Use of Tracer Elements for Estimating Community Exposure to Marcellus Shale Development Operations

Since 2009, unconventional natural gas development (UNGD) has significantly increased in Appalachia’s Marcellus Shale formation. Elevations of fine particulate matter <2.5 µm (PM2.5), have been documented in areas surrounding drilling operations during well stimulation. Fur...

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Main Authors: Maya Nye, Travis Knuckles, Beizhan Yan, James Ross, William Orem, Matthew Varonka, George Thurston, Alexandria Dzomba, Michael McCawley
Format: Article
Language:English
Published: MDPI AG 2020-03-01
Series:International Journal of Environmental Research and Public Health
Subjects:
Online Access:https://www.mdpi.com/1660-4601/17/6/1837
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spelling doaj-6ef6ae001bfb4c51ad3640224a7d65202020-11-25T01:41:51ZengMDPI AGInternational Journal of Environmental Research and Public Health1660-46012020-03-01176183710.3390/ijerph17061837ijerph17061837Use of Tracer Elements for Estimating Community Exposure to Marcellus Shale Development OperationsMaya Nye0Travis Knuckles1Beizhan Yan2James Ross3William Orem4Matthew Varonka5George Thurston6Alexandria Dzomba7Michael McCawley8West Virginia University School of Public Health, Department of Occupational and Environmental Health Sciences, Morgantown, WV 26506, USAWest Virginia University School of Public Health, Department of Occupational and Environmental Health Sciences, Morgantown, WV 26506, USAThe Lamont-Doherty Earth Observatory at Columbia University, Palisades, NY 10964, USAThe Lamont-Doherty Earth Observatory at Columbia University, Palisades, NY 10964, USAUS Geological Survey, Reston, VA 201924, USAUS Geological Survey, Reston, VA 201924, USAProgram in Exposure Assessment and Human Health Effects at the Department of Environmental Medicine, New York University School of Medicine, Tuxedo, NY 10987, USAWest Virginia University School of Public Health, Department of Occupational and Environmental Health Sciences, Morgantown, WV 26506, USAWest Virginia University School of Public Health, Department of Occupational and Environmental Health Sciences, Morgantown, WV 26506, USASince 2009, unconventional natural gas development (UNGD) has significantly increased in Appalachia’s Marcellus Shale formation. Elevations of fine particulate matter <2.5 µm (PM2.5), have been documented in areas surrounding drilling operations during well stimulation. Furthermore, many communities are experiencing increased industrial activities and probable UNGD air pollutant exposures. Recent studies have associated UNGD emissions with health effects based on distances from well pads. In this study, PM2.5 filter samples were collected on an active gas well pad in Morgantown, West Virginia, and three locations downwind during hydraulic stimulation. Fine particulate samples were analyzed for major and trace elements. An experimental source identification model was developed to determine which elements appeared to be traceable downwind of the UNGD site and whether these elements corresponded to PM2.5 measurements. Results suggest that 1) magnesium may be useful for detecting the reach of UNGD point source emissions, 2) complex surface topographic and meteorological conditions in the Marcellus Shale region could be modeled and confounding sources discounted, and 3) well pad emissions may be measurable at distances of at least 7 km. If shown to be more widely applicable, future tracer studies could enhance epidemiological studies showing health effects of UNGD-associated emissions at ≥15 km.https://www.mdpi.com/1660-4601/17/6/1837tracer elementsunconventional natural gas developmentsource identificationparticulate matterpm2.5community exposure
collection DOAJ
language English
format Article
sources DOAJ
author Maya Nye
Travis Knuckles
Beizhan Yan
James Ross
William Orem
Matthew Varonka
George Thurston
Alexandria Dzomba
Michael McCawley
spellingShingle Maya Nye
Travis Knuckles
Beizhan Yan
James Ross
William Orem
Matthew Varonka
George Thurston
Alexandria Dzomba
Michael McCawley
Use of Tracer Elements for Estimating Community Exposure to Marcellus Shale Development Operations
International Journal of Environmental Research and Public Health
tracer elements
unconventional natural gas development
source identification
particulate matter
pm2.5
community exposure
author_facet Maya Nye
Travis Knuckles
Beizhan Yan
James Ross
William Orem
Matthew Varonka
George Thurston
Alexandria Dzomba
Michael McCawley
author_sort Maya Nye
title Use of Tracer Elements for Estimating Community Exposure to Marcellus Shale Development Operations
title_short Use of Tracer Elements for Estimating Community Exposure to Marcellus Shale Development Operations
title_full Use of Tracer Elements for Estimating Community Exposure to Marcellus Shale Development Operations
title_fullStr Use of Tracer Elements for Estimating Community Exposure to Marcellus Shale Development Operations
title_full_unstemmed Use of Tracer Elements for Estimating Community Exposure to Marcellus Shale Development Operations
title_sort use of tracer elements for estimating community exposure to marcellus shale development operations
publisher MDPI AG
series International Journal of Environmental Research and Public Health
issn 1660-4601
publishDate 2020-03-01
description Since 2009, unconventional natural gas development (UNGD) has significantly increased in Appalachia’s Marcellus Shale formation. Elevations of fine particulate matter <2.5 µm (PM2.5), have been documented in areas surrounding drilling operations during well stimulation. Furthermore, many communities are experiencing increased industrial activities and probable UNGD air pollutant exposures. Recent studies have associated UNGD emissions with health effects based on distances from well pads. In this study, PM2.5 filter samples were collected on an active gas well pad in Morgantown, West Virginia, and three locations downwind during hydraulic stimulation. Fine particulate samples were analyzed for major and trace elements. An experimental source identification model was developed to determine which elements appeared to be traceable downwind of the UNGD site and whether these elements corresponded to PM2.5 measurements. Results suggest that 1) magnesium may be useful for detecting the reach of UNGD point source emissions, 2) complex surface topographic and meteorological conditions in the Marcellus Shale region could be modeled and confounding sources discounted, and 3) well pad emissions may be measurable at distances of at least 7 km. If shown to be more widely applicable, future tracer studies could enhance epidemiological studies showing health effects of UNGD-associated emissions at ≥15 km.
topic tracer elements
unconventional natural gas development
source identification
particulate matter
pm2.5
community exposure
url https://www.mdpi.com/1660-4601/17/6/1837
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