Enhancement of UV Second-Harmonic Radiation at Nonlinear Interfaces with Discontinuous Second-order Susceptibilities

Abstract We investigate the generation of ultraviolet (UV) second-harmonic radiation at the boundary of a UV transparent crystal, which is derived from the automatic partial phase matching of the incident wave and the total internal reflection. By adhering to another UV non-transparent crystal with...

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Bibliographic Details
Main Authors: Xiaohui Zhao, Yuanlin Zheng, Ning An, Huaijin Ren, Xuewei Deng, Xianfeng Chen
Format: Article
Language:English
Published: Nature Publishing Group 2018-04-01
Series:Scientific Reports
Online Access:https://doi.org/10.1038/s41598-018-25041-3
Description
Summary:Abstract We investigate the generation of ultraviolet (UV) second-harmonic radiation at the boundary of a UV transparent crystal, which is derived from the automatic partial phase matching of the incident wave and the total internal reflection. By adhering to another UV non-transparent crystal with a larger second-order nonlinear coefficient χ (2), a nonlinear interface with large disparity in χ (2) is formed and the enhancement of UV second-harmonic radiation is observed experimentally. The intensity of enhanced second harmonic wave generated at the nonlinear interface is up to 11.6 times that at the crystal boundary. As a tunable phase-matching method, it may suggest potential applications in the UV, and even vacuum-UV region.
ISSN:2045-2322