Methane emission estimates using chamber and tracer release experiments for a municipal waste water treatment plant

This study presents two methods for estimating methane emissions from a waste water treatment plant (WWTP) along with results from a measurement campaign at a WWTP in Valence, France. These methods, chamber measurements and tracer release, rely on Fourier transform infrared spectroscopy and cavity r...

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Main Authors: C. E. Yver Kwok, D. Müller, C. Caldow, B. Lebègue, J. G. Mønster, C. W. Rella, C. Scheutz, M. Schmidt, M. Ramonet, T. Warneke, G. Broquet, P. Ciais
Format: Article
Language:English
Published: Copernicus Publications 2015-07-01
Series:Atmospheric Measurement Techniques
Online Access:http://www.atmos-meas-tech.net/8/2853/2015/amt-8-2853-2015.pdf
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spelling doaj-461e08c3d7924351a3b10968644eb0ee2020-11-24T22:36:11ZengCopernicus PublicationsAtmospheric Measurement Techniques1867-13811867-85482015-07-01872853286710.5194/amt-8-2853-2015Methane emission estimates using chamber and tracer release experiments for a municipal waste water treatment plantC. E. Yver Kwok0D. Müller1C. Caldow2B. Lebègue3J. G. Mønster4C. W. Rella5C. Scheutz6M. Schmidt7M. Ramonet8T. Warneke9G. Broquet10P. Ciais11Laboratoire des Sciences du Climat et l'Environnement (LSCE/IPSL), CNRS-CEA-UVSQ, Centre d'Etudes Orme des Merisiers, Gif sur Yvette, FranceInstitute of Environmental Physics, University of Bremen, Otto-Hahn-Allee 1, 28359 Bremen, GermanyCentre for Atmospheric Chemistry, University of Wollongong, Wollongong, NSW, 2522, AustraliaLaboratoire des Sciences du Climat et l'Environnement (LSCE/IPSL), CNRS-CEA-UVSQ, Centre d'Etudes Orme des Merisiers, Gif sur Yvette, FranceDepartment of Environmental Engineering, Technical University of Denmark, Bygningstorvet – Building 115, 2800 Lyngby, DenmarkPicarro Inc., 3105 Patrick Henry Drive, Santa Clara, CA, USADepartment of Environmental Engineering, Technical University of Denmark, Bygningstorvet – Building 115, 2800 Lyngby, DenmarkLaboratoire des Sciences du Climat et l'Environnement (LSCE/IPSL), CNRS-CEA-UVSQ, Centre d'Etudes Orme des Merisiers, Gif sur Yvette, FranceLaboratoire des Sciences du Climat et l'Environnement (LSCE/IPSL), CNRS-CEA-UVSQ, Centre d'Etudes Orme des Merisiers, Gif sur Yvette, FranceInstitute of Environmental Physics, University of Bremen, Otto-Hahn-Allee 1, 28359 Bremen, GermanyLaboratoire des Sciences du Climat et l'Environnement (LSCE/IPSL), CNRS-CEA-UVSQ, Centre d'Etudes Orme des Merisiers, Gif sur Yvette, FranceLaboratoire des Sciences du Climat et l'Environnement (LSCE/IPSL), CNRS-CEA-UVSQ, Centre d'Etudes Orme des Merisiers, Gif sur Yvette, FranceThis study presents two methods for estimating methane emissions from a waste water treatment plant (WWTP) along with results from a measurement campaign at a WWTP in Valence, France. These methods, chamber measurements and tracer release, rely on Fourier transform infrared spectroscopy and cavity ring-down spectroscopy instruments. We show that the tracer release method is suitable for quantifying facility- and some process-scale emissions, while the chamber measurements provide insight into individual process emissions. Uncertainties for the two methods are described and discussed. Applying the methods to CH<sub>4</sub> emissions of the WWTP, we confirm that the open basins are not a major source of CH<sub>4</sub> on the WWTP (about 10 % of the total emissions), but that the pretreatment and sludge treatment are the main emitters. Overall, the waste water treatment plant is representative of an average French WWTP.http://www.atmos-meas-tech.net/8/2853/2015/amt-8-2853-2015.pdf
collection DOAJ
language English
format Article
sources DOAJ
author C. E. Yver Kwok
D. Müller
C. Caldow
B. Lebègue
J. G. Mønster
C. W. Rella
C. Scheutz
M. Schmidt
M. Ramonet
T. Warneke
G. Broquet
P. Ciais
spellingShingle C. E. Yver Kwok
D. Müller
C. Caldow
B. Lebègue
J. G. Mønster
C. W. Rella
C. Scheutz
M. Schmidt
M. Ramonet
T. Warneke
G. Broquet
P. Ciais
Methane emission estimates using chamber and tracer release experiments for a municipal waste water treatment plant
Atmospheric Measurement Techniques
author_facet C. E. Yver Kwok
D. Müller
C. Caldow
B. Lebègue
J. G. Mønster
C. W. Rella
C. Scheutz
M. Schmidt
M. Ramonet
T. Warneke
G. Broquet
P. Ciais
author_sort C. E. Yver Kwok
title Methane emission estimates using chamber and tracer release experiments for a municipal waste water treatment plant
title_short Methane emission estimates using chamber and tracer release experiments for a municipal waste water treatment plant
title_full Methane emission estimates using chamber and tracer release experiments for a municipal waste water treatment plant
title_fullStr Methane emission estimates using chamber and tracer release experiments for a municipal waste water treatment plant
title_full_unstemmed Methane emission estimates using chamber and tracer release experiments for a municipal waste water treatment plant
title_sort methane emission estimates using chamber and tracer release experiments for a municipal waste water treatment plant
publisher Copernicus Publications
series Atmospheric Measurement Techniques
issn 1867-1381
1867-8548
publishDate 2015-07-01
description This study presents two methods for estimating methane emissions from a waste water treatment plant (WWTP) along with results from a measurement campaign at a WWTP in Valence, France. These methods, chamber measurements and tracer release, rely on Fourier transform infrared spectroscopy and cavity ring-down spectroscopy instruments. We show that the tracer release method is suitable for quantifying facility- and some process-scale emissions, while the chamber measurements provide insight into individual process emissions. Uncertainties for the two methods are described and discussed. Applying the methods to CH<sub>4</sub> emissions of the WWTP, we confirm that the open basins are not a major source of CH<sub>4</sub> on the WWTP (about 10 % of the total emissions), but that the pretreatment and sludge treatment are the main emitters. Overall, the waste water treatment plant is representative of an average French WWTP.
url http://www.atmos-meas-tech.net/8/2853/2015/amt-8-2853-2015.pdf
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