Methane emission estimates using chamber and tracer release experiments for a municipal waste water treatment plant
This study presents two methods for estimating methane emissions from a waste water treatment plant (WWTP) along with results from a measurement campaign at a WWTP in Valence, France. These methods, chamber measurements and tracer release, rely on Fourier transform infrared spectroscopy and cavity r...
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doaj-461e08c3d7924351a3b10968644eb0ee2020-11-24T22:36:11ZengCopernicus PublicationsAtmospheric Measurement Techniques1867-13811867-85482015-07-01872853286710.5194/amt-8-2853-2015Methane emission estimates using chamber and tracer release experiments for a municipal waste water treatment plantC. E. Yver Kwok0D. Müller1C. Caldow2B. Lebègue3J. G. Mønster4C. W. Rella5C. Scheutz6M. Schmidt7M. Ramonet8T. Warneke9G. Broquet10P. Ciais11Laboratoire des Sciences du Climat et l'Environnement (LSCE/IPSL), CNRS-CEA-UVSQ, Centre d'Etudes Orme des Merisiers, Gif sur Yvette, FranceInstitute of Environmental Physics, University of Bremen, Otto-Hahn-Allee 1, 28359 Bremen, GermanyCentre for Atmospheric Chemistry, University of Wollongong, Wollongong, NSW, 2522, AustraliaLaboratoire des Sciences du Climat et l'Environnement (LSCE/IPSL), CNRS-CEA-UVSQ, Centre d'Etudes Orme des Merisiers, Gif sur Yvette, FranceDepartment of Environmental Engineering, Technical University of Denmark, Bygningstorvet – Building 115, 2800 Lyngby, DenmarkPicarro Inc., 3105 Patrick Henry Drive, Santa Clara, CA, USADepartment of Environmental Engineering, Technical University of Denmark, Bygningstorvet – Building 115, 2800 Lyngby, DenmarkLaboratoire des Sciences du Climat et l'Environnement (LSCE/IPSL), CNRS-CEA-UVSQ, Centre d'Etudes Orme des Merisiers, Gif sur Yvette, FranceLaboratoire des Sciences du Climat et l'Environnement (LSCE/IPSL), CNRS-CEA-UVSQ, Centre d'Etudes Orme des Merisiers, Gif sur Yvette, FranceInstitute of Environmental Physics, University of Bremen, Otto-Hahn-Allee 1, 28359 Bremen, GermanyLaboratoire des Sciences du Climat et l'Environnement (LSCE/IPSL), CNRS-CEA-UVSQ, Centre d'Etudes Orme des Merisiers, Gif sur Yvette, FranceLaboratoire des Sciences du Climat et l'Environnement (LSCE/IPSL), CNRS-CEA-UVSQ, Centre d'Etudes Orme des Merisiers, Gif sur Yvette, FranceThis study presents two methods for estimating methane emissions from a waste water treatment plant (WWTP) along with results from a measurement campaign at a WWTP in Valence, France. These methods, chamber measurements and tracer release, rely on Fourier transform infrared spectroscopy and cavity ring-down spectroscopy instruments. We show that the tracer release method is suitable for quantifying facility- and some process-scale emissions, while the chamber measurements provide insight into individual process emissions. Uncertainties for the two methods are described and discussed. Applying the methods to CH<sub>4</sub> emissions of the WWTP, we confirm that the open basins are not a major source of CH<sub>4</sub> on the WWTP (about 10 % of the total emissions), but that the pretreatment and sludge treatment are the main emitters. Overall, the waste water treatment plant is representative of an average French WWTP.http://www.atmos-meas-tech.net/8/2853/2015/amt-8-2853-2015.pdf |
collection |
DOAJ |
language |
English |
format |
Article |
sources |
DOAJ |
author |
C. E. Yver Kwok D. Müller C. Caldow B. Lebègue J. G. Mønster C. W. Rella C. Scheutz M. Schmidt M. Ramonet T. Warneke G. Broquet P. Ciais |
spellingShingle |
C. E. Yver Kwok D. Müller C. Caldow B. Lebègue J. G. Mønster C. W. Rella C. Scheutz M. Schmidt M. Ramonet T. Warneke G. Broquet P. Ciais Methane emission estimates using chamber and tracer release experiments for a municipal waste water treatment plant Atmospheric Measurement Techniques |
author_facet |
C. E. Yver Kwok D. Müller C. Caldow B. Lebègue J. G. Mønster C. W. Rella C. Scheutz M. Schmidt M. Ramonet T. Warneke G. Broquet P. Ciais |
author_sort |
C. E. Yver Kwok |
title |
Methane emission estimates using chamber and tracer release experiments for a municipal waste water treatment plant |
title_short |
Methane emission estimates using chamber and tracer release experiments for a municipal waste water treatment plant |
title_full |
Methane emission estimates using chamber and tracer release experiments for a municipal waste water treatment plant |
title_fullStr |
Methane emission estimates using chamber and tracer release experiments for a municipal waste water treatment plant |
title_full_unstemmed |
Methane emission estimates using chamber and tracer release experiments for a municipal waste water treatment plant |
title_sort |
methane emission estimates using chamber and tracer release experiments for a municipal waste water treatment plant |
publisher |
Copernicus Publications |
series |
Atmospheric Measurement Techniques |
issn |
1867-1381 1867-8548 |
publishDate |
2015-07-01 |
description |
This study presents two methods for estimating methane emissions from
a waste water treatment plant (WWTP) along with results from a measurement
campaign at a WWTP in Valence, France. These methods, chamber measurements
and tracer release, rely on Fourier transform infrared spectroscopy
and cavity ring-down spectroscopy instruments. We show that the tracer
release method is suitable for quantifying facility- and some process-scale
emissions, while the chamber measurements provide insight into individual
process emissions. Uncertainties for the two methods are described and
discussed. Applying the methods to CH<sub>4</sub> emissions of the WWTP, we confirm
that the open basins are not a major source of CH<sub>4</sub> on the WWTP (about
10 % of the total emissions), but that the pretreatment and sludge
treatment are the main emitters. Overall, the waste water treatment plant is representative of an average French WWTP. |
url |
http://www.atmos-meas-tech.net/8/2853/2015/amt-8-2853-2015.pdf |
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