Modeling interaction between CO2, brine and chalk reservoir rock including temperature effect on petrophysical properties

Carbon dioxide (CO2) capture and sequestration through CO2 enhanced oil recovery (EOR) in oil reservoirs is one of the approaches considered to reduce CO2 emission into the atmosphere. The injection of CO2 into a subsurface geological formation may lead to chemical reactions that may affect the form...

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Main Authors: Hisham Ben Mahmud, Walid Mohamed Mahmud, Ali Al-Rubaye
Format: Article
Language:English
Published: KeAi Communications Co., Ltd. 2021-10-01
Series:Energy Geoscience
Subjects:
Online Access:http://www.sciencedirect.com/science/article/pii/S2666759221000020
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spelling doaj-79d67132950a48c08b5c476ade1cb2582021-09-21T04:10:14ZengKeAi Communications Co., Ltd.Energy Geoscience2666-75922021-10-0124337344Modeling interaction between CO2, brine and chalk reservoir rock including temperature effect on petrophysical propertiesHisham Ben Mahmud0Walid Mohamed Mahmud1Ali Al-Rubaye2Petroleum Engineering Department, Curtin University Malaysia, CDT 250, Miri, 98009, Malaysia; Corresponding author.Department of Petroleum Engineering, University of Tripoli, Tripoli, LibyaGudea Geoscience Group (GGSG), Thi Qar, IraqCarbon dioxide (CO2) capture and sequestration through CO2 enhanced oil recovery (EOR) in oil reservoirs is one of the approaches considered to reduce CO2 emission into the atmosphere. The injection of CO2 into a subsurface geological formation may lead to chemical reactions that may affect the formation pore structure and characteristics. In this study, the effect of CO2–brine–rock interaction on the rock petrophysical properties and mineral volume fraction was numerically investigated during CO2 injection into a chalk reservoir rock. A 3D numerical modeling and simulation were conducted using COMSOL® Multiphysics commercial software of computational fluid dynamics (CFD) to simulate CO2–brine core flooding process in a chalk core. The model was validated against a core–scale experimental data from literature. Simulation differential pressure data matched the literature experimental data closely and consistently indicating good agreement between them. Temperature effect on the performance of CO2–brine–chalk sequestration was also evaluated in the present study. Results indicated that porosity was only slightly affected by temperature increase during CO2 injection in contrast to permeability that was substantially affected by temperature. Moreover, chemical reactions enhanced as temperature increased leading to significant increase in permeability. Thus, carbonated brine sequestration excelled at elevated temperature due to increased acidity which governs the sequestration process. The developed model maybe considered as a reliable tool to optimize various operating parameters of CO2–brine sequestration.http://www.sciencedirect.com/science/article/pii/S2666759221000020CO2–brine injectionPetrophysical propertiesMineral volume fractionCOMSOL Multiphysics softwareTemperature effect on chalk rock
collection DOAJ
language English
format Article
sources DOAJ
author Hisham Ben Mahmud
Walid Mohamed Mahmud
Ali Al-Rubaye
spellingShingle Hisham Ben Mahmud
Walid Mohamed Mahmud
Ali Al-Rubaye
Modeling interaction between CO2, brine and chalk reservoir rock including temperature effect on petrophysical properties
Energy Geoscience
CO2–brine injection
Petrophysical properties
Mineral volume fraction
COMSOL Multiphysics software
Temperature effect on chalk rock
author_facet Hisham Ben Mahmud
Walid Mohamed Mahmud
Ali Al-Rubaye
author_sort Hisham Ben Mahmud
title Modeling interaction between CO2, brine and chalk reservoir rock including temperature effect on petrophysical properties
title_short Modeling interaction between CO2, brine and chalk reservoir rock including temperature effect on petrophysical properties
title_full Modeling interaction between CO2, brine and chalk reservoir rock including temperature effect on petrophysical properties
title_fullStr Modeling interaction between CO2, brine and chalk reservoir rock including temperature effect on petrophysical properties
title_full_unstemmed Modeling interaction between CO2, brine and chalk reservoir rock including temperature effect on petrophysical properties
title_sort modeling interaction between co2, brine and chalk reservoir rock including temperature effect on petrophysical properties
publisher KeAi Communications Co., Ltd.
series Energy Geoscience
issn 2666-7592
publishDate 2021-10-01
description Carbon dioxide (CO2) capture and sequestration through CO2 enhanced oil recovery (EOR) in oil reservoirs is one of the approaches considered to reduce CO2 emission into the atmosphere. The injection of CO2 into a subsurface geological formation may lead to chemical reactions that may affect the formation pore structure and characteristics. In this study, the effect of CO2–brine–rock interaction on the rock petrophysical properties and mineral volume fraction was numerically investigated during CO2 injection into a chalk reservoir rock. A 3D numerical modeling and simulation were conducted using COMSOL® Multiphysics commercial software of computational fluid dynamics (CFD) to simulate CO2–brine core flooding process in a chalk core. The model was validated against a core–scale experimental data from literature. Simulation differential pressure data matched the literature experimental data closely and consistently indicating good agreement between them. Temperature effect on the performance of CO2–brine–chalk sequestration was also evaluated in the present study. Results indicated that porosity was only slightly affected by temperature increase during CO2 injection in contrast to permeability that was substantially affected by temperature. Moreover, chemical reactions enhanced as temperature increased leading to significant increase in permeability. Thus, carbonated brine sequestration excelled at elevated temperature due to increased acidity which governs the sequestration process. The developed model maybe considered as a reliable tool to optimize various operating parameters of CO2–brine sequestration.
topic CO2–brine injection
Petrophysical properties
Mineral volume fraction
COMSOL Multiphysics software
Temperature effect on chalk rock
url http://www.sciencedirect.com/science/article/pii/S2666759221000020
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AT walidmohamedmahmud modelinginteractionbetweenco2brineandchalkreservoirrockincludingtemperatureeffectonpetrophysicalproperties
AT alialrubaye modelinginteractionbetweenco2brineandchalkreservoirrockincludingtemperatureeffectonpetrophysicalproperties
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