Non-Linear Response to Periodic Forcing of Methane-Air Global and Detailed Kinetics in Continuous Stirred Tank Reactors Close to Extinction Conditions

Non-Linear Response to Periodic Forcing of Methane-Air Global and Detailed Kinetics in Continuous Stirred Tank Reactors Close to Extinction Conditions

This paper focus on the behavior of a continuous stirred tank reactor (CSTR) subject to perturbations of finite amplitude and frequency. Two main objectives are pursued: to determine the extinction line in the equivalence ratio (φ) - residence time (τ) plane, fixed the thermodynamic state conditions...

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Main Authors: Francesco Saverio Marra, Luigi Acampora, Emanuele Martelli
Format: Article
Language:English
Published: SAGE Publishing 2015-09-01
Series:International Journal of Spray and Combustion Dynamics
Online Access:https://doi.org/10.1260/1756-8277.7.3.175
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spelling doaj-6ae15b200800459b972b99fccf74d2b92020-11-25T03:45:17ZengSAGE PublishingInternational Journal of Spray and Combustion Dynamics1756-82771756-82852015-09-01710.1260/1756-8277.7.3.17510.1260_1756-8277.7.3.175Non-Linear Response to Periodic Forcing of Methane-Air Global and Detailed Kinetics in Continuous Stirred Tank Reactors Close to Extinction ConditionsFrancesco Saverio Marra0Luigi Acampora1Emanuele Martelli2 Istituto di Ricerche sulla Combustione - CNR, Napoli, Italy Department of Industrial and Information Engineering - SUN, Aversa, Italy Department of Industrial and Information Engineering - SUN, Aversa, ItalyThis paper focus on the behavior of a continuous stirred tank reactor (CSTR) subject to perturbations of finite amplitude and frequency. Two main objectives are pursued: to determine the extinction line in the equivalence ratio (φ) - residence time (τ) plane, fixed the thermodynamic state conditions; and to characterize the response of the chemical system to periodic forcing of the residence time. Transient simulations of combustion of methane with air, using both global single-step and detailed chemical kinetic mechanisms, have been conducted and the corresponding asymptotic solutions analyzed. Results indicate very different dynamical behaviors, posing the issue of a proper choice of the kinetic scheme for the numerical study of combustion oscillations.https://doi.org/10.1260/1756-8277.7.3.175
collection DOAJ
language English
format Article
sources DOAJ
author Francesco Saverio Marra
Luigi Acampora
Emanuele Martelli
spellingShingle Francesco Saverio Marra
Luigi Acampora
Emanuele Martelli
Non-Linear Response to Periodic Forcing of Methane-Air Global and Detailed Kinetics in Continuous Stirred Tank Reactors Close to Extinction Conditions
International Journal of Spray and Combustion Dynamics
author_facet Francesco Saverio Marra
Luigi Acampora
Emanuele Martelli
author_sort Francesco Saverio Marra
title Non-Linear Response to Periodic Forcing of Methane-Air Global and Detailed Kinetics in Continuous Stirred Tank Reactors Close to Extinction Conditions
title_short Non-Linear Response to Periodic Forcing of Methane-Air Global and Detailed Kinetics in Continuous Stirred Tank Reactors Close to Extinction Conditions
title_full Non-Linear Response to Periodic Forcing of Methane-Air Global and Detailed Kinetics in Continuous Stirred Tank Reactors Close to Extinction Conditions
title_fullStr Non-Linear Response to Periodic Forcing of Methane-Air Global and Detailed Kinetics in Continuous Stirred Tank Reactors Close to Extinction Conditions
title_full_unstemmed Non-Linear Response to Periodic Forcing of Methane-Air Global and Detailed Kinetics in Continuous Stirred Tank Reactors Close to Extinction Conditions
title_sort non-linear response to periodic forcing of methane-air global and detailed kinetics in continuous stirred tank reactors close to extinction conditions
publisher SAGE Publishing
series International Journal of Spray and Combustion Dynamics
issn 1756-8277
1756-8285
publishDate 2015-09-01
description This paper focus on the behavior of a continuous stirred tank reactor (CSTR) subject to perturbations of finite amplitude and frequency. Two main objectives are pursued: to determine the extinction line in the equivalence ratio (φ) - residence time (τ) plane, fixed the thermodynamic state conditions; and to characterize the response of the chemical system to periodic forcing of the residence time. Transient simulations of combustion of methane with air, using both global single-step and detailed chemical kinetic mechanisms, have been conducted and the corresponding asymptotic solutions analyzed. Results indicate very different dynamical behaviors, posing the issue of a proper choice of the kinetic scheme for the numerical study of combustion oscillations.
url https://doi.org/10.1260/1756-8277.7.3.175
work_keys_str_mv AT francescosaveriomarra nonlinearresponsetoperiodicforcingofmethaneairglobalanddetailedkineticsincontinuousstirredtankreactorsclosetoextinctionconditions
AT luigiacampora nonlinearresponsetoperiodicforcingofmethaneairglobalanddetailedkineticsincontinuousstirredtankreactorsclosetoextinctionconditions
AT emanuelemartelli nonlinearresponsetoperiodicforcingofmethaneairglobalanddetailedkineticsincontinuousstirredtankreactorsclosetoextinctionconditions
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