Atomic-scale identification of novel planar defect phases in heteroepitaxial YBa2Cu3O7−δ thin films
We have discovered two novel types of planar defects that appear in heteroepitaxial YBa2Cu3O7−δ (YBCO123) thin films, grown by pulsed-laser deposition (PLD) either with or without a La2/3Ca1/3MnO3 (LCMO) overlayer, using the combination of high-angle annular dark-field scanning transmission electron...
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2018-05-01
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Online Access: | http://dx.doi.org/10.1063/1.5011761 |
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doaj-6419dbdc78614736b93d10c1371977662020-11-24T22:35:53ZengAIP Publishing LLCAIP Advances2158-32262018-05-0185055022055022-710.1063/1.5011761080805ADVAtomic-scale identification of novel planar defect phases in heteroepitaxial YBa2Cu3O7−δ thin filmsNicolas Gauquelin0Hao Zhang1Guozhen Zhu2John Y. T. Wei3Gianluigi A. Botton4Canadian Centre for Electron Microscopy, McMaster University, 1280 Main Street West, Hamilton, Ontario L8S 4M1, CanadaDepartment of Physics, University of Toronto, 60 St. George Street, ON M5S1A7, Toronto, CanadaCanadian Centre for Electron Microscopy, McMaster University, 1280 Main Street West, Hamilton, Ontario L8S 4M1, CanadaDepartment of Physics, University of Toronto, 60 St. George Street, ON M5S1A7, Toronto, CanadaCanadian Centre for Electron Microscopy, McMaster University, 1280 Main Street West, Hamilton, Ontario L8S 4M1, CanadaWe have discovered two novel types of planar defects that appear in heteroepitaxial YBa2Cu3O7−δ (YBCO123) thin films, grown by pulsed-laser deposition (PLD) either with or without a La2/3Ca1/3MnO3 (LCMO) overlayer, using the combination of high-angle annular dark-field scanning transmission electron microscopy (HAADF-STEM) imaging and electron energy loss spectroscopy (EELS) mapping for unambiguous identification. These planar lattice defects are based on the intergrowth of either a BaO plane between two CuO chains or multiple Y-O layers between two CuO2 planes, resulting in non-stoichiometric layer sequences that could directly impact the high-Tc superconductivity.http://dx.doi.org/10.1063/1.5011761 |
collection |
DOAJ |
language |
English |
format |
Article |
sources |
DOAJ |
author |
Nicolas Gauquelin Hao Zhang Guozhen Zhu John Y. T. Wei Gianluigi A. Botton |
spellingShingle |
Nicolas Gauquelin Hao Zhang Guozhen Zhu John Y. T. Wei Gianluigi A. Botton Atomic-scale identification of novel planar defect phases in heteroepitaxial YBa2Cu3O7−δ thin films AIP Advances |
author_facet |
Nicolas Gauquelin Hao Zhang Guozhen Zhu John Y. T. Wei Gianluigi A. Botton |
author_sort |
Nicolas Gauquelin |
title |
Atomic-scale identification of novel planar defect phases in heteroepitaxial YBa2Cu3O7−δ thin films |
title_short |
Atomic-scale identification of novel planar defect phases in heteroepitaxial YBa2Cu3O7−δ thin films |
title_full |
Atomic-scale identification of novel planar defect phases in heteroepitaxial YBa2Cu3O7−δ thin films |
title_fullStr |
Atomic-scale identification of novel planar defect phases in heteroepitaxial YBa2Cu3O7−δ thin films |
title_full_unstemmed |
Atomic-scale identification of novel planar defect phases in heteroepitaxial YBa2Cu3O7−δ thin films |
title_sort |
atomic-scale identification of novel planar defect phases in heteroepitaxial yba2cu3o7−δ thin films |
publisher |
AIP Publishing LLC |
series |
AIP Advances |
issn |
2158-3226 |
publishDate |
2018-05-01 |
description |
We have discovered two novel types of planar defects that appear in heteroepitaxial YBa2Cu3O7−δ (YBCO123) thin films, grown by pulsed-laser deposition (PLD) either with or without a La2/3Ca1/3MnO3 (LCMO) overlayer, using the combination of high-angle annular dark-field scanning transmission electron microscopy (HAADF-STEM) imaging and electron energy loss spectroscopy (EELS) mapping for unambiguous identification. These planar lattice defects are based on the intergrowth of either a BaO plane between two CuO chains or multiple Y-O layers between two CuO2 planes, resulting in non-stoichiometric layer sequences that could directly impact the high-Tc superconductivity. |
url |
http://dx.doi.org/10.1063/1.5011761 |
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