Electrochemical oxidation induced intermolecular aromatic C-H imidation

Electrochemical oxidation induced intermolecular aromatic C-H imidation

The dehydrogenative C-H/N-H cross-coupling serves to install nitrogen functionalities into arenes with the highest atom economy. Here, the authors report an electrochemical cross-coupling between aromatics and sulfonimides through an N-radical addition pathway under oxidant- and catalyst-free condit...

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Main Authors: Xia Hu, Guoting Zhang, Lei Nie, Taige Kong, Aiwen Lei
Format: Article
Language:English
Published: Nature Publishing Group 2019-11-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-019-13524-4
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spelling doaj-8d2b052c74514404a7e580dafa48794f2021-05-11T12:21:32ZengNature Publishing GroupNature Communications2041-17232019-11-0110111010.1038/s41467-019-13524-4Electrochemical oxidation induced intermolecular aromatic C-H imidationXia Hu0Guoting Zhang1Lei Nie2Taige Kong3Aiwen Lei4The Institute for Advanced Studies (IAS), College of Chemistry and Molecular Sciences, Wuhan UniversityThe Institute for Advanced Studies (IAS), College of Chemistry and Molecular Sciences, Wuhan UniversityThe Institute for Advanced Studies (IAS), College of Chemistry and Molecular Sciences, Wuhan UniversityThe Institute for Advanced Studies (IAS), College of Chemistry and Molecular Sciences, Wuhan UniversityThe Institute for Advanced Studies (IAS), College of Chemistry and Molecular Sciences, Wuhan UniversityThe dehydrogenative C-H/N-H cross-coupling serves to install nitrogen functionalities into arenes with the highest atom economy. Here, the authors report an electrochemical cross-coupling between aromatics and sulfonimides through an N-radical addition pathway under oxidant- and catalyst-free conditions.https://doi.org/10.1038/s41467-019-13524-4
collection DOAJ
language English
format Article
sources DOAJ
author Xia Hu
Guoting Zhang
Lei Nie
Taige Kong
Aiwen Lei
spellingShingle Xia Hu
Guoting Zhang
Lei Nie
Taige Kong
Aiwen Lei
Electrochemical oxidation induced intermolecular aromatic C-H imidation
Nature Communications
author_facet Xia Hu
Guoting Zhang
Lei Nie
Taige Kong
Aiwen Lei
author_sort Xia Hu
title Electrochemical oxidation induced intermolecular aromatic C-H imidation
title_short Electrochemical oxidation induced intermolecular aromatic C-H imidation
title_full Electrochemical oxidation induced intermolecular aromatic C-H imidation
title_fullStr Electrochemical oxidation induced intermolecular aromatic C-H imidation
title_full_unstemmed Electrochemical oxidation induced intermolecular aromatic C-H imidation
title_sort electrochemical oxidation induced intermolecular aromatic c-h imidation
publisher Nature Publishing Group
series Nature Communications
issn 2041-1723
publishDate 2019-11-01
description The dehydrogenative C-H/N-H cross-coupling serves to install nitrogen functionalities into arenes with the highest atom economy. Here, the authors report an electrochemical cross-coupling between aromatics and sulfonimides through an N-radical addition pathway under oxidant- and catalyst-free conditions.
url https://doi.org/10.1038/s41467-019-13524-4
work_keys_str_mv AT xiahu electrochemicaloxidationinducedintermoleculararomaticchimidation
AT guotingzhang electrochemicaloxidationinducedintermoleculararomaticchimidation
AT leinie electrochemicaloxidationinducedintermoleculararomaticchimidation
AT taigekong electrochemicaloxidationinducedintermoleculararomaticchimidation
AT aiwenlei electrochemicaloxidationinducedintermoleculararomaticchimidation
_version_ 1721444942920810496

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