Resolving atomic SAPO-34/18 intergrowth architectures for methanol conversion by identifying light atoms and bonds
The micro-structures of zeolite catalysts affect their macroarchitectures and catalytic performances. Here, the different SAPO-34/18 intergrowth catalysts are atomically resolved, and the correlation between synthesis conditions and zeolite structures is revealed to further enhance their performance...
Main Authors: | , , , , , , , |
---|---|
Format: | Article |
Language: | English |
Published: |
Nature Publishing Group
2021-04-01
|
Series: | Nature Communications |
Online Access: | https://doi.org/10.1038/s41467-021-22438-z |
id |
doaj-40d94ed261124ae7a3396ffb7aba75c0 |
---|---|
record_format |
Article |
spelling |
doaj-40d94ed261124ae7a3396ffb7aba75c02021-04-18T11:13:49ZengNature Publishing GroupNature Communications2041-17232021-04-011211910.1038/s41467-021-22438-zResolving atomic SAPO-34/18 intergrowth architectures for methanol conversion by identifying light atoms and bondsBoyuan Shen0Xiao Chen1Xiaoyu Fan2Hao Xiong3Huiqiu Wang4Weizhong Qian5Yao Wang6Fei Wei7Beijing Key Laboratory of Green Chemical Reaction Engineering and Technology, Department of Chemical Engineering, Tsinghua UniversityBeijing Key Laboratory of Green Chemical Reaction Engineering and Technology, Department of Chemical Engineering, Tsinghua UniversityBeijing Key Laboratory of Green Chemical Reaction Engineering and Technology, Department of Chemical Engineering, Tsinghua UniversityBeijing Key Laboratory of Green Chemical Reaction Engineering and Technology, Department of Chemical Engineering, Tsinghua UniversityBeijing Key Laboratory of Green Chemical Reaction Engineering and Technology, Department of Chemical Engineering, Tsinghua UniversityBeijing Key Laboratory of Green Chemical Reaction Engineering and Technology, Department of Chemical Engineering, Tsinghua UniversityBeijing Key Laboratory of Green Chemical Reaction Engineering and Technology, Department of Chemical Engineering, Tsinghua UniversityBeijing Key Laboratory of Green Chemical Reaction Engineering and Technology, Department of Chemical Engineering, Tsinghua UniversityThe micro-structures of zeolite catalysts affect their macroarchitectures and catalytic performances. Here, the different SAPO-34/18 intergrowth catalysts are atomically resolved, and the correlation between synthesis conditions and zeolite structures is revealed to further enhance their performances in methanol conversion.https://doi.org/10.1038/s41467-021-22438-z |
collection |
DOAJ |
language |
English |
format |
Article |
sources |
DOAJ |
author |
Boyuan Shen Xiao Chen Xiaoyu Fan Hao Xiong Huiqiu Wang Weizhong Qian Yao Wang Fei Wei |
spellingShingle |
Boyuan Shen Xiao Chen Xiaoyu Fan Hao Xiong Huiqiu Wang Weizhong Qian Yao Wang Fei Wei Resolving atomic SAPO-34/18 intergrowth architectures for methanol conversion by identifying light atoms and bonds Nature Communications |
author_facet |
Boyuan Shen Xiao Chen Xiaoyu Fan Hao Xiong Huiqiu Wang Weizhong Qian Yao Wang Fei Wei |
author_sort |
Boyuan Shen |
title |
Resolving atomic SAPO-34/18 intergrowth architectures for methanol conversion by identifying light atoms and bonds |
title_short |
Resolving atomic SAPO-34/18 intergrowth architectures for methanol conversion by identifying light atoms and bonds |
title_full |
Resolving atomic SAPO-34/18 intergrowth architectures for methanol conversion by identifying light atoms and bonds |
title_fullStr |
Resolving atomic SAPO-34/18 intergrowth architectures for methanol conversion by identifying light atoms and bonds |
title_full_unstemmed |
Resolving atomic SAPO-34/18 intergrowth architectures for methanol conversion by identifying light atoms and bonds |
title_sort |
resolving atomic sapo-34/18 intergrowth architectures for methanol conversion by identifying light atoms and bonds |
publisher |
Nature Publishing Group |
series |
Nature Communications |
issn |
2041-1723 |
publishDate |
2021-04-01 |
description |
The micro-structures of zeolite catalysts affect their macroarchitectures and catalytic performances. Here, the different SAPO-34/18 intergrowth catalysts are atomically resolved, and the correlation between synthesis conditions and zeolite structures is revealed to further enhance their performances in methanol conversion. |
url |
https://doi.org/10.1038/s41467-021-22438-z |
work_keys_str_mv |
AT boyuanshen resolvingatomicsapo3418intergrowtharchitecturesformethanolconversionbyidentifyinglightatomsandbonds AT xiaochen resolvingatomicsapo3418intergrowtharchitecturesformethanolconversionbyidentifyinglightatomsandbonds AT xiaoyufan resolvingatomicsapo3418intergrowtharchitecturesformethanolconversionbyidentifyinglightatomsandbonds AT haoxiong resolvingatomicsapo3418intergrowtharchitecturesformethanolconversionbyidentifyinglightatomsandbonds AT huiqiuwang resolvingatomicsapo3418intergrowtharchitecturesformethanolconversionbyidentifyinglightatomsandbonds AT weizhongqian resolvingatomicsapo3418intergrowtharchitecturesformethanolconversionbyidentifyinglightatomsandbonds AT yaowang resolvingatomicsapo3418intergrowtharchitecturesformethanolconversionbyidentifyinglightatomsandbonds AT feiwei resolvingatomicsapo3418intergrowtharchitecturesformethanolconversionbyidentifyinglightatomsandbonds |
_version_ |
1721522490784612352 |