Quantum Spectroscopy of Plasmonic Nanostructures

We use frequency-entangled photons, generated via spontaneous parametric down conversion, to measure the broadband spectral response of an array of gold nanoparticles exhibiting Fano-type plasmon resonance. Refractive-index sensing of a liquid is performed by measuring the shift of the array resonan...

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Bibliographic Details
Main Authors: Dmitry A. Kalashnikov, Zhenying Pan, Arseniy I. Kuznetsov, Leonid A. Krivitsky
Format: Article
Language:English
Published: American Physical Society 2014-03-01
Series:Physical Review X
Online Access:http://doi.org/10.1103/PhysRevX.4.011049
Description
Summary:We use frequency-entangled photons, generated via spontaneous parametric down conversion, to measure the broadband spectral response of an array of gold nanoparticles exhibiting Fano-type plasmon resonance. Refractive-index sensing of a liquid is performed by measuring the shift of the array resonance. This method is robust in excessively noisy conditions compared with conventional broadband transmission spectroscopy. Detection of a refractive-index change is demonstrated with a noise level 70 times higher than the signal, which is shown to be inaccessible with the conventional transmission spectroscopy. Use of low-photon fluxes makes this method suitable for measurements of photosensitive biosamples and chemical substances.
ISSN:2160-3308