Dynamic co-catalysis of Au single atoms and nanoporous Au for methane pyrolysis

Nanocatalysts and single‐atom catalysts are generally considered as two categories with distinct performances. Here, in situ TEM study of catalytic methane pyrolysis over nanoporous Au reveals a highly dynamic process where co‐catalysis exists among various catalyst forms.

Bibliographic Details
Main Authors:	Wei Xi, Kai Wang, Yongli Shen, Mengke Ge, Ziliang Deng, Yunfeng Zhao, Qiue Cao, Yi Ding, Guangzhi Hu, Jun Luo
Format:	Article
Language:	English
Published:	Nature Publishing Group 2020-04-01
Series:	Nature Communications
Online Access:	https://doi.org/10.1038/s41467-020-15806-8

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spelling	doaj-7390b87e73e844b3be5bf7fe3ed4c21d2021-05-11T08:51:46ZengNature Publishing GroupNature Communications2041-17232020-04-011111810.1038/s41467-020-15806-8Dynamic co-catalysis of Au single atoms and nanoporous Au for methane pyrolysisWei Xi0Kai Wang1Yongli Shen2Mengke Ge3Ziliang Deng4Yunfeng Zhao5Qiue Cao6Yi Ding7Guangzhi Hu8Jun Luo9Center for Electron Microscopy and Tianjin Key Lab of Advanced Functional Porous Materials, Institute for New Energy Materials & Low-Carbon Technologies, School of Materials Science and Engineering, Tianjin University of TechnologyCenter for Electron Microscopy and Tianjin Key Lab of Advanced Functional Porous Materials, Institute for New Energy Materials & Low-Carbon Technologies, School of Materials Science and Engineering, Tianjin University of TechnologyCenter for Electron Microscopy and Tianjin Key Lab of Advanced Functional Porous Materials, Institute for New Energy Materials & Low-Carbon Technologies, School of Materials Science and Engineering, Tianjin University of TechnologyCenter for Electron Microscopy and Tianjin Key Lab of Advanced Functional Porous Materials, Institute for New Energy Materials & Low-Carbon Technologies, School of Materials Science and Engineering, Tianjin University of TechnologyCenter for Electron Microscopy and Tianjin Key Lab of Advanced Functional Porous Materials, Institute for New Energy Materials & Low-Carbon Technologies, School of Materials Science and Engineering, Tianjin University of TechnologyCenter for Electron Microscopy and Tianjin Key Lab of Advanced Functional Porous Materials, Institute for New Energy Materials & Low-Carbon Technologies, School of Materials Science and Engineering, Tianjin University of TechnologySchool of Chemical Science and Technology, Key Laboratory of Medicinal Chemistry for Nature Resource, Ministry of Education, Yunnan UniversityCenter for Electron Microscopy and Tianjin Key Lab of Advanced Functional Porous Materials, Institute for New Energy Materials & Low-Carbon Technologies, School of Materials Science and Engineering, Tianjin University of TechnologySchool of Chemical Science and Technology, Key Laboratory of Medicinal Chemistry for Nature Resource, Ministry of Education, Yunnan UniversityCenter for Electron Microscopy and Tianjin Key Lab of Advanced Functional Porous Materials, Institute for New Energy Materials & Low-Carbon Technologies, School of Materials Science and Engineering, Tianjin University of TechnologyNanocatalysts and single‐atom catalysts are generally considered as two categories with distinct performances. Here, in situ TEM study of catalytic methane pyrolysis over nanoporous Au reveals a highly dynamic process where co‐catalysis exists among various catalyst forms.https://doi.org/10.1038/s41467-020-15806-8
collection	DOAJ
language	English
format	Article
sources	DOAJ
author	Wei Xi Kai Wang Yongli Shen Mengke Ge Ziliang Deng Yunfeng Zhao Qiue Cao Yi Ding Guangzhi Hu Jun Luo
spellingShingle	Wei Xi Kai Wang Yongli Shen Mengke Ge Ziliang Deng Yunfeng Zhao Qiue Cao Yi Ding Guangzhi Hu Jun Luo Dynamic co-catalysis of Au single atoms and nanoporous Au for methane pyrolysis Nature Communications
author_facet	Wei Xi Kai Wang Yongli Shen Mengke Ge Ziliang Deng Yunfeng Zhao Qiue Cao Yi Ding Guangzhi Hu Jun Luo
author_sort	Wei Xi
title	Dynamic co-catalysis of Au single atoms and nanoporous Au for methane pyrolysis
title_short	Dynamic co-catalysis of Au single atoms and nanoporous Au for methane pyrolysis
title_full	Dynamic co-catalysis of Au single atoms and nanoporous Au for methane pyrolysis
title_fullStr	Dynamic co-catalysis of Au single atoms and nanoporous Au for methane pyrolysis
title_full_unstemmed	Dynamic co-catalysis of Au single atoms and nanoporous Au for methane pyrolysis
title_sort	dynamic co-catalysis of au single atoms and nanoporous au for methane pyrolysis
publisher	Nature Publishing Group
series	Nature Communications
issn	2041-1723
publishDate	2020-04-01
description	Nanocatalysts and single‐atom catalysts are generally considered as two categories with distinct performances. Here, in situ TEM study of catalytic methane pyrolysis over nanoporous Au reveals a highly dynamic process where co‐catalysis exists among various catalyst forms.
url	https://doi.org/10.1038/s41467-020-15806-8
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Dynamic co-catalysis of Au single atoms and nanoporous Au for methane pyrolysis

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