One-Pot-Multicomponent Synthesis of 2,6-Diamino-4-arylpyridine-3,5-dicarbonitrile Derivatives Using Nanomagnetic Fe<sub>3</sub>O<sub>4</sub>@SiO<sub>2</sub>@ZnCl<sub>2</sub>

Nanomagnetic Fe3O4@SiO2@ZnCl2 was used as a simple, cost-effective, and reusable heterogeneous catalyst for the synthesis of 2,6-diamino-4-arylpyridine-3,5-dicarbonitriles by a one-pot-three-component condensation reaction of malononitrile, ammonium acetate, and aldehydes under solvent-free conditio...

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Main Authors: Behrooz Maleki, Hadi Natheghi, Vahid Sokhanvaran, Samaneh Sedigh Ashrafi
Format: Article
Language:English
Published: Universitas Gadjah Mada 2018-11-01
Series:Indonesian Journal of Chemistry
Subjects:
Online Access:https://jurnal.ugm.ac.id/ijc/article/view/33062
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spelling doaj-5d69591e09de42b1bf0aa362c2e836a12020-11-24T21:52:06ZengUniversitas Gadjah MadaIndonesian Journal of Chemistry1411-94202460-15782018-11-0118463964610.22146/ijc.3306222142One-Pot-Multicomponent Synthesis of 2,6-Diamino-4-arylpyridine-3,5-dicarbonitrile Derivatives Using Nanomagnetic Fe<sub>3</sub>O<sub>4</sub>@SiO<sub>2</sub>@ZnCl<sub>2</sub>Behrooz Maleki0Hadi Natheghi1Vahid Sokhanvaran2Samaneh Sedigh Ashrafi3Department of Chemistry, Faculty of Sciences, Hakim Sabzevari University, Sabzevar 96179-76487, IranDepartment of Chemistry, Faculty of Sciences, Hakim Sabzevari University, Sabzevar 96179-76487, IranFaculty of Basic Sciences, University of Neyshabur, Neyshabur, IranDepartment of Chemistry, Faculty of Sciences, Hakim Sabzevari University, Sabzevar 96179-76487, IranNanomagnetic Fe3O4@SiO2@ZnCl2 was used as a simple, cost-effective, and reusable heterogeneous catalyst for the synthesis of 2,6-diamino-4-arylpyridine-3,5-dicarbonitriles by a one-pot-three-component condensation reaction of malononitrile, ammonium acetate, and aldehydes under solvent-free conditions at 110 °C. Simple and mild reaction conditions, facile preparation of the catalyst, the use of a cheap catalyst and easy workup and isolation are notable features of this method.https://jurnal.ugm.ac.id/ijc/article/view/330622,6-diamino-4-arylpyridine-3,5-dicarbonitrilesnano magnetic Fe3O4@SiO2@ZnCl2green chemistrymulti-component reaction
collection DOAJ
language English
format Article
sources DOAJ
author Behrooz Maleki
Hadi Natheghi
Vahid Sokhanvaran
Samaneh Sedigh Ashrafi
spellingShingle Behrooz Maleki
Hadi Natheghi
Vahid Sokhanvaran
Samaneh Sedigh Ashrafi
One-Pot-Multicomponent Synthesis of 2,6-Diamino-4-arylpyridine-3,5-dicarbonitrile Derivatives Using Nanomagnetic Fe<sub>3</sub>O<sub>4</sub>@SiO<sub>2</sub>@ZnCl<sub>2</sub>
Indonesian Journal of Chemistry
2,6-diamino-4-arylpyridine-3,5-dicarbonitriles
nano magnetic Fe3O4@SiO2@ZnCl2
green chemistry
multi-component reaction
author_facet Behrooz Maleki
Hadi Natheghi
Vahid Sokhanvaran
Samaneh Sedigh Ashrafi
author_sort Behrooz Maleki
title One-Pot-Multicomponent Synthesis of 2,6-Diamino-4-arylpyridine-3,5-dicarbonitrile Derivatives Using Nanomagnetic Fe<sub>3</sub>O<sub>4</sub>@SiO<sub>2</sub>@ZnCl<sub>2</sub>
title_short One-Pot-Multicomponent Synthesis of 2,6-Diamino-4-arylpyridine-3,5-dicarbonitrile Derivatives Using Nanomagnetic Fe<sub>3</sub>O<sub>4</sub>@SiO<sub>2</sub>@ZnCl<sub>2</sub>
title_full One-Pot-Multicomponent Synthesis of 2,6-Diamino-4-arylpyridine-3,5-dicarbonitrile Derivatives Using Nanomagnetic Fe<sub>3</sub>O<sub>4</sub>@SiO<sub>2</sub>@ZnCl<sub>2</sub>
title_fullStr One-Pot-Multicomponent Synthesis of 2,6-Diamino-4-arylpyridine-3,5-dicarbonitrile Derivatives Using Nanomagnetic Fe<sub>3</sub>O<sub>4</sub>@SiO<sub>2</sub>@ZnCl<sub>2</sub>
title_full_unstemmed One-Pot-Multicomponent Synthesis of 2,6-Diamino-4-arylpyridine-3,5-dicarbonitrile Derivatives Using Nanomagnetic Fe<sub>3</sub>O<sub>4</sub>@SiO<sub>2</sub>@ZnCl<sub>2</sub>
title_sort one-pot-multicomponent synthesis of 2,6-diamino-4-arylpyridine-3,5-dicarbonitrile derivatives using nanomagnetic fe<sub>3</sub>o<sub>4</sub>@sio<sub>2</sub>@zncl<sub>2</sub>
publisher Universitas Gadjah Mada
series Indonesian Journal of Chemistry
issn 1411-9420
2460-1578
publishDate 2018-11-01
description Nanomagnetic Fe3O4@SiO2@ZnCl2 was used as a simple, cost-effective, and reusable heterogeneous catalyst for the synthesis of 2,6-diamino-4-arylpyridine-3,5-dicarbonitriles by a one-pot-three-component condensation reaction of malononitrile, ammonium acetate, and aldehydes under solvent-free conditions at 110 °C. Simple and mild reaction conditions, facile preparation of the catalyst, the use of a cheap catalyst and easy workup and isolation are notable features of this method.
topic 2,6-diamino-4-arylpyridine-3,5-dicarbonitriles
nano magnetic Fe3O4@SiO2@ZnCl2
green chemistry
multi-component reaction
url https://jurnal.ugm.ac.id/ijc/article/view/33062
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