Carrier dynamics of Mn-induced states in GaN thin films

Abstract GaN-based materials are widely used for light emission devices, but the intrinsic property of wide bandgap makes it improper for photovoltaic applications. Recently, manganese was doped into GaN for absorption of visible light, and the conversion efficiency of GaN-based solar cells has been...

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Main Authors: Yu-Ting Chen, Chi-Yuan Yang, Po-Cheng Chen, Jinn-Kong Sheu, Kung-Hsuan Lin
Format: Article
Language:English
Published: Nature Publishing Group 2017-07-01
Series:Scientific Reports
Online Access:https://doi.org/10.1038/s41598-017-06316-7
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spelling doaj-8f4832c2bd184eaea95fbd770d6b086c2020-12-08T01:25:44ZengNature Publishing GroupScientific Reports2045-23222017-07-01711810.1038/s41598-017-06316-7Carrier dynamics of Mn-induced states in GaN thin filmsYu-Ting Chen0Chi-Yuan Yang1Po-Cheng Chen2Jinn-Kong Sheu3Kung-Hsuan Lin4Institute of Physics, Academia SinicaInstitute of Physics, Academia SinicaDepartment of Photonics, National Cheng Kung UniversityDepartment of Photonics, National Cheng Kung UniversityInstitute of Physics, Academia SinicaAbstract GaN-based materials are widely used for light emission devices, but the intrinsic property of wide bandgap makes it improper for photovoltaic applications. Recently, manganese was doped into GaN for absorption of visible light, and the conversion efficiency of GaN-based solar cells has been greatly improved. We conducted transient optical measurements to study the carrier dynamics of Mn-doped GaN. The lifetime of carriers in the Mn-related intermediate bands (at 1.5 eV above the valence band edge) is around 1.7 ns. The carrier relaxation within the Mn-induced bandtail states was on the order of a few hundred picoseconds. The relaxation times of different states are important parameters for optimization of conversion efficiency for intermediate-band solar cells.https://doi.org/10.1038/s41598-017-06316-7
collection DOAJ
language English
format Article
sources DOAJ
author Yu-Ting Chen
Chi-Yuan Yang
Po-Cheng Chen
Jinn-Kong Sheu
Kung-Hsuan Lin
spellingShingle Yu-Ting Chen
Chi-Yuan Yang
Po-Cheng Chen
Jinn-Kong Sheu
Kung-Hsuan Lin
Carrier dynamics of Mn-induced states in GaN thin films
Scientific Reports
author_facet Yu-Ting Chen
Chi-Yuan Yang
Po-Cheng Chen
Jinn-Kong Sheu
Kung-Hsuan Lin
author_sort Yu-Ting Chen
title Carrier dynamics of Mn-induced states in GaN thin films
title_short Carrier dynamics of Mn-induced states in GaN thin films
title_full Carrier dynamics of Mn-induced states in GaN thin films
title_fullStr Carrier dynamics of Mn-induced states in GaN thin films
title_full_unstemmed Carrier dynamics of Mn-induced states in GaN thin films
title_sort carrier dynamics of mn-induced states in gan thin films
publisher Nature Publishing Group
series Scientific Reports
issn 2045-2322
publishDate 2017-07-01
description Abstract GaN-based materials are widely used for light emission devices, but the intrinsic property of wide bandgap makes it improper for photovoltaic applications. Recently, manganese was doped into GaN for absorption of visible light, and the conversion efficiency of GaN-based solar cells has been greatly improved. We conducted transient optical measurements to study the carrier dynamics of Mn-doped GaN. The lifetime of carriers in the Mn-related intermediate bands (at 1.5 eV above the valence band edge) is around 1.7 ns. The carrier relaxation within the Mn-induced bandtail states was on the order of a few hundred picoseconds. The relaxation times of different states are important parameters for optimization of conversion efficiency for intermediate-band solar cells.
url https://doi.org/10.1038/s41598-017-06316-7
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