Ground-based remote sensing of an elevated forest fire aerosol layer at Whistler, BC: implications for interpretation of mountaintop chemistry

On 30 August 2009, intense forest fires in interior British Columbia (BC) coupled with winds from the east and northeast resulted in transport of a broad forest fire plume across southwestern BC. The physico-chemical and optical characteristics of the plume as observed from Saturna Island (AERONET),...

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Main Authors: I. G. McKendry, J. Gallagher, P. Campuzano Jost, A. Bertram, K. Strawbridge, R. Leaitch, A. M. Macdonald
Format: Article
Language:English
Published: Copernicus Publications 2010-12-01
Series:Atmospheric Chemistry and Physics
Online Access:http://www.atmos-chem-phys.net/10/11921/2010/acp-10-11921-2010.pdf
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spelling doaj-49b62acbf08e47178d22353227eaf6bc2020-11-24T23:31:25ZengCopernicus PublicationsAtmospheric Chemistry and Physics1680-73161680-73242010-12-011023119211193010.5194/acp-10-11921-2010Ground-based remote sensing of an elevated forest fire aerosol layer at Whistler, BC: implications for interpretation of mountaintop chemistryI. G. McKendry0J. Gallagher1P. Campuzano Jost2A. Bertram3K. Strawbridge4R. Leaitch5A. M. Macdonald6Department of Geography, The University of British Columbia, Vancouver, CanadaDepartment of Geography, The University of British Columbia, Vancouver, CanadaDepartment of Chemistry, The University of British Columbia, Vancouver, CanadaDepartment of Chemistry, The University of British Columbia, Vancouver, CanadaCentre for Atmospheric Research Experiments, Environment Canada, Egbert, CanadaScience and Technology Branch, Environment Canada, Toronto, CanadaScience and Technology Branch, Environment Canada, Toronto, CanadaOn 30 August 2009, intense forest fires in interior British Columbia (BC) coupled with winds from the east and northeast resulted in transport of a broad forest fire plume across southwestern BC. The physico-chemical and optical characteristics of the plume as observed from Saturna Island (AERONET), CORALNet-UBC and the Whistler Mountain air chemistry facility were consistent with forest fire plumes that have been observed elsewhere in continental North America. However, the importance of three-dimensional transport in relation to the interpretation of mountaintop chemistry observations is highlighted on the basis of deployment of both a <i>CL31</i> ceilometer and a single particle mass spectrometer (SPMS) in a mountainous setting. The SPMS is used to identify the biomass plume based on levoglucosan and potassium markers. Data from the SPMS are also used to show that the biomass plume was correlated with nitrate, but not correlated with sulphate or sodium. This study not only provides baseline measurements of biomass burning plume physico-chemical characteristics in western Canada, but also highlights the importance of lidar remote sensing methods in the interpretation of mountaintop chemistry measurements.http://www.atmos-chem-phys.net/10/11921/2010/acp-10-11921-2010.pdf
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language English
format Article
sources DOAJ
author I. G. McKendry
J. Gallagher
P. Campuzano Jost
A. Bertram
K. Strawbridge
R. Leaitch
A. M. Macdonald
spellingShingle I. G. McKendry
J. Gallagher
P. Campuzano Jost
A. Bertram
K. Strawbridge
R. Leaitch
A. M. Macdonald
Ground-based remote sensing of an elevated forest fire aerosol layer at Whistler, BC: implications for interpretation of mountaintop chemistry
Atmospheric Chemistry and Physics
author_facet I. G. McKendry
J. Gallagher
P. Campuzano Jost
A. Bertram
K. Strawbridge
R. Leaitch
A. M. Macdonald
author_sort I. G. McKendry
title Ground-based remote sensing of an elevated forest fire aerosol layer at Whistler, BC: implications for interpretation of mountaintop chemistry
title_short Ground-based remote sensing of an elevated forest fire aerosol layer at Whistler, BC: implications for interpretation of mountaintop chemistry
title_full Ground-based remote sensing of an elevated forest fire aerosol layer at Whistler, BC: implications for interpretation of mountaintop chemistry
title_fullStr Ground-based remote sensing of an elevated forest fire aerosol layer at Whistler, BC: implications for interpretation of mountaintop chemistry
title_full_unstemmed Ground-based remote sensing of an elevated forest fire aerosol layer at Whistler, BC: implications for interpretation of mountaintop chemistry
title_sort ground-based remote sensing of an elevated forest fire aerosol layer at whistler, bc: implications for interpretation of mountaintop chemistry
publisher Copernicus Publications
series Atmospheric Chemistry and Physics
issn 1680-7316
1680-7324
publishDate 2010-12-01
description On 30 August 2009, intense forest fires in interior British Columbia (BC) coupled with winds from the east and northeast resulted in transport of a broad forest fire plume across southwestern BC. The physico-chemical and optical characteristics of the plume as observed from Saturna Island (AERONET), CORALNet-UBC and the Whistler Mountain air chemistry facility were consistent with forest fire plumes that have been observed elsewhere in continental North America. However, the importance of three-dimensional transport in relation to the interpretation of mountaintop chemistry observations is highlighted on the basis of deployment of both a <i>CL31</i> ceilometer and a single particle mass spectrometer (SPMS) in a mountainous setting. The SPMS is used to identify the biomass plume based on levoglucosan and potassium markers. Data from the SPMS are also used to show that the biomass plume was correlated with nitrate, but not correlated with sulphate or sodium. This study not only provides baseline measurements of biomass burning plume physico-chemical characteristics in western Canada, but also highlights the importance of lidar remote sensing methods in the interpretation of mountaintop chemistry measurements.
url http://www.atmos-chem-phys.net/10/11921/2010/acp-10-11921-2010.pdf
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