A thermally activated and highly miscible dopant for n-type organic thermoelectrics

Realizing efficient n-doping in organic thermoelectrics remains a challenge due to dopant-semiconductor immiscibility, poor dopant stability and low doping efficiency. Here, the authors use computer-assisted screening to develop n-dopants for thermoelectric polymers that show record power factors.

Bibliographic Details
Main Authors:	Chi-Yuan Yang, Yi-Fan Ding, Dazhen Huang, Jue Wang, Ze-Fan Yao, Chun-Xi Huang, Yang Lu, Hio-Ieng Un, Fang-Dong Zhuang, Jin-Hu Dou, Chong-an Di, Daoben Zhu, Jie-Yu Wang, Ting Lei, Jian Pei
Format:	Article
Language:	English
Published:	Nature Publishing Group 2020-07-01
Series:	Nature Communications
Online Access:	https://doi.org/10.1038/s41467-020-17063-1

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spelling	doaj-97e302950047467d9daebe73799990462021-07-04T11:46:44ZengNature Publishing GroupNature Communications2041-17232020-07-0111111010.1038/s41467-020-17063-1A thermally activated and highly miscible dopant for n-type organic thermoelectricsChi-Yuan Yang0Yi-Fan Ding1Dazhen Huang2Jue Wang3Ze-Fan Yao4Chun-Xi Huang5Yang Lu6Hio-Ieng Un7Fang-Dong Zhuang8Jin-Hu Dou9Chong-an Di10Daoben Zhu11Jie-Yu Wang12Ting Lei13Jian Pei14Beijing National Laboratory for Molecular Sciences (BNLMS), Key Laboratory of Polymer Chemistry and Physics of Ministry of Education, Center of Soft Matter Science and Engineering, College of Chemistry and Molecular Engineering, Peking UniversityBeijing National Laboratory for Molecular Sciences (BNLMS), Key Laboratory of Polymer Chemistry and Physics of Ministry of Education, Center of Soft Matter Science and Engineering, College of Chemistry and Molecular Engineering, Peking UniversityBeijing National Laboratory for Molecular Sciences (BNLMS), CAS Key Laboratory of Organic Solids, Institute of Chemistry, Chinese Academy of SciencesBeijing National Laboratory for Molecular Sciences (BNLMS), Key Laboratory of Polymer Chemistry and Physics of Ministry of Education, Center of Soft Matter Science and Engineering, College of Chemistry and Molecular Engineering, Peking UniversityBeijing National Laboratory for Molecular Sciences (BNLMS), Key Laboratory of Polymer Chemistry and Physics of Ministry of Education, Center of Soft Matter Science and Engineering, College of Chemistry and Molecular Engineering, Peking UniversityBeijing National Laboratory for Molecular Sciences (BNLMS), Key Laboratory of Polymer Chemistry and Physics of Ministry of Education, Center of Soft Matter Science and Engineering, College of Chemistry and Molecular Engineering, Peking UniversityBeijing National Laboratory for Molecular Sciences (BNLMS), Key Laboratory of Polymer Chemistry and Physics of Ministry of Education, Center of Soft Matter Science and Engineering, College of Chemistry and Molecular Engineering, Peking UniversityBeijing National Laboratory for Molecular Sciences (BNLMS), Key Laboratory of Polymer Chemistry and Physics of Ministry of Education, Center of Soft Matter Science and Engineering, College of Chemistry and Molecular Engineering, Peking UniversityBeijing National Laboratory for Molecular Sciences (BNLMS), Key Laboratory of Polymer Chemistry and Physics of Ministry of Education, Center of Soft Matter Science and Engineering, College of Chemistry and Molecular Engineering, Peking UniversityBeijing National Laboratory for Molecular Sciences (BNLMS), Key Laboratory of Polymer Chemistry and Physics of Ministry of Education, Center of Soft Matter Science and Engineering, College of Chemistry and Molecular Engineering, Peking UniversityBeijing National Laboratory for Molecular Sciences (BNLMS), CAS Key Laboratory of Organic Solids, Institute of Chemistry, Chinese Academy of SciencesBeijing National Laboratory for Molecular Sciences (BNLMS), CAS Key Laboratory of Organic Solids, Institute of Chemistry, Chinese Academy of SciencesBeijing National Laboratory for Molecular Sciences (BNLMS), Key Laboratory of Polymer Chemistry and Physics of Ministry of Education, Center of Soft Matter Science and Engineering, College of Chemistry and Molecular Engineering, Peking UniversityDepartment of Materials Science and Engineering, College of Engineering, Peking UniversityBeijing National Laboratory for Molecular Sciences (BNLMS), Key Laboratory of Polymer Chemistry and Physics of Ministry of Education, Center of Soft Matter Science and Engineering, College of Chemistry and Molecular Engineering, Peking UniversityRealizing efficient n-doping in organic thermoelectrics remains a challenge due to dopant-semiconductor immiscibility, poor dopant stability and low doping efficiency. Here, the authors use computer-assisted screening to develop n-dopants for thermoelectric polymers that show record power factors.https://doi.org/10.1038/s41467-020-17063-1
collection	DOAJ
language	English
format	Article
sources	DOAJ
author	Chi-Yuan Yang Yi-Fan Ding Dazhen Huang Jue Wang Ze-Fan Yao Chun-Xi Huang Yang Lu Hio-Ieng Un Fang-Dong Zhuang Jin-Hu Dou Chong-an Di Daoben Zhu Jie-Yu Wang Ting Lei Jian Pei
spellingShingle	Chi-Yuan Yang Yi-Fan Ding Dazhen Huang Jue Wang Ze-Fan Yao Chun-Xi Huang Yang Lu Hio-Ieng Un Fang-Dong Zhuang Jin-Hu Dou Chong-an Di Daoben Zhu Jie-Yu Wang Ting Lei Jian Pei A thermally activated and highly miscible dopant for n-type organic thermoelectrics Nature Communications
author_facet	Chi-Yuan Yang Yi-Fan Ding Dazhen Huang Jue Wang Ze-Fan Yao Chun-Xi Huang Yang Lu Hio-Ieng Un Fang-Dong Zhuang Jin-Hu Dou Chong-an Di Daoben Zhu Jie-Yu Wang Ting Lei Jian Pei
author_sort	Chi-Yuan Yang
title	A thermally activated and highly miscible dopant for n-type organic thermoelectrics
title_short	A thermally activated and highly miscible dopant for n-type organic thermoelectrics
title_full	A thermally activated and highly miscible dopant for n-type organic thermoelectrics
title_fullStr	A thermally activated and highly miscible dopant for n-type organic thermoelectrics
title_full_unstemmed	A thermally activated and highly miscible dopant for n-type organic thermoelectrics
title_sort	thermally activated and highly miscible dopant for n-type organic thermoelectrics
publisher	Nature Publishing Group
series	Nature Communications
issn	2041-1723
publishDate	2020-07-01
description	Realizing efficient n-doping in organic thermoelectrics remains a challenge due to dopant-semiconductor immiscibility, poor dopant stability and low doping efficiency. Here, the authors use computer-assisted screening to develop n-dopants for thermoelectric polymers that show record power factors.
url	https://doi.org/10.1038/s41467-020-17063-1
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A thermally activated and highly miscible dopant for n-type organic thermoelectrics

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