Critical Current Density and Vortex Dynamics in Pristine and Irradiated KCa<sub>2</sub>Fe<sub>4</sub>As<sub>4</sub>F<sub>2</sub>

We report the critical current density (<i>J</i><sub>c</sub>) and vortex pinning properties in single crystals of a novel iron-based superconductor (IBS) KCa<sub>2</sub>Fe<sub>4</sub>As<sub>4</sub>F<sub>2</sub> with large <i&...

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Main Authors: Sunseng Pyon, Soichi Taya, Yuto Kobayashi, Ayumu Takahashi, Wenjie Li, Toshihiro Taen, Teng Wang, Gang Mu, Hisashi Kitamura, Ataru Ichinose, Tsuyoshi Tamegai
Format: Article
Language:English
Published: MDPI AG 2021-09-01
Series:Materials
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Online Access:https://www.mdpi.com/1996-1944/14/18/5283
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spelling doaj-179025acb972421e9f9d3720d68f02e62021-09-26T00:36:41ZengMDPI AGMaterials1996-19442021-09-01145283528310.3390/ma14185283Critical Current Density and Vortex Dynamics in Pristine and Irradiated KCa<sub>2</sub>Fe<sub>4</sub>As<sub>4</sub>F<sub>2</sub>Sunseng Pyon0Soichi Taya1Yuto Kobayashi2Ayumu Takahashi3Wenjie Li4Toshihiro Taen5Teng Wang6Gang Mu7Hisashi Kitamura8Ataru Ichinose9Tsuyoshi Tamegai10Department of Applied Physics, The University of Tokyo, 7-3-1 Hongo, Bunkyo-ku, Tokyo 113-8656, JapanDepartment of Applied Physics, The University of Tokyo, 7-3-1 Hongo, Bunkyo-ku, Tokyo 113-8656, JapanDepartment of Applied Physics, The University of Tokyo, 7-3-1 Hongo, Bunkyo-ku, Tokyo 113-8656, JapanDepartment of Applied Physics, The University of Tokyo, 7-3-1 Hongo, Bunkyo-ku, Tokyo 113-8656, JapanDepartment of Applied Physics, The University of Tokyo, 7-3-1 Hongo, Bunkyo-ku, Tokyo 113-8656, JapanInstitute for Solid State Physics, The University of Tokyo, Kashiwa 277-8581, JapanState Key Laboratory of Functional Materials for Informatics, Shanghai Institute of Microsystem and Information Technology, Chinese Academy of Sciences, Shanghai 200050, ChinaNational Institute of Radiological Sciences, National Institutes for Quantum and Radiological Science and Technology, Anagawa, Chiba-shi 263-8555, JapanCentral Research Institute of Electric Power Industry, Grid Innovation Research Laboratory, 2-6-1, Nagasaka, Yokosuka-shi 240-0196, JapanCentral Research Institute of Electric Power Industry, Grid Innovation Research Laboratory, 2-6-1, Nagasaka, Yokosuka-shi 240-0196, JapanDepartment of Applied Physics, The University of Tokyo, 7-3-1 Hongo, Bunkyo-ku, Tokyo 113-8656, JapanWe report the critical current density (<i>J</i><sub>c</sub>) and vortex pinning properties in single crystals of a novel iron-based superconductor (IBS) KCa<sub>2</sub>Fe<sub>4</sub>As<sub>4</sub>F<sub>2</sub> with large <i>J</i><sub>c</sub> in the pristine state, before and after introduction of artificial defects by swift-particle irradiation. The effects of 2.6 GeV U and 3 MeV proton irradiations in KCa<sub>2</sub>Fe<sub>4</sub>As<sub>4</sub>F<sub>2</sub> single crystals on transition temperature <i>T</i><sub>c</sub> and <i>J</i><sub>c</sub>, including its dose dependence, are systematically studied. <i>J</i><sub>c</sub>~8 MA/cm<sup>2</sup> under a self-field at 2 K in the pristine crystal is strongly enhanced up to 19.4 and 17.5 MA/cm<sup>2</sup> by irradiation of 2.6 GeV U-ions and 3 MeV protons, respectively. Suppression of <i>T</i><sub>c</sub> and dose dependence of <i>J</i><sub>c</sub> in KCa<sub>2</sub>Fe<sub>4</sub>As<sub>4</sub>F<sub>2</sub> is different from that in a representative IBS of (Ba,K)Fe<sub>2</sub>As<sub>2</sub>, which can be explained by considering the presence of embedded defects in pristine KCa<sub>2</sub>Fe<sub>4</sub>As<sub>4</sub>F<sub>2</sub>. The vortex dynamics in the pristine and proton irradiated KCa<sub>2</sub>Fe<sub>4</sub>As<sub>4</sub>F<sub>2</sub> single crystals are also investigated from the analyses of the field dependence of <i>J</i><sub>c</sub> and the normalized magnetic relaxation rate. In addition to the contribution of embedded defects, weak collective pinning is considered for comprehensive analyses. Vortex dynamics in KCa<sub>2</sub>Fe<sub>4</sub>As<sub>4</sub>F<sub>2</sub> is similar to those in (Ba,K)Fe<sub>2</sub>As<sub>2</sub> to some extent, and different from that in anisotropic Li<sub>0.8</sub>Fe<sub>0.2</sub>OHFeSe. Large anisotropy, due to the presence of insulating blocking layers in KCa<sub>2</sub>Fe<sub>4</sub>As<sub>4</sub>F<sub>2</sub>, which leads to much lower irreversibility field (<i>H</i><sub>irr</sub>) compared with 122-type IBSs, strongly affect the vortex dynamics.https://www.mdpi.com/1996-1944/14/18/5283iron-based superconductors (IBS)vortex dynamicsion irradiationKCa<sub>2</sub>Fe<sub>4</sub>As<sub>4</sub>F<sub>2</sub>
