| Summary: | The passive radiative cooling approach refers to the physical process that pumps heat into outer space via the atmospheric window (8–13 μm) without energy input. The ability to continuously adjust the emissivity of thermal emitters in the sky window while maintaining high reflectivity in the solar spectrum remains a challenge. In order to achieve this task, a novel design referred to as double-layer nanoparticle-based coating is proposed. Our proposed emitter is appropriate for both high solar reflection and strong mid-infrared emissivity. The bottom and top layers are Al<sub>2</sub>O<sub>3</sub> embedded with Ni nanoparticles and a super-hydrophilic TiO<sub>2</sub>-SiO<sub>2</sub> layer. The bottom layer is designed to achieve high emissivity in “the atmospheric transparency window”. The top layer is designed to block solar illumination and to favor an enhanced cleanability of the coated design. Our double-layer coating as an optical solar reflector has excellent solar irradiation (<inline-formula><math xmlns="http://www.w3.org/1998/Math/MathML" display="inline"><semantics><mrow><mn>0.96</mn></mrow></semantics></math></inline-formula>) and is strongly emissive (0.97) across the “full sky window” at room temperature. Furthermore, a detailed numerical energy study has been performed, evaluating the temperature reduction and the radiative cooling performance under different conditions. The proposed simple coating can be used as an efficient radiative cooler on a large scale for energy conservation and thermoelectric devices.
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