Microscopic insight into non-radiative decay in perovskite semiconductors from temperature-dependent luminescence blinking
The mechanism of the non-radiative recombination in halide perovskite nanocrystals has not been fully understood. Here Gerhard et al. resolve the contributions of individual recombination centers by photoluminescence blinking measurements and identify ion migration as the underlying mechanism.
Main Authors: | , , , , , , , , |
---|---|
Format: | Article |
Language: | English |
Published: |
Nature Publishing Group
2019-04-01
|
Series: | Nature Communications |
Online Access: | https://doi.org/10.1038/s41467-019-09640-w |
id |
doaj-4226ca788dda4eaa921933a411af3918 |
---|---|
record_format |
Article |
spelling |
doaj-4226ca788dda4eaa921933a411af39182021-05-11T12:39:54ZengNature Publishing GroupNature Communications2041-17232019-04-0110111210.1038/s41467-019-09640-wMicroscopic insight into non-radiative decay in perovskite semiconductors from temperature-dependent luminescence blinkingMarina Gerhard0Boris Louis1Rafael Camacho2Aboma Merdasa3Jun Li4Alexander Kiligaridis5Alexander Dobrovolsky6Johan Hofkens7Ivan G. Scheblykin8Division of Chemical Physics and NanoLund, Lund UniversityDivision of Chemical Physics and NanoLund, Lund UniversityKU Leuven, Molecular Imaging and PhotonicsHybrid Materials Formation and Scaling, Helmholtz-Zentrum Berlin für Materialien und Energie GmbH, Helmholtz-Zentrum BerlinDivision of Chemical Physics and NanoLund, Lund UniversityDivision of Chemical Physics and NanoLund, Lund UniversityDivision of Chemical Physics and NanoLund, Lund UniversityKU Leuven, Molecular Imaging and PhotonicsDivision of Chemical Physics and NanoLund, Lund UniversityThe mechanism of the non-radiative recombination in halide perovskite nanocrystals has not been fully understood. Here Gerhard et al. resolve the contributions of individual recombination centers by photoluminescence blinking measurements and identify ion migration as the underlying mechanism.https://doi.org/10.1038/s41467-019-09640-w |
collection |
DOAJ |
language |
English |
format |
Article |
sources |
DOAJ |
author |
Marina Gerhard Boris Louis Rafael Camacho Aboma Merdasa Jun Li Alexander Kiligaridis Alexander Dobrovolsky Johan Hofkens Ivan G. Scheblykin |
spellingShingle |
Marina Gerhard Boris Louis Rafael Camacho Aboma Merdasa Jun Li Alexander Kiligaridis Alexander Dobrovolsky Johan Hofkens Ivan G. Scheblykin Microscopic insight into non-radiative decay in perovskite semiconductors from temperature-dependent luminescence blinking Nature Communications |
author_facet |
Marina Gerhard Boris Louis Rafael Camacho Aboma Merdasa Jun Li Alexander Kiligaridis Alexander Dobrovolsky Johan Hofkens Ivan G. Scheblykin |
author_sort |
Marina Gerhard |
title |
Microscopic insight into non-radiative decay in perovskite semiconductors from temperature-dependent luminescence blinking |
title_short |
Microscopic insight into non-radiative decay in perovskite semiconductors from temperature-dependent luminescence blinking |
title_full |
Microscopic insight into non-radiative decay in perovskite semiconductors from temperature-dependent luminescence blinking |
title_fullStr |
Microscopic insight into non-radiative decay in perovskite semiconductors from temperature-dependent luminescence blinking |
title_full_unstemmed |
Microscopic insight into non-radiative decay in perovskite semiconductors from temperature-dependent luminescence blinking |
title_sort |
microscopic insight into non-radiative decay in perovskite semiconductors from temperature-dependent luminescence blinking |
publisher |
Nature Publishing Group |
series |
Nature Communications |
issn |
2041-1723 |
publishDate |
2019-04-01 |
description |
The mechanism of the non-radiative recombination in halide perovskite nanocrystals has not been fully understood. Here Gerhard et al. resolve the contributions of individual recombination centers by photoluminescence blinking measurements and identify ion migration as the underlying mechanism. |
url |
https://doi.org/10.1038/s41467-019-09640-w |
work_keys_str_mv |
AT marinagerhard microscopicinsightintononradiativedecayinperovskitesemiconductorsfromtemperaturedependentluminescenceblinking AT borislouis microscopicinsightintononradiativedecayinperovskitesemiconductorsfromtemperaturedependentluminescenceblinking AT rafaelcamacho microscopicinsightintononradiativedecayinperovskitesemiconductorsfromtemperaturedependentluminescenceblinking AT abomamerdasa microscopicinsightintononradiativedecayinperovskitesemiconductorsfromtemperaturedependentluminescenceblinking AT junli microscopicinsightintononradiativedecayinperovskitesemiconductorsfromtemperaturedependentluminescenceblinking AT alexanderkiligaridis microscopicinsightintononradiativedecayinperovskitesemiconductorsfromtemperaturedependentluminescenceblinking AT alexanderdobrovolsky microscopicinsightintononradiativedecayinperovskitesemiconductorsfromtemperaturedependentluminescenceblinking AT johanhofkens microscopicinsightintononradiativedecayinperovskitesemiconductorsfromtemperaturedependentluminescenceblinking AT ivangscheblykin microscopicinsightintononradiativedecayinperovskitesemiconductorsfromtemperaturedependentluminescenceblinking |
_version_ |
1721444350745903104 |