One-Pot-Multicomponent Synthesis of 2,6-Diamino-4-arylpyridine-3,5-dicarbonitrile Derivatives Using Nanomagnetic Fe<sub>3</sub>O<sub>4</sub>@SiO<sub>2</sub>@ZnCl<sub>2</sub>
Nanomagnetic Fe3O4@SiO2@ZnCl2 was used as a simple, cost-effective, and reusable heterogeneous catalyst for the synthesis of 2,6-diamino-4-arylpyridine-3,5-dicarbonitriles by a one-pot-three-component condensation reaction of malononitrile, ammonium acetate, and aldehydes under solvent-free conditio...
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doaj-5d69591e09de42b1bf0aa362c2e836a12020-11-24T21:52:06ZengUniversitas Gadjah MadaIndonesian Journal of Chemistry1411-94202460-15782018-11-0118463964610.22146/ijc.3306222142One-Pot-Multicomponent Synthesis of 2,6-Diamino-4-arylpyridine-3,5-dicarbonitrile Derivatives Using Nanomagnetic Fe<sub>3</sub>O<sub>4</sub>@SiO<sub>2</sub>@ZnCl<sub>2</sub>Behrooz Maleki0Hadi Natheghi1Vahid Sokhanvaran2Samaneh Sedigh Ashrafi3Department of Chemistry, Faculty of Sciences, Hakim Sabzevari University, Sabzevar 96179-76487, IranDepartment of Chemistry, Faculty of Sciences, Hakim Sabzevari University, Sabzevar 96179-76487, IranFaculty of Basic Sciences, University of Neyshabur, Neyshabur, IranDepartment of Chemistry, Faculty of Sciences, Hakim Sabzevari University, Sabzevar 96179-76487, IranNanomagnetic Fe3O4@SiO2@ZnCl2 was used as a simple, cost-effective, and reusable heterogeneous catalyst for the synthesis of 2,6-diamino-4-arylpyridine-3,5-dicarbonitriles by a one-pot-three-component condensation reaction of malononitrile, ammonium acetate, and aldehydes under solvent-free conditions at 110 °C. Simple and mild reaction conditions, facile preparation of the catalyst, the use of a cheap catalyst and easy workup and isolation are notable features of this method.https://jurnal.ugm.ac.id/ijc/article/view/330622,6-diamino-4-arylpyridine-3,5-dicarbonitrilesnano magnetic Fe3O4@SiO2@ZnCl2green chemistrymulti-component reaction |
collection |
DOAJ |
language |
English |
format |
Article |
sources |
DOAJ |
author |
Behrooz Maleki Hadi Natheghi Vahid Sokhanvaran Samaneh Sedigh Ashrafi |
spellingShingle |
Behrooz Maleki Hadi Natheghi Vahid Sokhanvaran Samaneh Sedigh Ashrafi One-Pot-Multicomponent Synthesis of 2,6-Diamino-4-arylpyridine-3,5-dicarbonitrile Derivatives Using Nanomagnetic Fe<sub>3</sub>O<sub>4</sub>@SiO<sub>2</sub>@ZnCl<sub>2</sub> Indonesian Journal of Chemistry 2,6-diamino-4-arylpyridine-3,5-dicarbonitriles nano magnetic Fe3O4@SiO2@ZnCl2 green chemistry multi-component reaction |
author_facet |
Behrooz Maleki Hadi Natheghi Vahid Sokhanvaran Samaneh Sedigh Ashrafi |
author_sort |
Behrooz Maleki |
title |
One-Pot-Multicomponent Synthesis of 2,6-Diamino-4-arylpyridine-3,5-dicarbonitrile Derivatives Using Nanomagnetic Fe<sub>3</sub>O<sub>4</sub>@SiO<sub>2</sub>@ZnCl<sub>2</sub> |
title_short |
One-Pot-Multicomponent Synthesis of 2,6-Diamino-4-arylpyridine-3,5-dicarbonitrile Derivatives Using Nanomagnetic Fe<sub>3</sub>O<sub>4</sub>@SiO<sub>2</sub>@ZnCl<sub>2</sub> |
title_full |
One-Pot-Multicomponent Synthesis of 2,6-Diamino-4-arylpyridine-3,5-dicarbonitrile Derivatives Using Nanomagnetic Fe<sub>3</sub>O<sub>4</sub>@SiO<sub>2</sub>@ZnCl<sub>2</sub> |
title_fullStr |
One-Pot-Multicomponent Synthesis of 2,6-Diamino-4-arylpyridine-3,5-dicarbonitrile Derivatives Using Nanomagnetic Fe<sub>3</sub>O<sub>4</sub>@SiO<sub>2</sub>@ZnCl<sub>2</sub> |
title_full_unstemmed |
One-Pot-Multicomponent Synthesis of 2,6-Diamino-4-arylpyridine-3,5-dicarbonitrile Derivatives Using Nanomagnetic Fe<sub>3</sub>O<sub>4</sub>@SiO<sub>2</sub>@ZnCl<sub>2</sub> |
title_sort |
one-pot-multicomponent synthesis of 2,6-diamino-4-arylpyridine-3,5-dicarbonitrile derivatives using nanomagnetic fe<sub>3</sub>o<sub>4</sub>@sio<sub>2</sub>@zncl<sub>2</sub> |
publisher |
Universitas Gadjah Mada |
series |
Indonesian Journal of Chemistry |
issn |
1411-9420 2460-1578 |
publishDate |
2018-11-01 |
description |
Nanomagnetic Fe3O4@SiO2@ZnCl2 was used as a simple, cost-effective, and reusable heterogeneous catalyst for the synthesis of 2,6-diamino-4-arylpyridine-3,5-dicarbonitriles by a one-pot-three-component condensation reaction of malononitrile, ammonium acetate, and aldehydes under solvent-free conditions at 110 °C. Simple and mild reaction conditions, facile preparation of the catalyst, the use of a cheap catalyst and easy workup and isolation are notable features of this method. |
topic |
2,6-diamino-4-arylpyridine-3,5-dicarbonitriles nano magnetic Fe3O4@SiO2@ZnCl2 green chemistry multi-component reaction |
url |
https://jurnal.ugm.ac.id/ijc/article/view/33062 |
work_keys_str_mv |
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