Risk assessment and source apportionment of trace elements in multiple compartments in the lower reach of the Jinsha River, China

Abstract Studies on trace element (TE) pollution in abiotic matrices have typically focused on water, sediment, and soil, either separately or in pairs. The importance of multi-media connectivity has been ignored. This study analyzed the concentrations of 6 TEs in three connected environmental compa...

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Main Authors: Wenyan He, Fei Li, Jiang Yu, Min Chen, Yun Deng, Jia Li, Xiliang Tang, Zhuoyu Chen, Zhongluan Yan
Format: Article
Language:English
Published: Nature Publishing Group 2021-10-01
Series:Scientific Reports
Online Access:https://doi.org/10.1038/s41598-021-99626-w
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spelling doaj-1f6155136c294b1abea13d1e8125de5a2021-10-10T11:28:46ZengNature Publishing GroupScientific Reports2045-23222021-10-0111111410.1038/s41598-021-99626-wRisk assessment and source apportionment of trace elements in multiple compartments in the lower reach of the Jinsha River, ChinaWenyan He0Fei Li1Jiang Yu2Min Chen3Yun Deng4Jia Li5Xiliang Tang6Zhuoyu Chen7Zhongluan Yan8State Key Laboratory of Hydraulics and Mountain River Engineering, College of Water Resource and Hydropower, Sichuan UniversityChangjiang Water Resources Protection InstituteChina Three Gorges Projects Development Co., Ltd,State Key Laboratory of Hydraulics and Mountain River Engineering, College of Water Resource and Hydropower, Sichuan UniversityState Key Laboratory of Hydraulics and Mountain River Engineering, College of Water Resource and Hydropower, Sichuan UniversityState Key Laboratory of Hydraulics and Mountain River Engineering, College of Water Resource and Hydropower, Sichuan UniversityChina Three Gorges Projects Development Co., Ltd,State Key Laboratory of Hydraulics and Mountain River Engineering, College of Water Resource and Hydropower, Sichuan UniversityChina Three Gorges Projects Development Co., Ltd,Abstract Studies on trace element (TE) pollution in abiotic matrices have typically focused on water, sediment, and soil, either separately or in pairs. The importance of multi-media connectivity has been ignored. This study analyzed the concentrations of 6 TEs in three connected environmental compartments of a 28-km section of the lower reach of the Jinsha River. The ecological risk posed by TEs was higher in soil than in sediment. The contribution of exposure pathways to human health risk were ranked as ingestion > dermal contact > inhalation. An improved regional environmental risk index (RERI) method was then developed to evaluate the comprehensive risk on both ecology and human health caused by TEs. The average RERI value was generally higher in the wet season (0.42) than in the dry (0.41) and dry-to-wet transition seasons (0.08) because of the combined effects of the high TE concentrations in riparian soil and the long exposure time. Source apportionment indicated that industrial activities, weathering of parent rock, and agricultural activities were possible sources of TEs in this region. The methods and results of this study could inform local environmental management and provide references for similar cases wherein multiple compartments of river systems should be considered.https://doi.org/10.1038/s41598-021-99626-w
collection DOAJ
language English
format Article
sources DOAJ
author Wenyan He
Fei Li
Jiang Yu
Min Chen
Yun Deng
Jia Li
Xiliang Tang
Zhuoyu Chen
Zhongluan Yan
spellingShingle Wenyan He
Fei Li
Jiang Yu
Min Chen
Yun Deng
Jia Li
Xiliang Tang
Zhuoyu Chen
Zhongluan Yan
Risk assessment and source apportionment of trace elements in multiple compartments in the lower reach of the Jinsha River, China
Scientific Reports
author_facet Wenyan He
Fei Li
Jiang Yu
Min Chen
Yun Deng
Jia Li
Xiliang Tang
Zhuoyu Chen
Zhongluan Yan
author_sort Wenyan He
title Risk assessment and source apportionment of trace elements in multiple compartments in the lower reach of the Jinsha River, China
title_short Risk assessment and source apportionment of trace elements in multiple compartments in the lower reach of the Jinsha River, China
title_full Risk assessment and source apportionment of trace elements in multiple compartments in the lower reach of the Jinsha River, China
title_fullStr Risk assessment and source apportionment of trace elements in multiple compartments in the lower reach of the Jinsha River, China
title_full_unstemmed Risk assessment and source apportionment of trace elements in multiple compartments in the lower reach of the Jinsha River, China
title_sort risk assessment and source apportionment of trace elements in multiple compartments in the lower reach of the jinsha river, china
publisher Nature Publishing Group
series Scientific Reports
issn 2045-2322
publishDate 2021-10-01
description Abstract Studies on trace element (TE) pollution in abiotic matrices have typically focused on water, sediment, and soil, either separately or in pairs. The importance of multi-media connectivity has been ignored. This study analyzed the concentrations of 6 TEs in three connected environmental compartments of a 28-km section of the lower reach of the Jinsha River. The ecological risk posed by TEs was higher in soil than in sediment. The contribution of exposure pathways to human health risk were ranked as ingestion > dermal contact > inhalation. An improved regional environmental risk index (RERI) method was then developed to evaluate the comprehensive risk on both ecology and human health caused by TEs. The average RERI value was generally higher in the wet season (0.42) than in the dry (0.41) and dry-to-wet transition seasons (0.08) because of the combined effects of the high TE concentrations in riparian soil and the long exposure time. Source apportionment indicated that industrial activities, weathering of parent rock, and agricultural activities were possible sources of TEs in this region. The methods and results of this study could inform local environmental management and provide references for similar cases wherein multiple compartments of river systems should be considered.
url https://doi.org/10.1038/s41598-021-99626-w
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