energy, Iowa State UniversityAmes Laboratory of US Department of Energy, Iowa State UniversityAmes Laboratory of US Department of Energy, Iowa State UniversityAmes Laboratory of US Department of Energy, Iowa State UniversityAmes Laboratory of US Department of Energy, Iowa State UniversityAmes Laboratory of US Department of Energy, Iowa State UniversityAmes Laboratory of US Department of Energy, Iowa State UniversityAmes Laboratory of US Department of Energy, Iowa State UniversityDepartment of Chemistry, Iowa State UniversityDepartment of Chemistry, Iowa State UniversityAmes Laboratory of US Department of Energy, Iowa State UniversityAmes Laboratory of US Department of Energy, Iowa State UniversityAmes Laboratory of US Department of Energy, Iowa State University3D heterostructures offer properties that are inaccessible in bulk single-phase solids, but synthetic approaches are limited. The authors use mechanochemical reshuffling of binary precursors and subsequent annealing to design structurally aligned misfit heterostructures with well-defined atomic arrangements.https://doi.org/10.1038/s41467-020-16672-0
collection	DOAJ
language	English
format	Article
sources	DOAJ
author	Oleksandr Dolotko Ihor Z. Hlova Arjun K. Pathak Yaroslav Mudryk Vitalij K. Pecharsky Prashant Singh Duane D. Johnson Brett W. Boote Jingzhe Li Emily A. Smith Scott L. Carnahan Aaron J. Rossini Lin Zhou Ely M. Eastman Viktor P. Balema
spellingShingle	Oleksandr Dolotko Ihor Z. Hlova Arjun K. Pathak Yaroslav Mudryk Vitalij K. Pecharsky Prashant Singh Duane D. Johnson Brett W. Boote Jingzhe Li Emily A. Smith Scott L. Carnahan Aaron J. Rossini Lin Zhou Ely M. Eastman Viktor P. Balema Unprecedented generation of 3D heterostructures by mechanochemical disassembly and re-ordering of incommensurate metal chalcogenides Nature Communications
author_facet	Oleksandr Dolotko Ihor Z. Hlova Arjun K. Pathak Yaroslav Mudryk Vitalij K. Pecharsky Prashant Singh Duane D. Johnson Brett W. Boote Jingzhe Li Emily A. Smith Scott L. Carnahan Aaron J. Rossini Lin Zhou Ely M. Eastman Viktor P. Balema
author_sort	Oleksandr Dolotko
title	Unprecedented generation of 3D heterostructures by mechanochemical disassembly and re-ordering of incommensurate metal chalcogenides
title_short	Unprecedented generation of 3D heterostructures by mechanochemical disassembly and re-ordering of incommensurate metal chalcogenides
title_full	Unprecedented generation of 3D heterostructures by mechanochemical disassembly and re-ordering of incommensurate metal chalcogenides
title_fullStr	Unprecedented generation of 3D heterostructures by mechanochemical disassembly and re-ordering of incommensurate metal chalcogenides
title_full_unstemmed	Unprecedented generation of 3D heterostructures by mechanochemical disassembly and re-ordering of incommensurate metal chalcogenides
title_sort	unprecedented generation of 3d heterostructures by mechanochemical disassembly and re-ordering of incommensurate metal chalcogenides
publisher	Nature Publishing Group
series	Nature Communications
issn	2041-1723
publishDate	2020-06-01
description	3D heterostructures offer properties that are inaccessible in bulk single-phase solids, but synthetic approaches are limited. The authors use mechanochemical reshuffling of binary precursors and subsequent annealing to design structurally aligned misfit heterostructures with well-defined atomic arrangements.
url	https://doi.org/10.1038/s41467-020-16672-0
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Unprecedented generation of 3D heterostructures by mechanochemical disassembly and re-ordering of incommensurate metal chalcogenides

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