Recent Progresses in the Design and Fabrication of Highly Efficient Ni-Based Catalysts With Advanced Catalytic Activity and Enhanced Anti-coke Performance Toward CO2 Reforming of Methane
CO2 reforming of methane (CRM) can effectively convert two greenhouse gases (CO2 and CH4) into syngas (CO + H2). This process can achieve the efficient resource utilization of CO2 and CH4 and reduce greenhouse gases. Therefore, CRM has been considered as a significantly promising route to solve envi...
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| Format: | Article |
| Language: | English |
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Frontiers Media S.A.
2020-09-01
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| Series: | Frontiers in Chemistry |
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| Online Access: | https://www.frontiersin.org/article/10.3389/fchem.2020.581923/full |
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doaj-72a583c12047479e873ffe6bcdce9489 |
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Article |
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DOAJ |
| language |
English |
| format |
Article |
| sources |
DOAJ |
| author |
Xianyun Wu Leilei Xu Mindong Chen Chufei Lv Xueying Wen Yan Cui Cai-e Wu Bo Yang Zhichao Miao Xun Hu |
| spellingShingle |
Xianyun Wu Leilei Xu Mindong Chen Chufei Lv Xueying Wen Yan Cui Cai-e Wu Bo Yang Zhichao Miao Xun Hu Recent Progresses in the Design and Fabrication of Highly Efficient Ni-Based Catalysts With Advanced Catalytic Activity and Enhanced Anti-coke Performance Toward CO2 Reforming of Methane Frontiers in Chemistry advanced Ni-based catalyst sintering-proof and anti-coke carbon dioxide dry reforming of methane recent progresses |
| author_facet |
Xianyun Wu Leilei Xu Mindong Chen Chufei Lv Xueying Wen Yan Cui Cai-e Wu Bo Yang Zhichao Miao Xun Hu |
| author_sort |
Xianyun Wu |
| title |
Recent Progresses in the Design and Fabrication of Highly Efficient Ni-Based Catalysts With Advanced Catalytic Activity and Enhanced Anti-coke Performance Toward CO2 Reforming of Methane |
| title_short |
Recent Progresses in the Design and Fabrication of Highly Efficient Ni-Based Catalysts With Advanced Catalytic Activity and Enhanced Anti-coke Performance Toward CO2 Reforming of Methane |
| title_full |
Recent Progresses in the Design and Fabrication of Highly Efficient Ni-Based Catalysts With Advanced Catalytic Activity and Enhanced Anti-coke Performance Toward CO2 Reforming of Methane |
| title_fullStr |
Recent Progresses in the Design and Fabrication of Highly Efficient Ni-Based Catalysts With Advanced Catalytic Activity and Enhanced Anti-coke Performance Toward CO2 Reforming of Methane |
| title_full_unstemmed |
Recent Progresses in the Design and Fabrication of Highly Efficient Ni-Based Catalysts With Advanced Catalytic Activity and Enhanced Anti-coke Performance Toward CO2 Reforming of Methane |
| title_sort |
recent progresses in the design and fabrication of highly efficient ni-based catalysts with advanced catalytic activity and enhanced anti-coke performance toward co2 reforming of methane |
| publisher |
Frontiers Media S.A. |
| series |
Frontiers in Chemistry |
| issn |
2296-2646 |
| publishDate |
2020-09-01 |
| description |
CO2 reforming of methane (CRM) can effectively convert two greenhouse gases (CO2 and CH4) into syngas (CO + H2). This process can achieve the efficient resource utilization of CO2 and CH4 and reduce greenhouse gases. Therefore, CRM has been considered as a significantly promising route to solve environmental problems caused by greenhouse effect. Ni-based catalysts have been widely investigated in CRM reactions due to their various advantages, such as high catalytic activity, low price, and abundant reserves. However, Ni-based catalysts usually suffer from rapid deactivation because of thermal sintering of metallic Ni active sites and surface coke deposition, which restricted the industrialization of Ni-based catalysts toward the CRM process. In order to address these challenges, scientists all around the world have devoted great efforts to investigating various influencing factors, such as the option of appropriate supports and promoters and the construction of strong metal-support interaction. Therefore, we carefully summarized recent development in the design and preparation of Ni-based catalysts with advanced catalytic activity and enhanced anti-coke performance toward CRM reactions in this review. Specifically, recent progresses of Ni-based catalysts with different supports, additives, preparation methods, and so on, have been summarized in detail. Furthermore, recent development of reaction mechanism studies over Ni-based catalysts was also covered by this review. Finally, it is prospected that the Ni-based catalyst supported by an ordered mesoporous framework and the combined reforming of methane will become the future development trend. |
