Operando NMR spectroscopic analysis of proton transfer in heterogeneous photocatalytic reactions

Identifying proton transfer processes in catalytic reactions is a technically challenging task. Here, the authors employ operando nuclear magnetic resonance spectroscopy to study the reaction mechanism and intermediates of the photocatalytic hydrogen evolution, and to identify the proton sources.

Bibliographic Details
Main Authors:	Xue Lu Wang, Wenqing Liu, Yan-Yan Yu, Yanhong Song, Wen Qi Fang, Daxiu Wei, Xue-Qing Gong, Ye-Feng Yao, Hua Gui Yang
Format:	Article
Language:	English
Published:	Nature Publishing Group 2016-06-01
Series:	Nature Communications
Online Access:	https://doi.org/10.1038/ncomms11918

id	doaj-31e8bef2ceb04491bee4f35c0ce9e2e1
record_format	Article
spelling	doaj-31e8bef2ceb04491bee4f35c0ce9e2e12021-05-11T11:02:10ZengNature Publishing GroupNature Communications2041-17232016-06-01711710.1038/ncomms11918Operando NMR spectroscopic analysis of proton transfer in heterogeneous photocatalytic reactionsXue Lu Wang0Wenqing Liu1Yan-Yan Yu2Yanhong Song3Wen Qi Fang4Daxiu Wei5Xue-Qing Gong6Ye-Feng Yao7Hua Gui Yang8Key Laboratory for Ultrafine Materials of Ministry of Education, School of Materials Science and Engineering, East China University of Science and TechnologyDepartment of Physics, Shanghai Key Laboratory of Magnetic Resonance, East China Normal UniversityKey Laboratory for Advanced Materials, Centre for Computational Chemistry, Research Institute of Industrial Catalysis, East China University of Science and TechnologyDepartment of Physics, Shanghai Key Laboratory of Magnetic Resonance, East China Normal UniversityKey Laboratory for Ultrafine Materials of Ministry of Education, School of Materials Science and Engineering, East China University of Science and TechnologyDepartment of Physics, Shanghai Key Laboratory of Magnetic Resonance, East China Normal UniversityKey Laboratory for Advanced Materials, Centre for Computational Chemistry, Research Institute of Industrial Catalysis, East China University of Science and TechnologyDepartment of Physics, Shanghai Key Laboratory of Magnetic Resonance, East China Normal UniversityKey Laboratory for Ultrafine Materials of Ministry of Education, School of Materials Science and Engineering, East China University of Science and TechnologyIdentifying proton transfer processes in catalytic reactions is a technically challenging task. Here, the authors employ operando nuclear magnetic resonance spectroscopy to study the reaction mechanism and intermediates of the photocatalytic hydrogen evolution, and to identify the proton sources.https://doi.org/10.1038/ncomms11918
collection	DOAJ
language	English
format	Article
sources	DOAJ
author	Xue Lu Wang Wenqing Liu Yan-Yan Yu Yanhong Song Wen Qi Fang Daxiu Wei Xue-Qing Gong Ye-Feng Yao Hua Gui Yang
spellingShingle	Xue Lu Wang Wenqing Liu Yan-Yan Yu Yanhong Song Wen Qi Fang Daxiu Wei Xue-Qing Gong Ye-Feng Yao Hua Gui Yang Operando NMR spectroscopic analysis of proton transfer in heterogeneous photocatalytic reactions Nature Communications
author_facet	Xue Lu Wang Wenqing Liu Yan-Yan Yu Yanhong Song Wen Qi Fang Daxiu Wei Xue-Qing Gong Ye-Feng Yao Hua Gui Yang
author_sort	Xue Lu Wang
title	Operando NMR spectroscopic analysis of proton transfer in heterogeneous photocatalytic reactions
title_short	Operando NMR spectroscopic analysis of proton transfer in heterogeneous photocatalytic reactions
title_full	Operando NMR spectroscopic analysis of proton transfer in heterogeneous photocatalytic reactions
title_fullStr	Operando NMR spectroscopic analysis of proton transfer in heterogeneous photocatalytic reactions
title_full_unstemmed	Operando NMR spectroscopic analysis of proton transfer in heterogeneous photocatalytic reactions
title_sort	operando nmr spectroscopic analysis of proton transfer in heterogeneous photocatalytic reactions
publisher	Nature Publishing Group
series	Nature Communications
issn	2041-1723
publishDate	2016-06-01
description	Identifying proton transfer processes in catalytic reactions is a technically challenging task. Here, the authors employ operando nuclear magnetic resonance spectroscopy to study the reaction mechanism and intermediates of the photocatalytic hydrogen evolution, and to identify the proton sources.
url	https://doi.org/10.1038/ncomms11918
work_keys_str_mv	AT xueluwang operandonmrspectroscopicanalysisofprotontransferinheterogeneousphotocatalyticreactions AT wenqingliu operandonmrspectroscopicanalysisofprotontransferinheterogeneousphotocatalyticreactions AT yanyanyu operandonmrspectroscopicanalysisofprotontransferinheterogeneousphotocatalyticreactions AT yanhongsong operandonmrspectroscopicanalysisofprotontransferinheterogeneousphotocatalyticreactions AT wenqifang operandonmrspectroscopicanalysisofprotontransferinheterogeneousphotocatalyticreactions AT daxiuwei operandonmrspectroscopicanalysisofprotontransferinheterogeneousphotocatalyticreactions AT xueqinggong operandonmrspectroscopicanalysisofprotontransferinheterogeneousphotocatalyticreactions AT yefengyao operandonmrspectroscopicanalysisofprotontransferinheterogeneousphotocatalyticreactions AT huaguiyang operandonmrspectroscopicanalysisofprotontransferinheterogeneousphotocatalyticreactions
_version_	1721447166892834816

Operando NMR spectroscopic analysis of proton transfer in heterogeneous photocatalytic reactions

Similar Items