Restructuring highly electron-deficient metal-metal oxides for boosting stability in acidic oxygen evolution reaction
The poor catalyst stability for oxygen evolution in acidic media has been a long-time issue. Here, authors demonstrate iridium on MoO3 exhibits a low overpotential for oxygen evolution and excellent durability in acidic media due to the high oxidation state of iridium metal on MoO3.
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2021-09-01
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Series: | Nature Communications |
Online Access: | https://doi.org/10.1038/s41467-021-26025-0 |
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doaj-868b471339644a9eb5a33a92a6dc103c2021-10-03T11:50:03ZengNature Publishing GroupNature Communications2041-17232021-09-0112111110.1038/s41467-021-26025-0Restructuring highly electron-deficient metal-metal oxides for boosting stability in acidic oxygen evolution reactionXinghui Liu0Shibo Xi1Hyunwoo Kim2Ashwani Kumar3Jinsun Lee4Jian Wang5Ngoc Quang Tran6Taehun Yang7Xiaodong Shao8Mengfang Liang9Min Gyu Kim10Hyoyoung Lee11Center for Integrated Nanostructure Physics (CINAP), Institute of Basic Science (IBS)Institute of Chemical and Engineering Sciences, A*STARDepartment of Energy Science, Sungkyunkwan University (SKKU)Center for Integrated Nanostructure Physics (CINAP), Institute of Basic Science (IBS)Center for Integrated Nanostructure Physics (CINAP), Institute of Basic Science (IBS)Department of Chemistry, College of Science, Seoul National UniversityCenter for Integrated Nanostructure Physics (CINAP), Institute of Basic Science (IBS)Center for Integrated Nanostructure Physics (CINAP), Institute of Basic Science (IBS)Center for Integrated Nanostructure Physics (CINAP), Institute of Basic Science (IBS)Center for Integrated Nanostructure Physics (CINAP), Institute of Basic Science (IBS)Beamline Research Division, Pohang Accelerator Laboratory (PAL), Pohang University of Science and TechnologyCenter for Integrated Nanostructure Physics (CINAP), Institute of Basic Science (IBS)The poor catalyst stability for oxygen evolution in acidic media has been a long-time issue. Here, authors demonstrate iridium on MoO3 exhibits a low overpotential for oxygen evolution and excellent durability in acidic media due to the high oxidation state of iridium metal on MoO3.https://doi.org/10.1038/s41467-021-26025-0 |
collection |
DOAJ |
language |
English |
format |
Article |
sources |
DOAJ |
author |
Xinghui Liu Shibo Xi Hyunwoo Kim Ashwani Kumar Jinsun Lee Jian Wang Ngoc Quang Tran Taehun Yang Xiaodong Shao Mengfang Liang Min Gyu Kim Hyoyoung Lee |
spellingShingle |
Xinghui Liu Shibo Xi Hyunwoo Kim Ashwani Kumar Jinsun Lee Jian Wang Ngoc Quang Tran Taehun Yang Xiaodong Shao Mengfang Liang Min Gyu Kim Hyoyoung Lee Restructuring highly electron-deficient metal-metal oxides for boosting stability in acidic oxygen evolution reaction Nature Communications |
author_facet |
Xinghui Liu Shibo Xi Hyunwoo Kim Ashwani Kumar Jinsun Lee Jian Wang Ngoc Quang Tran Taehun Yang Xiaodong Shao Mengfang Liang Min Gyu Kim Hyoyoung Lee |
author_sort |
Xinghui Liu |
title |
Restructuring highly electron-deficient metal-metal oxides for boosting stability in acidic oxygen evolution reaction |
title_short |
Restructuring highly electron-deficient metal-metal oxides for boosting stability in acidic oxygen evolution reaction |
title_full |
Restructuring highly electron-deficient metal-metal oxides for boosting stability in acidic oxygen evolution reaction |
title_fullStr |
Restructuring highly electron-deficient metal-metal oxides for boosting stability in acidic oxygen evolution reaction |
title_full_unstemmed |
Restructuring highly electron-deficient metal-metal oxides for boosting stability in acidic oxygen evolution reaction |
title_sort |
restructuring highly electron-deficient metal-metal oxides for boosting stability in acidic oxygen evolution reaction |
publisher |
Nature Publishing Group |
series |
Nature Communications |
issn |
2041-1723 |
publishDate |
2021-09-01 |
description |
The poor catalyst stability for oxygen evolution in acidic media has been a long-time issue. Here, authors demonstrate iridium on MoO3 exhibits a low overpotential for oxygen evolution and excellent durability in acidic media due to the high oxidation state of iridium metal on MoO3. |
url |
https://doi.org/10.1038/s41467-021-26025-0 |
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