| topic |
advanced Ni-based catalyst sintering-proof and anti-coke carbon dioxide dry reforming of methane recent progresses |
| url |
https://www.frontiersin.org/article/10.3389/fchem.2020.581923/full |
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doaj-72a583c12047479e873ffe6bcdce94892020-11-25T03:47:00ZengFrontiers Media S.A.Frontiers in Chemistry2296-26462020-09-01810.3389/fchem.2020.581923581923Recent Progresses in the Design and Fabrication of Highly Efficient Ni-Based Catalysts With Advanced Catalytic Activity and Enhanced Anti-coke Performance Toward CO2 Reforming of MethaneXianyun Wu0Leilei Xu1Mindong Chen2Chufei Lv3Xueying Wen4Yan Cui5Cai-e Wu6Bo Yang7Zhichao Miao8Xun Hu9Jiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control, Collaborative Innovation Center of the Atmospheric Environment and Equipment Technology, School of Environmental Science and Engineering, Nanjing University of Information Science and Technology, Nanjing, ChinaJiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control, Collaborative Innovation Center of the Atmospheric Environment and Equipment Technology, School of Environmental Science and Engineering, Nanjing University of Information Science and Technology, Nanjing, ChinaJiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control, Collaborative Innovation Center of the Atmospheric Environment and Equipment Technology, School of Environmental Science and Engineering, Nanjing University of Information Science and Technology, Nanjing, ChinaJiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control, Collaborative Innovation Center of the Atmospheric Environment and Equipment Technology, School of Environmental Science and Engineering, Nanjing University of Information Science and Technology, Nanjing, ChinaJiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control, Collaborative Innovation Center of the Atmospheric Environment and Equipment Technology, School of Environmental Science and Engineering, Nanjing University of Information Science and Technology, Nanjing, ChinaJiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control, Collaborative Innovation Center of the Atmospheric Environment and Equipment Technology, School of Environmental Science and Engineering, Nanjing University of Information Science and Technology, Nanjing, ChinaCollege of Light Industry and Food Engineering, Nanjing Forestry University, Nanjing, ChinaJiangsu Key Laboratory of Atmospheric Environment Monitoring and Pollution Control, Collaborative Innovation Center of the Atmospheric Environment and Equipment Technology, School of Environmental Science and Engineering, Nanjing University of Information Science and Technology, Nanjing, ChinaSchool of Chemistry and Chemical Engineering, Shandong University of Technology, Zibo, ChinaSchool of Material Science and Engineering, University of Jinan, Jinan, ChinaCO2 reforming of methane (CRM) can effectively convert two greenhouse gases (CO2 and CH4) into syngas (CO + H2). This process can achieve the efficient resource utilization of CO2 and CH4 and reduce greenhouse gases. Therefore, CRM has been considered as a significantly promising route to solve environmental problems caused by greenhouse effect. Ni-based catalysts have been widely investigated in CRM reactions due to their various advantages, such as high catalytic activity, low price, and abundant reserves. However, Ni-based catalysts usually suffer from rapid deactivation because of thermal sintering of metallic Ni active sites and surface coke deposition, which restricted the industrialization of Ni-based catalysts toward the CRM process. In order to address these challenges, scientists all around the world have devoted great efforts to investigating various influencing factors, such as the option of appropriate supports and promoters and the construction of strong metal-support interaction. Therefore, we carefully summarized recent development in the design and preparation of Ni-based catalysts with advanced catalytic activity and enhanced anti-coke performance toward CRM reactions in this review. Specifically, recent progresses of Ni-based catalysts with different supports, additives, preparation methods, and so on, have been summarized in detail. Furthermore, recent development of reaction mechanism studies over Ni-based catalysts was also covered by this review. Finally, it is prospected that the Ni-based catalyst supported by an ordered mesoporous framework and the combined reforming of methane will become the future development trend.https://www.frontiersin.org/article/10.3389/fchem.2020.581923/fulladvanced Ni-based catalystsintering-proof and anti-cokecarbon dioxidedry reforming of methanerecent progresses |