On the Exceptionally High Loading of L-Proline on Multi-Wall Carbon Nanotubes

L-proline is directly loaded on the multi-wall carbon nanotubes (MWCNTs) with exceptionally high loading content of 67 wt.%. The obtained L-proline/MWCNTs catalyst is on par with the catalytic activity of free L-proline, even after 7 rounds of recycling and reusing. The excellent activity of L-proli...

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Main Authors: Jiafang Xu, Jichao Liang, Sheng Huang, Ge Yang, Keyi Tian, Ruonan Chen, Hongyu Chen, Yanhua Zhang
Format: Article
Language:English
Published: MDPI AG 2020-10-01
Series:Catalysts
Subjects:
Online Access:https://www.mdpi.com/2073-4344/10/11/1246
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spelling doaj-8ebaedb32e4e4ae89a8c2d510c6abe0b2020-11-25T04:08:01ZengMDPI AGCatalysts2073-43442020-10-01101246124610.3390/catal10111246On the Exceptionally High Loading of L-Proline on Multi-Wall Carbon NanotubesJiafang Xu0Jichao Liang1Sheng Huang2Ge Yang3Keyi Tian4Ruonan Chen5Hongyu Chen6Yanhua Zhang7Institute of Advanced Synthesis and School of Chemistry and Molecular Engineering, Nanjing Tech University, Nanjing 211816, ChinaInstitute of Advanced Synthesis and School of Chemistry and Molecular Engineering, Nanjing Tech University, Nanjing 211816, ChinaInstitute of Advanced Synthesis and School of Chemistry and Molecular Engineering, Nanjing Tech University, Nanjing 211816, ChinaInstitute of Advanced Synthesis and School of Chemistry and Molecular Engineering, Nanjing Tech University, Nanjing 211816, ChinaInstitute of Advanced Synthesis and School of Chemistry and Molecular Engineering, Nanjing Tech University, Nanjing 211816, ChinaInstitute of Advanced Synthesis and School of Chemistry and Molecular Engineering, Nanjing Tech University, Nanjing 211816, ChinaInstitute of Advanced Synthesis and School of Chemistry and Molecular Engineering, Nanjing Tech University, Nanjing 211816, ChinaInstitute of Advanced Synthesis and School of Chemistry and Molecular Engineering, Nanjing Tech University, Nanjing 211816, ChinaL-proline is directly loaded on the multi-wall carbon nanotubes (MWCNTs) with exceptionally high loading content of 67 wt.%. The obtained L-proline/MWCNTs catalyst is on par with the catalytic activity of free L-proline, even after 7 rounds of recycling and reusing. The excellent activity of L-proline/MWCNTs in typical Aldol reaction, Mannich reaction, Michael reaction, α-oxyamination reaction, and Knoevenagel condensation shows a broad applicability of the composite catalyst in different reactions and solvent systems. We believe that the unusual loading mode may open a window for designing heterogenized organo-catalysts.https://www.mdpi.com/2073-4344/10/11/1246L-proline/MWCNTshigh loadingrecycling stabilitycatalytic efficiencyheterogenized organo-catalysis
collection DOAJ
language English
format Article
sources DOAJ
author Jiafang Xu
Jichao Liang
Sheng Huang
Ge Yang
Keyi Tian
Ruonan Chen
Hongyu Chen
Yanhua Zhang
spellingShingle Jiafang Xu
Jichao Liang
Sheng Huang
Ge Yang
Keyi Tian
Ruonan Chen
Hongyu Chen
Yanhua Zhang
On the Exceptionally High Loading of L-Proline on Multi-Wall Carbon Nanotubes
Catalysts
L-proline/MWCNTs
high loading
recycling stability
catalytic efficiency
heterogenized organo-catalysis
author_facet Jiafang Xu
Jichao Liang
Sheng Huang
Ge Yang
Keyi Tian
Ruonan Chen
Hongyu Chen
Yanhua Zhang
author_sort Jiafang Xu
title On the Exceptionally High Loading of L-Proline on Multi-Wall Carbon Nanotubes
title_short On the Exceptionally High Loading of L-Proline on Multi-Wall Carbon Nanotubes
title_full On the Exceptionally High Loading of L-Proline on Multi-Wall Carbon Nanotubes
title_fullStr On the Exceptionally High Loading of L-Proline on Multi-Wall Carbon Nanotubes
title_full_unstemmed On the Exceptionally High Loading of L-Proline on Multi-Wall Carbon Nanotubes
title_sort on the exceptionally high loading of l-proline on multi-wall carbon nanotubes
publisher MDPI AG
series Catalysts
issn 2073-4344
publishDate 2020-10-01
description L-proline is directly loaded on the multi-wall carbon nanotubes (MWCNTs) with exceptionally high loading content of 67 wt.%. The obtained L-proline/MWCNTs catalyst is on par with the catalytic activity of free L-proline, even after 7 rounds of recycling and reusing. The excellent activity of L-proline/MWCNTs in typical Aldol reaction, Mannich reaction, Michael reaction, α-oxyamination reaction, and Knoevenagel condensation shows a broad applicability of the composite catalyst in different reactions and solvent systems. We believe that the unusual loading mode may open a window for designing heterogenized organo-catalysts.
topic L-proline/MWCNTs
high loading
recycling stability
catalytic efficiency
heterogenized organo-catalysis
url https://www.mdpi.com/2073-4344/10/11/1246
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