Compton Scattering Imaging of Liquid Water in Porous Carbon-Based Materials

Synchrotron-based Compton scattering imaging with intense high-energy X-rays allows the visualization of light element substances in an electrochemical device under an operando condition. In this study, we apply this imaging technique to a water-contained, porous carbon-based composite, which is use...

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Main Authors: Naruki Tsuji, Yoichiro Tsuji, Yoshiharu Uchimoto, Hideto Imai, Yoshiharu Sakurai
Format: Article
Language:English
Published: MDPI AG 2021-04-01
Series:Applied Sciences
Subjects:
Online Access:https://www.mdpi.com/2076-3417/11/9/3851
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spelling doaj-39750d814477450f941d31a5913372f22021-04-24T23:00:55ZengMDPI AGApplied Sciences2076-34172021-04-01113851385110.3390/app11093851Compton Scattering Imaging of Liquid Water in Porous Carbon-Based MaterialsNaruki Tsuji0Yoichiro Tsuji1Yoshiharu Uchimoto2Hideto Imai3Yoshiharu Sakurai4Japan Synchrotron Radiation Research Institute (JASRI), Hyogo 679-5198, JapanFuel Cell Cutting-Edge Research Center Technology Research Association (FC-Cubic TRA), Tokyo 135-0064, JapanGraduate School of Human and Environmental Studies, Kyoto University, Kyoto 606-8501, JapanNissan Analysis and Research Center (NISSAN ARC), Kanagawa 237-0061, JapanJapan Synchrotron Radiation Research Institute (JASRI), Hyogo 679-5198, JapanSynchrotron-based Compton scattering imaging with intense high-energy X-rays allows the visualization of light element substances in an electrochemical device under an operando condition. In this study, we apply this imaging technique to a water-contained, porous carbon-based composite, which is used as a material for the gas diffusion layer in polymer electrolyte fuel cells. Analyses of the two-dimensional intensity images of Compton scattered X-rays provide the cross-sectional distributions of liquid water, as well as the depth dependency of the water content. In addition, the analyses reveal a significant interaction between the carbon materials and water droplets.https://www.mdpi.com/2076-3417/11/9/3851X-ray Compton scatteringporous carbon materialsfuel cellscross-sectional imaginghigh-energy X-rays
collection DOAJ
language English
format Article
sources DOAJ
author Naruki Tsuji
Yoichiro Tsuji
Yoshiharu Uchimoto
Hideto Imai
Yoshiharu Sakurai
spellingShingle Naruki Tsuji
Yoichiro Tsuji
Yoshiharu Uchimoto
Hideto Imai
Yoshiharu Sakurai
Compton Scattering Imaging of Liquid Water in Porous Carbon-Based Materials
Applied Sciences
X-ray Compton scattering
porous carbon materials
fuel cells
cross-sectional imaging
high-energy X-rays
author_facet Naruki Tsuji
Yoichiro Tsuji
Yoshiharu Uchimoto
Hideto Imai
Yoshiharu Sakurai
author_sort Naruki Tsuji
title Compton Scattering Imaging of Liquid Water in Porous Carbon-Based Materials
title_short Compton Scattering Imaging of Liquid Water in Porous Carbon-Based Materials
title_full Compton Scattering Imaging of Liquid Water in Porous Carbon-Based Materials
title_fullStr Compton Scattering Imaging of Liquid Water in Porous Carbon-Based Materials
title_full_unstemmed Compton Scattering Imaging of Liquid Water in Porous Carbon-Based Materials
title_sort compton scattering imaging of liquid water in porous carbon-based materials
publisher MDPI AG
series Applied Sciences
issn 2076-3417
publishDate 2021-04-01
description Synchrotron-based Compton scattering imaging with intense high-energy X-rays allows the visualization of light element substances in an electrochemical device under an operando condition. In this study, we apply this imaging technique to a water-contained, porous carbon-based composite, which is used as a material for the gas diffusion layer in polymer electrolyte fuel cells. Analyses of the two-dimensional intensity images of Compton scattered X-rays provide the cross-sectional distributions of liquid water, as well as the depth dependency of the water content. In addition, the analyses reveal a significant interaction between the carbon materials and water droplets.
topic X-ray Compton scattering
porous carbon materials
fuel cells
cross-sectional imaging
high-energy X-rays
url https://www.mdpi.com/2076-3417/11/9/3851
work_keys_str_mv AT narukitsuji comptonscatteringimagingofliquidwaterinporouscarbonbasedmaterials
AT yoichirotsuji comptonscatteringimagingofliquidwaterinporouscarbonbasedmaterials
AT yoshiharuuchimoto comptonscatteringimagingofliquidwaterinporouscarbonbasedmaterials
AT hidetoimai comptonscatteringimagingofliquidwaterinporouscarbonbasedmaterials
AT yoshiharusakurai comptonscatteringimagingofliquidwaterinporouscarbonbasedmaterials
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