Carbon Footprint for Mercury Capture from Coal-Fired Boiler Flue Gas

Power production from coal combustion is one of two major anthropogenic sources of mercury emission to the atmosphere. The aim of this study is the analysis of the carbon footprint of mercury removal technologies through sorbents injection related to the removal of 1 kg of mercury from flue gases. T...

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Main Authors: Magdalena Gazda-Grzywacz, Łukasz Winconek, Piotr Burmistrz
Format: Article
Language:English
Published: MDPI AG 2021-06-01
Series:Energies
Subjects:
Online Access:https://www.mdpi.com/1996-1073/14/13/3844
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spelling doaj-3305201ab505413c859aaab29cf7cf442021-07-15T15:33:10ZengMDPI AGEnergies1996-10732021-06-01143844384410.3390/en14133844Carbon Footprint for Mercury Capture from Coal-Fired Boiler Flue GasMagdalena Gazda-Grzywacz0Łukasz Winconek1Piotr Burmistrz2Faculty of Energy & Fuels, AGH University of Science and Technology, Mickiewicz Avenue 30, 30-059 Krakow, PolandGrand Activated Sp. z o.o., Białostocka 1, 17-200 Hajnówka, PolandFaculty of Energy & Fuels, AGH University of Science and Technology, Mickiewicz Avenue 30, 30-059 Krakow, PolandPower production from coal combustion is one of two major anthropogenic sources of mercury emission to the atmosphere. The aim of this study is the analysis of the carbon footprint of mercury removal technologies through sorbents injection related to the removal of 1 kg of mercury from flue gases. Two sorbents, i.e., powdered activated carbon and the coke dust, were analysed. The assessment included both direct and indirect emissions related to various energy and material needs life cycle including coal mining and transport, sorbents production, transport of sorbents to the power plants, and injection into flue gases. The results show that at the average mercury concentration in processed flue gasses accounting to 28.0 µg Hg/Nm<sup>3</sup>, removal of 1 kg of mercury from flue gases required 14.925 Mg of powdered activated carbon and 33.594 Mg of coke dust, respectively. However, the whole life cycle carbon footprint for powdered activated carbon amounted to 89.548 Mg CO<sub>2-e</sub>·kg<sup>−1</sup> Hg, whereas for coke dust this value was around three times lower and amounted to 24.452 Mg CO<sub>2-e</sub>·kg<sup>−1</sup> Hg. Considering the relatively low price of coke dust and its lower impact on GHG emissions, it can be found as a promising alternative to commercial powdered activated carbon.https://www.mdpi.com/1996-1073/14/13/3844carbon footprintpowdered activated carboncoke dustflue gasesmercury emissionsmercury removal
collection DOAJ
language English
format Article
sources DOAJ
author Magdalena Gazda-Grzywacz
Łukasz Winconek
Piotr Burmistrz
spellingShingle Magdalena Gazda-Grzywacz
Łukasz Winconek
Piotr Burmistrz
Carbon Footprint for Mercury Capture from Coal-Fired Boiler Flue Gas
Energies
carbon footprint
powdered activated carbon
coke dust
flue gases
mercury emissions
mercury removal
author_facet Magdalena Gazda-Grzywacz
Łukasz Winconek
Piotr Burmistrz
author_sort Magdalena Gazda-Grzywacz
title Carbon Footprint for Mercury Capture from Coal-Fired Boiler Flue Gas
title_short Carbon Footprint for Mercury Capture from Coal-Fired Boiler Flue Gas
title_full Carbon Footprint for Mercury Capture from Coal-Fired Boiler Flue Gas
title_fullStr Carbon Footprint for Mercury Capture from Coal-Fired Boiler Flue Gas
title_full_unstemmed Carbon Footprint for Mercury Capture from Coal-Fired Boiler Flue Gas
title_sort carbon footprint for mercury capture from coal-fired boiler flue gas
publisher MDPI AG
series Energies
issn 1996-1073
publishDate 2021-06-01
description Power production from coal combustion is one of two major anthropogenic sources of mercury emission to the atmosphere. The aim of this study is the analysis of the carbon footprint of mercury removal technologies through sorbents injection related to the removal of 1 kg of mercury from flue gases. Two sorbents, i.e., powdered activated carbon and the coke dust, were analysed. The assessment included both direct and indirect emissions related to various energy and material needs life cycle including coal mining and transport, sorbents production, transport of sorbents to the power plants, and injection into flue gases. The results show that at the average mercury concentration in processed flue gasses accounting to 28.0 µg Hg/Nm<sup>3</sup>, removal of 1 kg of mercury from flue gases required 14.925 Mg of powdered activated carbon and 33.594 Mg of coke dust, respectively. However, the whole life cycle carbon footprint for powdered activated carbon amounted to 89.548 Mg CO<sub>2-e</sub>·kg<sup>−1</sup> Hg, whereas for coke dust this value was around three times lower and amounted to 24.452 Mg CO<sub>2-e</sub>·kg<sup>−1</sup> Hg. Considering the relatively low price of coke dust and its lower impact on GHG emissions, it can be found as a promising alternative to commercial powdered activated carbon.
topic carbon footprint
powdered activated carbon
coke dust
flue gases
mercury emissions
mercury removal
url https://www.mdpi.com/1996-1073/14/13/3844
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