Quantum Spectroscopy of Plasmonic Nanostructures
We use frequency-entangled photons, generated via spontaneous parametric down conversion, to measure the broadband spectral response of an array of gold nanoparticles exhibiting Fano-type plasmon resonance. Refractive-index sensing of a liquid is performed by measuring the shift of the array resonan...
Main Authors: | , , , |
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Format: | Article |
Language: | English |
Published: |
American Physical Society
2014-03-01
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Series: | Physical Review X |
Online Access: | http://doi.org/10.1103/PhysRevX.4.011049 |
Summary: | We use frequency-entangled photons, generated via spontaneous parametric down conversion, to measure the broadband spectral response of an array of gold nanoparticles exhibiting Fano-type plasmon resonance. Refractive-index sensing of a liquid is performed by measuring the shift of the array resonance. This method is robust in excessively noisy conditions compared with conventional broadband transmission spectroscopy. Detection of a refractive-index change is demonstrated with a noise level 70 times higher than the signal, which is shown to be inaccessible with the conventional transmission spectroscopy. Use of low-photon fluxes makes this method suitable for measurements of photosensitive biosamples and chemical substances. |
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ISSN: | 2160-3308 |