collection DOAJ
language English
format Article
sources DOAJ
author Sunseng Pyon
Soichi Taya
Yuto Kobayashi
Ayumu Takahashi
Wenjie Li
Toshihiro Taen
Teng Wang
Gang Mu
Hisashi Kitamura
Ataru Ichinose
Tsuyoshi Tamegai
spellingShingle Sunseng Pyon
Soichi Taya
Yuto Kobayashi
Ayumu Takahashi
Wenjie Li
Toshihiro Taen
Teng Wang
Gang Mu
Hisashi Kitamura
Ataru Ichinose
Tsuyoshi Tamegai
Critical Current Density and Vortex Dynamics in Pristine and Irradiated KCa<sub>2</sub>Fe<sub>4</sub>As<sub>4</sub>F<sub>2</sub>
Materials
iron-based superconductors (IBS)
vortex dynamics
ion irradiation
KCa<sub>2</sub>Fe<sub>4</sub>As<sub>4</sub>F<sub>2</sub>
author_facet Sunseng Pyon
Soichi Taya
Yuto Kobayashi
Ayumu Takahashi
Wenjie Li
Toshihiro Taen
Teng Wang
Gang Mu
Hisashi Kitamura
Ataru Ichinose
Tsuyoshi Tamegai
author_sort Sunseng Pyon
title Critical Current Density and Vortex Dynamics in Pristine and Irradiated KCa<sub>2</sub>Fe<sub>4</sub>As<sub>4</sub>F<sub>2</sub>
title_short Critical Current Density and Vortex Dynamics in Pristine and Irradiated KCa<sub>2</sub>Fe<sub>4</sub>As<sub>4</sub>F<sub>2</sub>
title_full Critical Current Density and Vortex Dynamics in Pristine and Irradiated KCa<sub>2</sub>Fe<sub>4</sub>As<sub>4</sub>F<sub>2</sub>
title_fullStr Critical Current Density and Vortex Dynamics in Pristine and Irradiated KCa<sub>2</sub>Fe<sub>4</sub>As<sub>4</sub>F<sub>2</sub>
title_full_unstemmed Critical Current Density and Vortex Dynamics in Pristine and Irradiated KCa<sub>2</sub>Fe<sub>4</sub>As<sub>4</sub>F<sub>2</sub>
title_sort critical current density and vortex dynamics in pristine and irradiated kca<sub>2</sub>fe<sub>4</sub>as<sub>4</sub>f<sub>2</sub>
publisher MDPI AG
series Materials
issn 1996-1944
publishDate 2021-09-01
description We report the critical current density (<i>J</i><sub>c</sub>) and vortex pinning properties in single crystals of a novel iron-based superconductor (IBS) KCa<sub>2</sub>Fe<sub>4</sub>As<sub>4</sub>F<sub>2</sub> with large <i>J</i><sub>c</sub> in the pristine state, before and after introduction of artificial defects by swift-particle irradiation. The effects of 2.6 GeV U and 3 MeV proton irradiations in KCa<sub>2</sub>Fe<sub>4</sub>As<sub>4</sub>F<sub>2</sub> single crystals on transition temperature <i>T</i><sub>c</sub> and <i>J</i><sub>c</sub>, including its dose dependence, are systematically studied. <i>J</i><sub>c</sub>~8 MA/cm<sup>2</sup> under a self-field at 2 K in the pristine crystal is strongly enhanced up to 19.4 and 17.5 MA/cm<sup>2</sup> by irradiation of 2.6 GeV U-ions and 3 MeV protons, respectively. Suppression of <i>T</i><sub>c</sub> and dose dependence of <i>J</i><sub>c</sub> in KCa<sub>2</sub>Fe<sub>4</sub>As<sub>4</sub>F<sub>2</sub> is different from that in a representative IBS of (Ba,K)Fe<sub>2</sub>As<sub>2</sub>, which can be explained by considering the presence of embedded defects in pristine KCa<sub>2</sub>Fe<sub>4</sub>As<sub>4</sub>F<sub>2</sub>. The vortex dynamics in the pristine and proton irradiated KCa<sub>2</sub>Fe<sub>4</sub>As<sub>4</sub>F<sub>2</sub> single crystals are also investigated from the analyses of the field dependence of <i>J</i><sub>c</sub> and the normalized magnetic relaxation rate. In addition to the contribution of embedded defects, weak collective pinning is considered for comprehensive analyses. Vortex dynamics in KCa<sub>2</sub>Fe<sub>4</sub>As<sub>4</sub>F<sub>2</sub> is similar to those in (Ba,K)Fe<sub>2</sub>As<sub>2</sub> to some extent, and different from that in anisotropic Li<sub>0.8</sub>Fe<sub>0.2</sub>OHFeSe. Large anisotropy, due to the presence of insulating blocking layers in KCa<sub>2</sub>Fe<sub>4</sub>As<sub>4</sub>F<sub>2</sub>, which leads to much lower irreversibility field (<i>H</i><sub>irr</sub>) compared with 122-type IBSs, strongly affect the vortex dynamics.
topic iron-based superconductors (IBS)
vortex dynamics
ion irradiation
KCa<sub>2</sub>Fe<sub>4</sub>As<sub>4</sub>F<sub>2</sub>
url https://www.mdpi.com/1996-1944/14/18/5283
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